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We present a general formulation to calculate the dynamic optical conductivity, beyond the linear response regime, of any electronic system whose quasiparticle dispersion is described by a two band model. Our phenomenological model is based…

Mesoscale and Nanoscale Physics · Physics 2017-04-19 Ashutosh Singh , Tuhina Satpati , Kirill I. Bolotin , Saikat Ghosh , Amit Agarwal

Quadratic Lindbladians encompass a rich class of dissipative electronic and bosonic quantum systems, which have been predicted to host new and exotic physics. In this study, we develop a Lindblad-Keldysh spectroscopic response formalism for…

Mesoscale and Nanoscale Physics · Physics 2026-01-22 Spenser Talkington , Martin Claassen

We compute the nonlinear optical response of doped mono- and bilayer graphene using the full dispersion based on tight-binding models. The response is derived with the density matrix formalism using the length gauge and is valid for any…

Mesoscale and Nanoscale Physics · Physics 2018-12-05 F. Hipolito , Alireza Taghizadeh , T. G. Pedersen

Two-dimensional materials constitute an exciting platform for nonlinear optics with large nonlinearities that are tunable by gating. Hence, gate-tunable harmonic generation and intensity-dependent refraction have been observed in e.g.…

Mesoscale and Nanoscale Physics · Physics 2019-05-15 F. Hipolito , Darko Dimitrovski , T. G. Pedersen

In this work, the difficulties inherent to perturbative calculations in the velocity gauge are addressed. In particular, it is shown how calculations of nonlinear optical responses in the independent particle approximation can be done to…

Using an enhanced optically heterodyned optical Kerr effect method and a theoretical description of the interactions between an optical beam, a single layer of graphene, and its substrate, we provide experimental answers to questions raised…

Optics · Physics 2017-12-20 Evdokia Dremetsika , Pascal Kockaert

We present a method, based on noncollinear second harmonic generation, to evaluate the non-zero elements of the nonlinear optical susceptibility. At a fixed incidence angle, the generated signal is investigated by varying the polarization…

We demonstrate the power of a first principle-based and practicable method that allows for the perturbative computation of reduced density matrix elements of an open quantum system without making use of any master equations. The approach is…

High Energy Physics - Theory · Physics 2023-06-12 Christian Käding , Mario Pitschmann

We present a formulation for the nonlinear optical response in gapped graphene, where the low-energy single-particle spectrum is modeled by massive Dirac theory. As a representative example of the formulation presented here, we obtain…

Strongly Correlated Electrons · Physics 2012-05-30 S. A. Jafari

We adapted a recently proposed framework to characterize the optical response of interacting electrons in solids in order to expedite its computation without compromise in accuracy at the microscopic level. Our formulation is based on…

Materials Science · Physics 2021-03-02 Emilia Ridolfi , Paolo E. Trevisanutto , Vitor M. Pereira

We establish a steady-state theory for nonlinear optical conductivity in pseudo-Hermitian systems. We derive compact formulas for the first and second order conductivity tensors in both the velocity and length gauges and prove their exact…

Mesoscale and Nanoscale Physics · Physics 2025-10-09 S. Sajad Dabiri , Reza Asgari

We develop a non-perturbative formulation based on the Green-function quantization method, that can describe spontaneous parametric down-conversion in the high-gain regime in nonlinear optical structures with arbitrary amount of loss and…

Quantum Physics · Physics 2023-12-13 Aleksa Krstić , Frank Setzpfandt , Sina Saravi

An $\it{ab \,\, initio}$ based fully microscopic approach is applied to study the nonlinear optical response of bulk Tellurium. The structural and electronic properties are calculated from first principles using the shLDA-1/2 method within…

Optics · Physics 2021-08-20 S. C. Liebscher , M. K. Hagen , J. Hader , J. V. Moloney , S. W. Koch

An adaptive scheme to generate reduced-order models for parametric nonlinear dynamical systems is proposed. It aims to automatize the POD-Greedy algorithm combined with empirical interpolation. At each iteration, it is able to adaptively…

Numerical Analysis · Mathematics 2021-10-13 Sridhar Chellappa , Lihong Feng , Peter Benner

Coherent nonlinear optical micro-spectroscopy is a frequently used tool in modern material science, as it is sensitive to many different local observables, which comprise, among others, crystal symmetry and vibrational properties. The…

Optics · Physics 2023-04-12 Kai J. Spychala , Zeeshan H. Amber , Lukas M. Eng , Michael Rüsing

Nonequilibrium quantum mechanics can be solved with the Keldysh formalism, which evolves the quantum mechanical states forward in time in the presence of a time-dependent field, and then evolves them backward in time, undoing the effect of…

Strongly Correlated Electrons · Physics 2007-05-23 J. K. Freericks , V. Turkowski , V. Zlatic

We introduce a numerical variational method based on the Rayleigh-Ritz optimization principle for predicting two-dimensional self-trapped beams in nonlinear media. This technique overcomes the limitation of the traditional variational…

Optics · Physics 2018-04-04 Erick I. Duque , Servando Lopez-Aguayo , Boris A. Malomed

We introduce a new numerical strategy to solve a class of oscillatory transport PDE models which is able to captureaccurately the solutions without numerically resolving the high frequency oscillations {\em in both space and time}.Such PDE…

Numerical Analysis · Mathematics 2016-06-01 Nicolas Crouseilles , Shi Jin , Mohammed Lemou

Nonperturbative approach based on exact solution of Boltzmann kinetic equation in the relaxation time approximation is developed for the study of nonlinear response of electron-doped few-layer graphene to a high-frequency electromagnetic…

Mesoscale and Nanoscale Physics · Physics 2020-03-06 D. V. Fil

We propose a novel and systematic recurrence method for the energy spectra of non-Hermitian systems under open boundary conditions based on the recurrence relations of their characteristic polynomials. Our formalism exhibits better accuracy…

Mesoscale and Nanoscale Physics · Physics 2025-04-16 Haoyan Chen , Yi Zhang
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