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We show that the recently observed class of long-range ion-Rydberg molecules can be divided into two families of states, which are characterised by their unique electronic structures resulting from the ion-induced admixture of quantum…

Atomic Physics · Physics 2023-02-14 Daniel J. Bosworth , Frederic Hummel , Peter Schmelcher

Since their first experimental observation, ultralong-range Rydberg molecules consisting of a highly excited Rydberg atom and a ground state atom have attracted the interest in the field of ultracold chemistry. Especially the intriguing…

We predict the existence of a class of ultracold giant molecules formed from trapped ultracold Rydberg atoms and polar molecules. The interaction which leads to the formation of such molecules is the anisotropic charge-dipole interaction…

Atomic Physics · Physics 2015-05-18 Seth T. Rittenhouse , H. R. Sadeghpour

Rydberg molecules, often exemplified by long-range "trilobite" molecules, are a subject of much recent interest at high principal quantum number $n$. States that use the same bonding mechanism can exist at much lower $n$ and less-extreme…

Atomic Physics · Physics 2017-05-01 R. A. Carollo , J. L. Carini , E. E. Eyler , P. L. Gould , W. C. Stwalley

The coupling of an isolated quantum state to a continuum is typically associated with decoherence and decreased lifetime. Here, we demonstrate that Rydberg macrodimers, weakly bound pairs of Rydberg atoms, can overcome this dissipative…

When ultracold plasma is generated using photonization of laser cooled atoms, some atoms reach only upto Rydberg states. These in turn interact with the free electrons of the plasma and get ionized further. We study the interaction of…

Atomic Physics · Physics 2026-03-18 Satyam Prakash , Ashok S Vudayagiri

We investigate the quantum dynamics of ultra-long-range trilobite molecules exposed to homogeneous electric fields. A trilobite molecule consists of a Rydberg atom and a ground-state atom, which is trapped at large internuclear distances in…

Atomic Physics · Physics 2021-02-24 Frederic Hummel , Kevin Keiler , Peter Schmelcher

We report on the induction of magnetization in Rydberg systems by means of the inverse Faraday effect, and propose the appearance of the effect in two such systems, Rydberg atoms proper and shallow dopants in semiconductors. Rydberg atoms…

Atomic Physics · Physics 2025-03-05 Patrick J. Wong , Ivan M. Khaymovich , Gabriel Aeppli , Alexander V. Balatsky

Highly excited Rydberg atoms inherit their level structure, symmetries, and scaling behavior from the hydrogen atom. We demonstrate that these fundamental properties enable a thermodynamic limit of a single Rydberg atom subjected to…

Atomic Physics · Physics 2023-06-23 Matthew T. Eiles , Alexander Eisfeld , Jan M. Rost

We introduce the Rydberg Composite, a new class of Rydberg matter where a single Rydberg atom is interfaced with a dense environment of neutral ground state atoms. The properties of the Composite depend on both the Rydberg excitation, which…

Atomic Physics · Physics 2020-09-02 Andrew L. Hunter , Matthew T. Eiles , Alex Eisfeld , Jan M. Rost

We observe a series of conical intersections in the potential energy curves governing both the collision between a Rydberg atom and a ground-state atom and the structure of Rydberg molecules. By employing the electronic energy of the…

Atomic Physics · Physics 2021-07-14 Frederic Hummel , Matthew T. Eiles , Peter Schmelcher

Controlling quantum entanglement between parts of a many-body system is the key to unlocking the power of quantum information processing for applications such as quantum computation, high-precision sensing, and simulation of many-body…

Quantum Physics · Physics 2016-01-07 Y. -Y. Jau , A. M. Hankin , Tyler Keating , I. H. Deutsch , G. W. Biedermann

A remarkable property of Rydberg atoms is the possibility to create molecules formed by one highly excited atom and another atom in the ground state. The first realisation of such a Rydberg molecule has opened an active field of physical…

Atomic Physics · Physics 2013-04-02 Andrej Junginger , Jörg Main , Günter Wunner

A molecular description for magic-number configurations of interacting electrons in a quantum dot in high magnetic fields developed by one of the authors has been elaborated for four, five and six electron dots. For four electrons, the…

Mesoscale and Nanoscale Physics · Physics 2009-10-30 Hiroshi Imamura , Peter A. Maksym , Hideo Aoki

Using the method of breaking of circular symmetry and of subsequent symmetry restoration via projection techiques, we present calculations for the ground-state energies and excitation spectra of N-electron parabolic quantum dots in strong…

Mesoscale and Nanoscale Physics · Physics 2009-11-11 Yuesong Li , Constantine Yannouleas , Uzi Landman

We present fast Rydberg-mediated entanglement involving nuclear spins of divalent atoms with $^{171}$Yb as an example. First, we show a nuclear-spin controlled phase gate of an arbitrary phase realizable either with two laser pulses when…

Quantum Physics · Physics 2023-12-12 Xiao-Feng Shi

Ultralong-range Rydberg molecules provide an exciting testbed for molecular physics at exaggerated scales. In the so-called trilobite and butterfly Rydberg molecules, the Born-Oppenheimer approximation can fail due to strong non-adiabatic…

Atomic Physics · Physics 2023-02-23 Frederic Hummel , Peter Schmelcher , Matthew T. Eiles

We investigate triatomic molecules that consist of two ground state atoms and a highly excited Rydberg atom, bound at large internuclear distances of thousands of \AA ngstroms. In the molecular state the Rydberg electron is in a…

Atomic Physics · Physics 2019-02-27 Christian Fey , Frederic Hummel , Peter Schmelcher

We introduce a class of spin models with long-range interactions---in the sense that they extend significantly beyond nearest neighbors---whose ground states can be constructed analytically and have a simple matrix product state…

Strongly Correlated Electrons · Physics 2015-06-19 Emanuele Levi , Igor Lesanovsky

By investigating the quantum properties of magnetically trapped nS Rydberg atoms, it is demonstrated that the composite nature of Rydberg atoms significantly alters their trapping properties opposed to point-like particles with the same…

Atomic Physics · Physics 2009-04-22 M. Mayle , I. Lesanovsky , P. Schmelcher