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Related papers: Phase behaviour in ionic solutions: restricted pri…

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Employing simplified models in computer simulation is on the one hand often enforced by computer time limitations but on the other hand it offers insights into the molecular properties determining a given physical phenomenon. We employ this…

Statistical Mechanics · Physics 2008-04-18 Bortolo Matteo Mognetti , Martin Oettel , Leonid Yelash , Peter Virnau , Wolfgang Paul , Kurt Binder

The analytic equation of state of nonideal Coulomb plasmas consisting of pointlike ions immersed in a polarizable electron background (physics/9807042) is improved, and its applicability range is considerably extended. First, the fit of the…

Astrophysics · Physics 2008-11-26 A. Y. Potekhin , G. Chabrier

We propose a new coarse-grained model for the description of liquid-vapor phase separation of colloid-polymer mixtures. The hard-sphere repulsion between colloids and between colloids and polymers, which is used in the well-known…

Soft Condensed Matter · Physics 2009-11-13 Jochen Zausch , Peter Virnau , Kurt Binder , Juergen Horbach , Richard L. Vink

Coupled cluster theory provides hierarchical many-particle models and is presently considered as the ultimate benchmark in quantum chemistry. Despite is practical significance, a rigorous mathematical analysis of its properties is still in…

Mathematical Physics · Physics 2018-01-24 Heinz-Jürgen Flad , Gohar Flad-Harutyunyan

A robust method to handle vacuum and near vacuum regions in hybrid simulations for space and astrophysical plasmas is presented. The conventional hybrid simulation model dealing with kinetic ions and a massless charge-neutralizing electron…

Plasma Physics · Physics 2015-06-22 Takanobu Amano , Katsuaki Higashimori , Keisuke Shirakawa

The phase behavior of the lattice restricted primitive model (RPM) for ionic systems with additional short-range nearest neighbor (nn) repulsive interactions has been studied by grand canonical Monte Carlo simulations. We obtain a rich…

Soft Condensed Matter · Physics 2009-11-10 Alexandre Diehl , Athanassios Z. Panagiotopoulos

Phase separation and criticality are analyzed in $z$:1 charge-asymmetric ionic fluids of equisized hard spheres by generalizing the Debye-H\"{u}ckel approach combined with ionic association, cluster solvation by charged ions, and hard-core…

Statistical Mechanics · Physics 2009-11-10 Jean-Noel Aqua , Shubho Banerjee , Michael E. Fisher

Structural and thermodynamic properties of ionic fluids are related to those of a simpler ``mimic'' system with short ranged intermolecular interactions in a spatially varying effective field by use of Local Molecular Field (LMF) theory,…

Statistical Mechanics · Physics 2007-05-23 Yng-gwei Chen , Charanbir Kaur , John D. Weeks

We study collective modes in a classical system of particles with repulsive inverse-power-law (IPL) interactions in the fluid phase, near the fluid-solid coexistence (IPL melts). The IPL exponent is varied from $n=10$ to $n=100$ to mimic…

Soft Condensed Matter · Physics 2017-08-17 Sergey Khrapak , Boris Klumov , Lenaic Couedel

We study fluid structure and water-like anomalies of a system constituted by dimeric particles interacting via a purely repulsive core-softened potential by means of integral equation theories. In our model, dimers interact through a…

Soft Condensed Matter · Physics 2017-03-08 Gianmarco Munaò , Franz Saija

We present a new method to obtain interaction part of a model Hamiltonian from the result of the first-principles calculation. The effective interaction contained in the model is determined based on the random phase approximation (RPA). In…

Materials Science · Physics 2017-04-26 Hirofumi Sakakibara , Seung Woo Jang , Hiori Kino , Myung Joon Han , Kazuhiko Kuroki , Takao Kotani

The Asakura-Oosawa model for colloid-polymer mixtures is studied by Monte Carlo simulations at densities inside the two-phase coexistence region of fluid and solid. Choosing a geometry where the system is confined between two flat walls,…

Soft Condensed Matter · Physics 2015-06-04 Debabrata Deb , Alexander Winkler , Peter Virnau , Kurt Binder

This paper is Part II of a two-part series on coexistence states study in stochastic generalized Kolmogorov systems under small diffusion. Part I provided a complete characterization for approximating invariant probability measures and…

Dynamical Systems · Mathematics 2024-07-16 Baoquan Zhou , Hao Wang , Tianxu Wang , Daqing Jiang

Using the Deep Potential methodology, we construct a model that reproduces accurately the potential energy surface of the SCAN approximation of density functional theory for water, from low temperature and pressure to about 2400 K and 50…

Chemical Physics · Physics 2021-06-16 Linfeng Zhang , Han Wang , Roberto Car , Weinan E

Integral equation theory calculations within the mean spherical approximation (MSA) and grand canonical Monte Carlo (MC) simulations are employed to study the phase behaviour of a symmetrical binary fluid mixture in the presence of a field…

Statistical Mechanics · Physics 2009-11-11 Juergen Koefinger , Gerhard Kahl , Nigel B. Wilding

Practical applications of fragment embedding and closely related local correlation methods critically depend on a judicious choice of a low-level theory to define the local embedding subspace and to capture long-range electrostatic and…

Chemical Physics · Physics 2026-05-14 Ruiheng Song , Xiliang Gong , Aamy Bakry , Hong-Zhou Ye

We develop and implement a formalism which enables calculating the analytical gradients of particle-hole random-phase approximation (RPA) ground-state energy with respect to the atomic positions within the atomic orbital basis set…

Chemical Physics · Physics 2021-09-03 Muhammad N. Tahir , Tong Zhu , Honghui Shang , Jia Li , Volker Blum , Xinguo Ren

We present a new method for modeling disordered solid solutions, based on the virtual crystal approximation (VCA). The VCA is a tractable way of studying configurationally disordered systems; traditionally, the potentials which represent…

Materials Science · Physics 2009-10-31 Nicholas J. Ramer , Andrew M. Rappe

We have investigated the phase transition of the gas-liquid type, with an upper critical point, in a variant of the One Component Plasma model (OCP) that has a uniform but compressible compensating background. We have calculated the…

Plasma Physics · Physics 2009-03-27 Igor Iosilevskiy

The Linear Mixing Approximation (LMA) is often used in planetary models for calculating the equations of state (EoSs) of mixtures. A commonly assumed planetary composition is a mixture of rock and water. Here we assess the accuracy of the…

Earth and Planetary Astrophysics · Physics 2024-11-27 Valiantsin Darafeyeu , Stephanie Rimle , Guglielmo Mazzola , Ravit Helled