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We present a novel optical transient absorption and reflection microscope based on a diffraction-limited pump pulse in combination with a wide-field probe pulse, for the spatio-temporal investigation of ultrafast population transport in…

We examine electron-electron mediated relaxation following excitation of a correlated system by an ultrafast electric field pump pulse. The results reveal a dichotomy in the temporal evolution as one tunes through a Mott metal-to-insulator…

Strongly Correlated Electrons · Physics 2013-08-20 B. Moritz , A. F. Kemper , M. Sentef , T. P. Devereaux , J. K. Freericks

Ultracold atom magnetic field microscopy enables the probing of current flow patterns in planar structures with unprecedented sensitivity. In polycrystalline metal (gold) films we observe long-range correlations forming organized patterns…

Materials Science · Physics 2008-03-08 S. Aigner , L. Della Pietra , Y. Japha , O. Entin-Wohlman , T. David , R. Salem , R. Folman , J. Schmiedmayer

Ultrafast electron diffraction (UED) is a powerful method for studying time-resolved structural changes. Currently, space charge induced temporal broadening prevents obtaining high brightness electron pulses with sub-100 fs durations…

Instrumentation and Detectors · Physics 2013-10-29 Yihua Wang , Nuh Gedik

The element specificity of soft X-ray spectroscopy makes it an ideal tool for analyzing the microscopic origin of ultrafast dynamics induced by localized optical excitation in metal-insulator heterostructures. Using [Fe/MgO]$_n$ as a model…

The motion of electrons in or near solids, liquids and gases can be tracked by forcing their ejection with attosecond x-ray pulses, derived from femtosecond lasers. The momentum of these emitted electrons carries the imprint of the…

Mesoscale and Nanoscale Physics · Physics 2017-06-14 C. W. Barlow-Myers , N. J. Pine , W. A. Bryan

Quantitative knowledge of electron-phonon coupling is important for many applications as well as for the fundamental understanding of nonequilibrium relaxation processes. Time-resolved diffraction provides direct access to this knowledge…

Materials Science · Physics 2021-11-18 Daniela Zahn , Hélène Seiler , Yoav William Windsor , Ralph Ernstorfer

The advent of pump-probe spectroscopy techniques paved the way to the exploration of the ultrafast dynamics of electrons and phonons in crystalline solids. Following photo-absorption of a pump pulse and the initial electronic…

Materials Science · Physics 2023-07-14 Fabio Caruso , Dino Novko

We demonstrate that the dispersion of surface plasmon polaritons in a periodically perforated gold film can be efficiently manipulated by femtosecond laser pulses with the wavelengths far from the intrinsic resonances of gold. Using a time-…

In ultrafast electron diffraction (UED) experiments, accurate retrieval of time-resolved structural parameters, such as atomic coordinates and thermal displacement parameters, requires an accurate scattering model. Unfortunately,…

Materials Science · Physics 2023-01-03 Daniel B. Durham , Colin Ophus , Khalid M. Siddiqui , Andrew M. Minor , Daniele Filippetto

We study the ultrafast structural dynamics, in response to electronic excitations, in heterostructures composed of Au$_{923}$ nanoclusters on thin-film substrates with the use of femtosecond electron diffraction. Various forms of atomic…

Metallic nanostructures can support so-called plasma oscillations (plasmons). Plasmons allow for the concentration of the energy from light, down to sizes well below the conventional diffraction limit known from optics. Plasmonics thus…

Mesoscale and Nanoscale Physics · Physics 2019-06-05 Christian Frydendahl

Ultrafast processes in matter, such as the electron emission following light absorption, can now be studied using ultrashort light pulses of attosecond duration ($10^{-18}$s) in the extreme ultraviolet spectral range. The lack of spectral…

Quantum material systems upon applying ultrashort laser pulses provide a rich platform to access excited material phases and their transformations that are not entirely like their equilibrium counterparts. The addressability and potential…

Strongly Correlated Electrons · Physics 2021-08-19 Xiaoyi Sun , Shuaishuai Sun , Chong-Yu Ruan

Intense ultrashort laser pulse irradiation of solid targets was systematically investigated at the first-principles level, both theoretically and computationally. In the method, the propagation of a pulsed light through a thin film is…

Optics · Physics 2024-01-25 Atsushi Yamada , Kazuhiro Yabana

Efficient thermal management is essential for the reliability of modern power electronics, where increasing device density leads to severe heat dissipation challenges. However, in thin-film systems, thermal transport is often compromised by…

Rapid modulation of the electromagnetic response in both time and space creates temporal boundaries in the medium and leads to time-reflection and time-refraction of light and to the eventual formation of the photonic time crystal within…

Optics · Physics 2024-10-01 Evgenii E. Narimanov

Dispersion decomposes compound light into monochromatic components at different spatial locations, which needs to be eliminated in imaging but utilized in spectral detection. Metasurfaces provide a unique path to modulate the dispersion…

Optics · Physics 2021-12-30 Yueqiang Hu , Yuting Jiang , Yi Zhang , Jiajie Lai , Peng He , Xiangnian Ou , Ling Li , Huigao Duan

The ability to modulate light at high speeds is of paramount importance for telecommunications, information processing, and medical imaging technologies. This has stimulated intense efforts to master optoelectronic switching at visible and…

Mesoscale and Nanoscale Physics · Physics 2014-04-01 A. Manjavacas , F. J. Garcia de Abajo

The temperature dependence of ultrafast photoinduced reflectivity transients is reported in Nd$_{0.5}$Sr$_{0.5}$MnO$_{3}$ thin film. The photoinduced reflectivity shows a complex response with very different temperature dependences on…

Condensed Matter · Physics 2009-11-10 T. Mertelj , D. Mihailovic , Z. Jagličič , A. A. Bosak , O. Yu. Gorbenko , A. R. Kaul
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