Related papers: Turning a molecule into a coherent two-level quant…
The pioneering experiments of linear spectroscopy were performed using flames in the 1800s, but nonlinear optical measurements had to wait until lasers became available in the twentieth century. Because the nonlinear cross section of…
Organic dye molecules have been used in great many scientific and technological applications, but their wider use in quantum optics has been hampered by transitions to short-lived vibrational levels, which limit their coherence properties.…
Photonic molecules - particular systems composed of coupled optical resonators - emulate the behavior of complex physical systems exhibiting discrete energy levels. In this work, we present a novel photonic molecule composed of two strongly…
Physical systems with discrete energy levels are ubiquitous in nature and are fundamental building blocks of quantum technology. Realizing controllable artifcial atom- and molecule-like systems for light would allow for coherent and dynamic…
Intense light-matter interaction largely relies on the use of high-power light sources, creating fields comparable to, or even stronger than, the field keeping the electrons bound in atoms. Under such conditions, the interaction induces…
A quantum emitter interacting with photons in a single optical-mode constitutes a one-dimensional atom. A coherent and efficiently coupled one-dimensional atom provides a large nonlinearity, enabling photonic quantum gates. Achieving a high…
Isolating single molecules in the solid state has allowed fundamental experiments in basic and applied sciences. When cooled down to liquid helium temperature, certain molecules show transition lines, that are tens of megahertz wide,…
Photonic molecules, named by analogy with chemical molecules, are clusters of closely located electromagnetically interacting microcavities or "photonic atoms". As two or several microcavities are brought close together, their optical modes…
Semiconductor microcavities with artificial single-photon emitters have become one of the backbones of semiconductor quantum optics. In many cases however, technical and physical issues limit the study of optical fields to incoherently…
Molecular complexes are held together via a variety of bonds, but they all share the common feature that their individual entities are in contact. In this work, we introduce and demonstrate the concept of a \textit{molecular optical bond},…
This chapter reviews the fundamental optical properties and applications of pho-tonic molecules (PMs) - photonic structures formed by electromagnetic coupling of two or more optical microcavities (photonic atoms). Controllable interaction…
Linear optics quantum computing (LOQC) is a leading candidate for the implementation of large scale quantum computers. Here quantum information is encoded into the quantum states of light and computation proceeds via a linear optics…
The generation and control of entanglement in a quantum mechanical system is a critical element of nearly all quantum applications. Molecular systems are a promising candidate, with numerous degrees of freedom able to be targeted. However,…
Two-level emitters constitute main building blocks of photonic quantum systems and are model systems for the exploration of quantum optics in the solid state. Most interesting is the strict-resonant excitation of such emitters to generate…
Quantum optics has been a major driving force behind the rapid experimental developments that have led from the first laser cooling schemes to the Bose-Einstein condensation (BEC) of dilute atomic and molecular gases. Not only has it…
A functioning quantum computer will be a machine that builds up, in a programmable way, nonclassical correlations in a multipartite quantum system. Linear optics quantum computation (LOQC) is an approach for achieving this function that…
The extraordinary success in laser cooling, trapping, and coherent manipulation of atoms has energized the efforts in extending this exquisite control to molecules. Not only are molecules ubiquitous in nature, but the control of their…
Enhancing optical nonlinearities so that they become appreciable on the single photon level and lead to nonclassical light fields has been a central objective in quantum optics for many years. After this has been achieved in individual…
Under appropriate conditions, superconducting electronic circuits behave quantum mechanically, with properties that can be designed and controlled at will. We have realized an experiment in which a superconducting two-level system, playing…
An array of radiatively coupled emitters is an exciting new platform for generating, storing, and manipulating quantum light. However, the simultaneous positioning and tuning of multiple lifetime-limited emitters into resonance remains a…