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We address the long-standing problem of the microscopic origin of the richly diverse phenomena in the chromium breathing pyrochlore material family. Combining electronic structure and renormalization group techniques we resolve the magnetic…

We study the antiferromagnetic {\it XY} model on a triangular lattice by extensive Monte Carlo simulations, focusing on its ordering and critical properties. Our result clearly shows that two separate transitions occur at two distinct…

Statistical Mechanics · Physics 2012-05-31 Tomoyuki Obuchi , Hikaru Kawamura

We present a general framework for deriving effective spin Hamiltonians of correlated magnetic systems based on a combination of relativistic ab initio density functional theory calculations (DFT), exact diagonalization of a generalized…

Strongly Correlated Electrons · Physics 2016-07-13 Kira Riedl , Daniel Guterding , Harald O. Jeschke , Michel J. P. Gingras , Roser Valenti

Pyrochlore oxides show several fascinating phenomena, such as the formation of heavy fermions and the thermal Hall effect. Although a key to understanding some phenomena may be the Dzyaloshinsky-Moriya (DM) interaction, its microscopic…

Strongly Correlated Electrons · Physics 2016-10-26 Naoya Arakawa

A possibility of the uniform antiferromagnetic order is pointed out in an S=1/2 ferromagnetic (F) - antiferromagnetic (AF) random alternating Heisenberg quantum spin chain compound: (CH_3)_2 CHNH_3 Cu(Cl_x Br_{1-x})_3. The system possesses…

Statistical Mechanics · Physics 2009-11-07 Tota Nakamura

We investigate the magnetic behavior and critical exponents of quaternary CoFeV$_{0.8}$Mn$_{0.2}$Si Heusler alloy to understand the interactions across the Curie temperature ($T_{\rm C}$). The Rietveld refinement of the x-ray diffraction…

Materials Science · Physics 2023-10-04 Guru Dutt Gupt , P. D. Babu , R. S. Dhaka

We present the first study of a magnetic quantum phase transition in the itinerant-electron ferromagnet Ni3Al at high pressures. Electrical resistivity measurements in a diamond anvil cell at hydrostatic pressures up to 100 kbar and…

Strongly Correlated Electrons · Physics 2007-05-23 P. G. Niklowitz , F. Beckers , G. G. Lonzarich , G. Knebel , B. Salce , J. Thomasson , N. Bernhoeft , D. Braithwaite , J. Flouquet

CuSiO_3, isotypic to the spin - Peierls compound CuGeO_3, was discovered recently as a metastable decomposition product of the silicate mineral dioptase, Cu_6Si_6O_{18}\cdot6H_2O. We investigated the physical properties of CuSiO_3 using…

Strongly Correlated Electrons · Physics 2009-10-31 M. Baenitz , C. Geibel , M. Dischner , G. Sparn , F. Steglich , H. H. Otto , M. Meibohm , A. A. Gippius

The pyrochlore lattice Heisenberg antiferromagnet has a massive classical ground state degeneracy. We summarize three approximation schemes, valid for large spin length $S$, to capture the (partial) lifting of this degeneracy when…

Strongly Correlated Electrons · Physics 2015-06-25 Uzi Hizi , Christopher L. Henley

The effective quantum pseudospin-1/2 model for interacting rare-earth magnetic moments, which are locally described with atomic doublets, is studied theoretically for magnetic pyrochlore oxides. It is derived microscopically for localized…

Strongly Correlated Electrons · Physics 2015-03-17 Shigeki Onoda , Yoichi Tanaka

The very low temperature properties of two pyrochlore compounds, Yb2Ti2O7 and Gd2Sn2O7, were investigated using an ensemble of microscopic and bulk techniques. In both compounds, a first order transition is evidenced, as well as spin…

We report the synthesis, structure, and magnetic and transport properties of a new ternary intermetallic compound PrRhSn3 which crystallizes in LaRuSn3-type cubic structure (space group Pm-3n). At low applied fields the dc magnetic…

Strongly Correlated Electrons · Physics 2014-07-22 V. K. Anand , D. T. Adroja , A. D. Hillier

Spin-singlet orders are studied for the antiferromagnetic Heisenberg model with spin $S$>1/2 on a breathing pyrochlore lattice, where tetrahedron units are weakly coupled and exchange constants have two values $0<J' \ll J$. The ground state…

Strongly Correlated Electrons · Physics 2017-02-16 Hirokazu Tsunetsugu

Iron sesquioxide (Fe2O3) displays pressure and temperature induced spin and structural transitions. Our calculations show that, density functional theory (DFT), in the generalized gradient approximation (GGA) scheme, is capable of capturing…

Materials Science · Physics 2009-05-22 Dipta Bhanu Ghosh , Stefano de Gironcoli

The spin order in cubic perovskite SrFeO3 and BaFeO3 under high pressure is studied by density functional theory (DFT) calculation with local spin density approximation plus Hubbard U (LSDA+U). At ambient pressure, A-type and G-type helical…

Strongly Correlated Electrons · Physics 2015-06-11 Zhi Li , Toshiaki Iitaka , Takami Tohyama

We investigate the nature of phase transitions induced by Dzyaloshinskii-Moriya (DM) interactions on a classical pyrochlore antiferromagnet. For both symmetry-allowed antisymmetric exchange interactions, the macroscopic degeneracy due to…

Strongly Correlated Electrons · Physics 2010-08-19 Gia-Wei Chern

For disordered Heisenberg systems with small single ion anisotropy, two spin glass transitions below the long range ordered phase transition temperature has been predicted theoretically for compositions close to the percolation threshold.…

Materials Science · Physics 2018-03-13 Arun Kumar , S. D. Kaushik , V. Siruguri , Dhananjai Pandey

The (three-dimensional) pyrochlore lattice antiferromagnet with Heisenberg spins of large spin length $S$ is a highly frustrated model with an macroscopic degeneracy of classical ground states. The zero-point energy of (harmonic order) spin…

Strongly Correlated Electrons · Physics 2009-11-11 Christopher L. Henley

We report the low temperature magnetic properties of the pyrochlore Pr$_2$Hf$_2$O$_7$. Polycrystalline and single-crystal samples are investigated using time-of-flight neutron spectroscopy and macroscopic measurements, respectively. The…

We study the ground state and thermodynamic properties of the spin-half XXZ model, with an Ising interaction $J_z$ and a transverse exchange interaction $J_{x}$, on a pyrochlore tube obtained by joining together elementary cubes in a…

Strongly Correlated Electrons · Physics 2022-08-31 Chunhan Feng , Alexander Wietek , E. Miles Stoudenmire , Rajiv R. P. Singh