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We analyze thermodynamics of water samples confined in nanopores and prove that although the freezing temperature can be dramatically lower, the suppression of the ice nucleation leading to the freezing temperature depression is a truly…

Soft Condensed Matter · Physics 2012-06-18 P. O. Fedichev , L. I. Menshikov

A fluid in a pore can form diverse heterogeneous structures. We combine a capillary description with the cubic-plus-association equation of state to study the thermodynamic stability of droplets, bubbles and films of water at 358 K in a…

Computational Physics · Physics 2019-09-04 Magnus Aa. Gjennestad , Øivind Wilhelmsen

Protein nanoparticles have been proven to be highly effective stabilizers of water-in-water emulsions obtained from a number of different types of aqueous two-phase systems (ATPS). The stabilizing efficiency of such particles is attributed…

Soft Condensed Matter · Physics 2025-02-14 Andrzej Balis , Georgi Gochev , Domenico Truzzolillo , Dawid Lupa , Liliana Szyk-Warszynska , Jan Zawala

The interaction of water with surfaces is crucially important in a wide range of natural and technological settings. In particular, at low temperatures, unveiling the atomistic structure of adsorbed water clusters would provide valuable…

Materials Science · Physics 2024-02-23 F. Priante , N. Oinonen , Y. Tian , D. Guan , C. Xu , S. Cai , P. Liljeroth , Y. Jiang , A. S. Foster

The method of formation of nanoparticle aggregates such as high-coverage spherical shells of microspheres or 3-D micro crystals grown in the geometry unaffected by a substrate is described. In the reported experiment, the evaporation of…

Soft Condensed Matter · Physics 2011-04-05 GGennadiy Derkachov , Krystyna Kolwas , Daniel Jakubczyk , Marcin Zientara , Maciej Kolwas

In this study, molecular dynamic simulations are employed to investigate the nucleation of NaCl crystal in solutions. According to the simulations, the dissolved behaviors of NaCl in water are dependent on ion concentrations. With…

Chemical Physics · Physics 2018-11-29 Qiang Sun

Scatterer induced modal coupling and the consequent mode splitting in a whispering gallery mode resonator is demonstrated in aqueous environment. The rate of change in splitting as particles enter the resonator mode volume strongly depends…

Optics · Physics 2010-11-05 Woosung Kim , Sahin Kaya Ozdemir , Jiangang Zhu , Lina He , Lan Yang

The liquid and supercooled states of water show a series of anomalies whose nature is debated. A key role is attributed to the formation of structural aggregates induced by critical phenomena occurring deep in the supercooled region; the…

Chemical Physics · Physics 2013-12-18 A. Taschin , P. Bartolini , R. Eramo , R. Righini , R. Torre

Water is the most important liquid in the Universe. At the same time it is the most anomalous liquid. It demonstrates several dozens of anomalies, among which are density anomaly, diffusion anomaly etc. Anomalous behavior of water is a…

Soft Condensed Matter · Physics 2017-06-12 Yu. D. Fomin , E. N. Tsiok , V. N. Ryzhov , V. V. Brazhkin

The static and dynamical properties of heavy water have been studied at ambient conditions with extensive Car-Parrinello molecular-dynamics simulations in the canonical ensemble, with temperatures ranging between 325 K and 400 K.…

Soft Condensed Matter · Physics 2007-05-23 P. H-L. Sit , Nicola Marzari

The condensational growth of spherical water microdroplets is studied in a laboratory setup and with a mathematical model. In the experiment, droplet clusters are kept in a freely levitated state within an upward-oriented flow of water…

Soft Condensed Matter · Physics 2019-06-25 Dmitrii N. Gabyshev , Alexander A. Fedorets , Nurken E. Aktaev , Otto Klemm , Stepan N. Andreev

The pronounced light-matter interactions in photonic crystals make them interesting as opto-fludic "building blocks" for lab-on-a-chip applications. We show how conducting electrolytes cause dissipation and smearing of the…

Optics · Physics 2007-05-23 Niels Asger Mortensen , Simon Ejsing , Sanshui Xiao

Fluids with spatial density variations of single or mixed molecules play a key role in biophysics, soft matter and materials science. The fluid structures usually form via spinodal decomposition or nucleation following an instantaneous…

Chemical Physics · Physics 2018-01-24 Charley Schaefer

Direct observations of the surface and shape of model nano-colloidal gels associated with measurements of the spatial distribution of water content during drying show that air starts to significantly penetrate the sample when the material…

Materials Science · Physics 2015-11-11 J Thiery , Stéphane Rodts , E Keita , Xavier Chateau , P Faure , D Courtier-Murias , T Kodger , P Coussot

While the water molecule is simple, its condensed phase liquid behavior is so complex that no consensus description has emerged despite three centuries of effort. Here we identify features of its behavior that are the most peculiar, hence…

Chemical Physics · Physics 2014-04-16 Stacey L. Meadley , C. Austen Angell

Molecular segregation in methanol-water mixtures is studied across a wide concentration range as a function of temperature and pressure. Cluster distributions obtained from both neutron diffraction and molecular dynamics simulations point…

Soft Condensed Matter · Physics 2009-11-10 L. Dougan , R. Hargreaves , S. P. Bates , J. L. Finney , V. Reat , A. K. Soper , J. Crain

Water behaves very differently at surfaces and under extreme confinement, but the boundary between these two regimes has remained unclear. Despite evidence that interfacial effects persist under sub-nanometre confinement, the…

Chemical Physics · Physics 2025-12-15 Xavier R. Advincula , Christoph Schran , Angelos Michaelides

Capillary condensation of water is ubiquitous in nature and technology. It routinely occurs in granular and porous media, can strongly alter such properties as adhesion, lubrication, friction and corrosion, and is important in many…

Mesoscale and Nanoscale Physics · Physics 2020-12-14 Qian Yang , P. Z. Sun , L. Fumagalli , Y. V. Stebunov , S. J. Haigh , Z. W. Zhou , I. V. Grigorieva , F. C. Wang , A. K. Geim

Molecular Dynamics simulations of water confined in nanometer sized, hydrophobic channels show that water forms localized cavities for pore diameter ~ 2.0 nm. The cavities present non-spherical shape and lay preferentially adjacent to the…

Soft Condensed Matter · Physics 2009-11-13 John Russo , Simone Melchionna , Francesco De Luca , Cinzia Casieri

Relations between the thermodynamics and dynamics of supercooled liquids approaching a glass transition have been proposed over many years. The potential energy surface of model liquids has been increasingly studied since it provides a…