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Neutron diffraction and nuclear quadrupole resonance (NQR) measurements were employed to investigate magnetic order in the non-ferroelectric phase preceding the low-temperature multiferroic state in FeTe2O5Br. Refnement of the neutron…

Strongly Correlated Electrons · Physics 2013-04-10 M. Pregelj , P. Jeglič , A. Zorko , O. Zaharko , T. Apih , A. Gradišek , M. Komelj , H. Berger , D. Arčon

Alkali superoxides differ from conventional transition metal magnets, exhibit magnetism from partially occupied oxygen molecular $\pi^*$-orbitals. Among them, CsO$_2$ stands out for its potential to exhibit novel quantum collective…

Strongly Correlated Electrons · Physics 2024-11-12 Ryota Ono , Ravi Kaushik , Sergey Artyukhin , Martin Jansen , Igor Solovyev , Russell A. Ewings

By performing accurate ab-initio density functional theory calculations, we study the role of $4f$ electrons in stabilizing the magnetic-field-induced ferroelectric state of DyFeO$_{3}$. We confirm that the ferroelectric polarization is…

Materials Science · Physics 2015-05-14 Alessandro Stroppa , Martijn Marsman , Georg Kresse , Silvia Picozzi

We report the results of our investigation of magnetic, thermodynamic and dielectric properties of Ca substituted half-doped orthochromite, Dy0.6Ca0.4Fe0.5Cr0.5O3. Magnetic susceptibility and heat capacity data bring out that this compound…

Materials Science · Physics 2017-03-29 Mohit K Sharma , Tathamay Basu , K Mukherjee , E V Sampathkumaran

It was discovered in La1-xSrxMnO3(x~1/8) that a field induced phase transition occurs from a ferromagnetic metal(FM) phase to a ferromagnetic insulator (FI) phase. The magnetization shows a sharp jump at the transition field accompanying…

Strongly Correlated Electrons · Physics 2016-08-31 H. Nojiri , K. Kaneko , M. Motokawa , K. Hirota , K. Takahashi , Y. Endoh

The transmission electron microscopy observations of the charge ordering (CO) which governs the electronic polarization in LuFe2O4-x clearly show the presence of a remarkable phase separation at low temperatures. Two CO ground states are…

Strongly Correlated Electrons · Physics 2015-05-14 H. X. Yang , H. F. Tian , Y. Zhang , Y. B. Qin , L. J. Zeng , C. Ma , H. L. Shi , J. B. Lu , J. Q. Li

Hexagonal manganites are multiferroic materials with two highly-dissimilar phase transitions: a ferroelectric transition (from P63/mmc to P63cm) at a temperature higher than 1000 K and an antiferromagnetic transition at TN=65 - 130 K.…

Strongly Correlated Electrons · Physics 2018-02-20 Hasung Sim , Jaehong Jeong , Haeri Kim , S-W Cheong , Je-Geun Park

Using density functional theory calculations, ultrathin films of SrVO3(d1) and SrCrO3(d2) on SrTiO3 substrates have been studied as possible multiferroics. Although both are metallic in the bulk limit, they are found to be insulating as a…

Materials Science · Physics 2015-06-16 Kapil Gupta , Priya Mahadevan , Phivos Mavropoulos , Marjana Lezaic

Two-dimensional multiferroic materials are highly sought after due to their huge potential for applications in nanoelectronic and spintronic devices. Here, we predict, based on first-principle calculations, a single phase {\it triferroic}…

Materials Science · Physics 2022-11-07 Srishti Bhardwaj , T. Maitra

In hybrid improper ferroelectric systems, polarization arises from the onset of successive nonpolar lattice modes. In this work, measurements and modeling were performed to determine the spatial symmetries of the phases involved in the…

Materials Science · Physics 2019-07-03 S. Liu , H. Zhang , S. Ghose , M. Balasubramanian , Zhenxian Liu , S. G. Wang , Y-S. Chen , B. Gao , J. Kim , S. -W. Cheong , T. A. Tyson

We present magnetodielectric measurements in single crystals of the cubic spin-1/2 compound Cu$_2$OSeO$_3$. A magnetic field-induced electric polarization ($\vec{P}$) and a finite magnetocapacitance (MC) is observed at the onset of the…

Strongly Correlated Electrons · Physics 2012-06-14 M. Belesi , I. Rousochatzakis , M. Abid , U. K. Rößler , H. Berger , J. -Ph. Ansermet

Monte Carlo simulations are used to examine cooperative creation of polar state in fluids of two-state particles with nonzero dipole in the excited state. With lowering temperature such systems undergo a second order transition from…

Soft Condensed Matter · Physics 2009-11-11 Dmitry V. Matyushov , Andriy Okhrimovskyy

The quadruple perovskite CaMn$_7$O$_{12}$ is a topical multiferroic, in which the hierarchy of electronic correlations driving structural distortions, modulated magnetism, and orbital order is not well known and may vary with temperature.…

Materials Science · Physics 2020-06-30 K. Gautam , S. S. Majid , S. Francoual , A. Ahad , K. Dey , M. C. Rahn , R. Sankar , F. C. Chou , D. K. Shukla

The question of how ferroelectric polarization is coupled to magnetism in magnetoelectric multiferroics, in which both types of order are simultaneously present, is of considerable scientific and practical interest. A recent Letter…

Materials Science · Physics 2009-07-13 Rogerio de Sousa , Joel E. Moore

We report on the microwave, terahertz (THz), infrared and Raman spectroscopic studies of $BiMn_{7}O_{12}$ ceramics, shedding more light into the nature of two structural phase transitions and their possible relation with ferroelectricity in…

Materials Science · Physics 2024-01-08 A. Maia , M. Kempa , V. Bovtun , R. Vilarinho , C. Kadlec , J. Agostinho Moreira , A. A. Belik , P. Proschek , S. Kamba

Magnetization and specific heat measurements on a UIrSi3 single crystal reveal Ising-like antiferromagnetism below T$_N$ = 41.7 K with easy magnetization direction along the c-axis of tetragonal structure. The antiferromagentic ordering is…

The electron spin polarization on half-metallic double-perovskites is usually conditioned to the ordered rock-salt arrangement of the transition-metal ions along the lattice. In this work, we investigate a polycrystalline sample of the…

Two-dimensional (2D) multiferroic materials are ideal systems for exploring new coupling mechanisms between different ferroic orders and producing novel quantum phenomena with potential applications. We employed first-principles density…

Materials Science · Physics 2022-09-20 Weiwei Gao , Jijun Zhao , James R. Chelikowsky

We propose mechanism for pressure-induced transitions between ferromagnetic and antiferromagnetic phases that relies on a competition between characteristic energy scales ubiquitous among $d$-electron metallic magnetic compounds. Principles…

Strongly Correlated Electrons · Physics 2019-12-20 Marcin M. Wysokiński

It is shown that the time-reversal symmetry is broken during the phase transition causing orbital ordering in a crystal with Jahn-Teller (J-T) ions. This means that such phase transitions are magnetic ones. As an example we have considered…

Strongly Correlated Electrons · Physics 2023-11-27 Khisa Borlakov , Dalkhat Ediev , Amina Borlakova