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Helical dichroism (HD) is a proposed method for the resolution of molecular chirality, employing the orbital angular momentum (OAM) of light. Going beyond the conventional assumptions about HD, this work proposes a rigid theoretical…

Atomic Physics · Physics 2026-01-09 Mateja Hrast , Georgios M. Koutentakis , Mikhail Maslov , Mikhail Lemeshko

Circular dichroism, arising from interactions with light fields of opposite spin angular momentum, has become a fundamental tool for molecular characterization. Meanwhile, helical dichroism (HD) - the dichroic response to vortex beams…

Chirality is a structural property of molecules lacking mirror symmetry that has strong implications in diverse fields, ranging from life to materials sciences. Established spectroscopic methods that are sensitive to chirality, such as…

Investigating chiral light-matter interactions is essential for advancing applications in sensing, imaging, and pharmaceutical development. However, the chiroptical response in natural chiral molecules and subwavelength chiral structures is…

Circular dichroism (CD) caused by the response of a chiral object to circularly polarized light has been well established, and the strong CD of plasmonic meta-molecules has also become of interest in recent years; however, their response if…

Optics · Physics 2020-09-30 Yangzhe Guo , Guodong Zhu , Wanlu Bian , Bin Dong , Yurui Fang

Helical dichroism (HD), originating from the interplay between chiral plasmonic structures and left and right vortex light carrying orbital angular momentum (OAM), has attracted significant attention across various disciplines owing to its…

Optics · Physics 2025-08-08 Takahiro Uto , An'an Wu , Tsutomu Shimura , Yoshito Y. Tanaka

The controlled fabrication and chiroptical characterization of microscale chiral structures remain central challenges in photonics, sensing, and metamaterial engineering. Here we demonstrate an accessible, low-cost platform that combines…

Optics · Physics 2026-05-07 Jing Xu , Rik Strobbe , Yovan de Coene , Renaud A. L. Vallée , Koen Clays

Circular dichroism (CD), induced by chirality, is an important tool for manipulating light or for characterizing morphology of molecules, proteins, crystals and nano-structures. CD is manifested over a wide size-range, from molecules to…

Whether or not chiral interaction exists between the optical orbital angular momentum (OAM) and a chiral molecule remains unanswered. So far, such an interaction has not been observed experimentally. Here we present a T-matrix method to…

Optics · Physics 2018-01-01 Tong Wu , Rongyao Wang , Xiangdong Zhang

Circular dichroism (CD), i.e. the differential response of a system to left and right circularly polarized light, is one of the only techniques capable of providing morphological information of certain samples. In biology, for instance, CD…

Chiral light-matter interactions have traditionally been understood in terms of electric-magnetic dipolar interference driven by light with spin angular momentum. Here, we show that optical chirality can also originate from the orbital…

Optics · Physics 2025-08-13 Shun Hashiyada , An'an Wu , Yoshito Y. Tanaka

We show, by way of tight-binding and first-principles calculations, that a one-to-one correspondence between electron's crystal momentum k and non-zero orbital angular momentum (OAM) is a generic feature of surface bands. The OAM forms a…

Materials Science · Physics 2013-05-30 Jin-Hong Park , Choong H. Kim , Jun Won Rhim , Jung Hoon Han

We explore experimentally if the light's orbital angular momentum (OAM) interacts with chiral nematic polymer films. Specifically, we measure the circular dichroism of such a material using light beams with different OAM. We investigate the…

Optics · Physics 2011-06-20 W. Löffler , D. J. Broer , J. P. Woerdman

A light beam can carry both spin angular momentum (SAM) and orbital angular momentum (OAM). SAM is commonly evidenced by circular dichroism (CD) experiments {\em i. e.} differential absorption of left and right-handed circularly polarized…

Molecular chirality plays an important role in chemistry and biology, allows control of biological interactions, affects drugs efficacy and safety, and promotes synthesis of new materials. In general, chirality manifests itself in optical…

Optics · Physics 2026-04-10 Yuanyang Xie , Alexey V. Krasavin , Anatoly V. Zayats

In the close vicinity of a chiral nanostructure, the circular dichroism of a biomolecule could be greatly enhanced, due to the interaction with the local superchiral fields. Modest enhancement of optical activity using a planar…

The chiral state of a molecule plays a crucial role in molecular recognition and biochemical reactions. Because of this and owing to the fact that most modern drugs are chiral, the sensitive and reliable detection of the chirality of…

Mesoscale and Nanoscale Physics · Physics 2019-04-30 Luisa M. Kneer , Eva-Maria Roller , Lucas V. Besteiro , Robert Schreiber , Alexander O. Govorov , Tim Liedl

Identifying and imaging spin textures of ever more complex magnetic structures has become a major challenge in the past decade, especially at ultrashort timescales. Most of current approaches are based on the analysis of their polarization…

Optics · Physics 2020-05-26 Thierry Ruchon , Mauro Fanciulli

This paper presents a full 3D Method of Moments (MoM) simulation for analysis of scattering from nano-scale chiral ribbon structures under optical vortex illumination to aim to investigate electromagnetic mechanism of circular dichroism…

Materials Science · Physics 2026-01-27 Chenxu Wang , Hideki Kawaguchi , Hiroaki Nakamura , Koichi Matsuo , Masahiro Katoh

Chirality is a fundamental feature in all domains of nature, ranging from particle physics over electromagnetism to chemistry and biology. Chiral objects lack a mirror plane and inversion symmetry and therefore cannot be spatially aligned…

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