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A kinetic model of the electron transfer at the electrode / electrolyte solution interface is developed, implemented in a Monte Carlo framework, and applied to simulate this process in idealised systems consisting of the primitive model of…

Faraday's experiment measures -- within a modern view -- the charge adiabatically transported over a macroscopic distance by a given nuclear species in insulating liquids: the reason why it is integer is deeply rooted in topology. Whole…

Materials Science · Physics 2022-01-12 Raffaele Resta

The response of a model micro-electrochemical system to a time-dependent applied voltage is analyzed. The article begins with a fresh historical review including electrochemistry, colloidal science, and microfluidics. The model problem…

Soft Condensed Matter · Physics 2009-11-10 Martin Z. Bazant , Katsuyo Thornton , Armand Ajdari

Charge fluctuations in nano-circuits with capacitor components are shown to give rise to a novel type of long-ranged interaction, which co-exist with the regular Casimir/van der Waals force. The developed theory distinguishes between…

Mesoscale and Nanoscale Physics · Physics 2016-01-27 D. Drosdoff , Igor V. Bondarev , Allan Widom , Rudolph Podgornik , Lilia M. Woods

Bioimpedance measurements are a non-invasive method to determine the composition of organic tissue. For measuring the complex bioimpedance between two electrodes, an alternating current with a constant amplitude is injected into the tissue.…

Instrumentation and Detectors · Physics 2020-08-07 Roman Kusche , Steffen Kaufmann , Martin Ryschka

Supercapacitors are promising electrochemical energy storage devices due to their prominent performance in rapid charging/discharging rates, long cycle life, stability, etc. Experimental measurement and theoretical prediction on charging…

Numerical Analysis · Mathematics 2023-05-31 Lijie Ji , Zhenli Xu , Shenggao Zhou

The ability to reversibly toggle between two distinct states in a non-volatile method is important for information storage applications. Such devices have been realized for phase-change materials, which utilizes local heating methods to…

We study the electrode polarization behaviour of different Na-Ca-phosphosilicate glasses by measuring the differential capacitance between blocking Pt electrodes. At low applied dc bias voltages, we detect a linear capacitance regime with…

Disordered Systems and Neural Networks · Physics 2009-11-11 C. R. Mariappan , T. P. Heins , B. Roling

Porous electrodes are found in energy storage devices such as supercapacitors and pseudocapacitors. However, the effect of electrode-pore-size distribution over their energy storage properties remains unclear. Here, we develop a model for…

Chemical Physics · Physics 2021-12-03 Filipe Henrique , Pawel J. Zuk , Ankur Gupta

Through experimentation, we have discovered that with the changing of driving conditions, the Faraday waves undergo two abrupt transitions in spatiotemporal order: onset and instability. The driving amplitudes and frequencies corresponding…

Fluid Dynamics · Physics 2023-05-16 Peizhao Li , Tiancheng Yu , Xuechang Tu , Han Yan , Wei Wang , Luqun Zhou

The negative differential thermal conductance (NDTC) provides the key mechanism for realizing thermal transistors. This exotic effect has been the object of an extensive theoretical investigation, but the implementation is still limited to…

Mesoscale and Nanoscale Physics · Physics 2023-04-17 Shobhit Saheb Dey , Giuliano Timossi , Luigi Amico , Giampiero Marchegiani

In this paper we report on some new results concerning the behavior of forces between two equal circular electrodes with finite thickness. We show that for close electrodes different scenarios can result, depending on the thickness and on…

Classical Physics · Physics 2018-01-26 Giampiero Paffuti

We investigate the electronic and structural changes at the nanoscale in vanadium dioxide (VO2) in the vicinity of its thermally driven phase transition. Both electronic and structural changes exhibit phase coexistence leading to…

The dynamics of an argon plasma in the gap of a thermionic diode is investigated using particle-in-cell (PIC) simulations. The time-averaged diode current, as a function of the relative electrical potential between the electrodes, is…

Plasma Physics · Physics 2021-02-24 R. E. Groenewald , S. Clark , A. Kannan , P. Scherpelz

Energy and charge transfer across metal-semiconductor interfaces are the fundamental driving forces for a broad range of applications, such as computing, energy harvesting, and photodetection. However, the exact roles and physical…

Porous electrodes{made of hierarchically nanostructured materials{are omnipresent in various electrochemical energy technologies from batteries and supercapacitors to sensors and electrocatalysis. Modeling the system-level macroscopic…

Applied Physics · Physics 2022-02-03 Anis Allagui , Hachemi Benaoum

Net atomic charges (NACs) are widely used in all chemical sciences to concisely summarize key information about the partitioning of electrons among atoms in materials. Although widely used, there is currently no atomic population analysis…

Chemical Physics · Physics 2015-12-29 Thomas A. Manz , Nidia Gabaldon Limas

The split-charge equilibration method is extended to describe dissipative charge transfer similarly as the Drude model, whereby the generic frequency-dependent dielectric permitivitties or conductivities of dielectrics and metals can be…

Materials Science · Physics 2024-10-02 Martin H. Müser

We discuss possible patterns of electron fractionalization in strongly interacting electron systems. A popular possibility is one in which the charge of the electron has been liberated from its Fermi statistics. Such a fractionalized phase…

Strongly Correlated Electrons · Physics 2013-07-19 Eugene Demler , Chetan Nayak , Hae-Young Kee , Yong Baek Kim , T. Senthil

The proposed switching mechanism is based on an electronically-induced metal-insulator transition occurring in conditions of the excess non-equilibrium carrier density under the applied electric field. First, this mechanism is developed on…

Materials Science · Physics 2007-05-23 P. P. Boriskov , A. L. Pergament , A. A. Velichko , G. B. Stefanovich , N. A. Kuldin
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