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Sr$_{2}$IrO$_{4}$ with strong spin-orbit coupling (SOC) and Hubbard repulsion (U) hosts Mott insulating states. The similar crystal structure, magnetic and electronic properties, particularly the $d$-wave gap observed in Sr$_{2}$IrO$_{4}$…

Strongly Correlated Electrons · Physics 2023-12-04 Haozhe Wang , Madalynn Marshall , Zhen Wang , Kemp W. Plumb , Martha Greenblatt , Yimei Zhu , David Walker , Weiwei Xie

A neutron scattering study of the Mott-Hubbard insulator LaTiO$_{3}$ (T$_{{\rm N}}=132$ K) reveals a spin wave spectrum that is well described by a nearest-neighbor superexchange constant $J=15.5$ meV and a small Dzyaloshinskii-Moriya…

Strongly Correlated Electrons · Physics 2009-10-31 B. Keimer , D. Casa , A. Ivanov , J. W. Lynn , M. v. Zimmermann , J. P. Hill , D. Gibbs , Y. Taguchi , Y. Tokura

We measured two magnetic modes with finite and discrete energies in an antiferromagnetic ordered phase of a geometrically frustrated magnet MgCr2O4 by single-crystal inelastic neutron scattering, and clarified the spatial spin correlations…

Strongly Correlated Electrons · Physics 2008-10-22 K. Tomiyasu , H. Suzuki , M. Toki , S. Itoh , M. Matsuura , N. Aso , K. Yamada

We present a thorough experimental study of the three-dimensional hyperhoneycomb Kitaev magnet $\beta$-Li$_2$IrO$_3$, using a combination of inelastic neutron scattering (INS), time-domain THz spectroscopy, and heat capacity measurements.…

We present a parametric study of the diffuse magnetic scattering at (1/2,1/2,1/2) positions in reciprocal space, ascribed to a frozen antiferromagnetic spin ice state in single crystalline Tb2Ti2O7. Our high-resolution neutron scattering…

Strongly Correlated Electrons · Physics 2015-06-18 K. Fritsch , E. Kermarrec , K. A. Ross , Y. Qiu , J. R. D. Copley , D. Pomaranski , J. B. Kycia , H. A. Dabkowska , B. D. Gaulin

Sr$_{3}$Cr$_{2}$O$_{8}$ consist of a lattice of spin-1/2 Cr$^{5+}$ ions, which form hexagonal bilayers and which are paired into dimers by the dominant antiferromagnetic intrabilayer coupling. The dimers are coupled three-dimensionally by…

We have studied the evolution of magnetic and orbital excitations as a function of hole-doping in single crystal samples of Sr2Ir(1-x)Rh(x)O4 (0.07 < x < 0.42) using high resolution Ir L3-edge resonant inelastic x-ray scattering (RIXS).…

Strongly Correlated Electrons · Physics 2019-09-18 J. P. Clancy , H. Gretarsson , M. H. Upton , Jungho Kim , G. Cao , Young-June Kim

Inelastic neutron scattering profiles of spin waves in the dilute quasi-one-dimensional Ising-like antiferromagnet CsCo_{0.83}Mg_{0.17}Br_3 have been investigated. Calculations of S^{xx}(Q,omega), based on an effective spin Hamiltonian,…

Condensed Matter · Physics 2009-11-07 Y. S. Yang , F. Marsiglio , M. Madsen , B. D. Gaulin , R. B. Rogge , J. A. Fernandez-Baca

We have used a combination of resonant magnetic x-ray scattering (RMXS) and x-ray absorption spectroscopy (XAS) to investigate the properties of the doped spin-orbital Mott insulator Sr2Ir(1-x)Rh(x)O4 (0.07 < x < 0.70). We show that…

Strongly Correlated Electrons · Physics 2014-02-12 J. P. Clancy , A. Lupascu , H. Gretarsson , Z. Islam , Y. F. Hu , D. Casa , C. S. Nelson , S. C. Lamarra , G. Cao , Young-June Kim

We report inelastic neutron scattering experiments on single crystals of superconducting Ba0.67K0.33Fe2As2 (Tc = 38 K). In addition to confirming the resonance previously found in powder samples, we find that spin excitations in the normal…

The role of dipolar interactions and anisotropy are important to obtain, otherwise forbidden, ferromagnetic ordering at finite temperature for ions arranged in two-dimensional (2D) arrays (monolayers). Here we demonstrate that conventional…

Mesoscale and Nanoscale Physics · Physics 2007-05-23 M. K. Mukhopadhyay , M. K. Sanyal , T. Sakakibara , V. Leiner , R. M. Dalgliesh , S. Langridge

We report point-contact measurements of anisotropic magnetoresistance (AMR) in a single crystal of antiferromagnetic (AFM) Mott insulator Sr2IrO4. The point-contact technique is used here as a local probe of magnetotransport properties on…

Mesoscale and Nanoscale Physics · Physics 2014-12-03 Cheng Wang , Heidi Seinige , Gang Cao , Jian-Shi Zhou , John B. Goodenough , Maxim Tsoi

The tetrameric Ni(II) spin cluster Ni4Mo12 has been studied by INS. The data were analyzed extensively in terms of a very general spin Hamiltonian, which includes antiferromagnetic Heisenberg interactions, biquadratic 2-spin and 3-spin…

Mesoscale and Nanoscale Physics · Physics 2010-06-11 J. Nehrkorn , M. Höck , M. Brüger , H. Mutka , J. Schnack , O. Waldmann

We report $^{63}$Cu nuclear magnetic resonance and muon spin rotation measurements on the S=1/2 antiferromagnetic Heisenberg spin chain compound Sr$_{1.9}$Ca$_{0.1}$CuO$_3$. An exponentially decreasing spin-lattice relaxation rate 1/T$_1$…

Strongly Correlated Electrons · Physics 2014-05-21 F. Hammerath , E. M. Brüning , S. Sanna , Y. Utz , N. S. Beesetty , R. Saint-Martin , A. Revcolevschi , C. Hess , B. Büchner , H. -J. Grafe

The single ion physics of Ho$_2$Ti$_2$O$_7$ is well-understood to produce strong Ising anisotropy, which is an essential ingredient to its low-temperature spin ice state. We present inelastic neutron scattering measurements on…

Strongly Correlated Electrons · Physics 2018-07-25 J. Gaudet , A. M. Hallas , C. R. C. Buhariwalla , G. Sala , M. B. Stone , M. Tachibana , K. Baroudi , R. J. Cava , B. D. Gaulin

CoO has an odd number of electrons in its unit cell, and therefore is expected to be metallic. Yet, CoO is strongly insulating owing to significant electronic correlations, thus classifying it as a Mott insulator. We investigate the…

Inelastic neutron scattering measurements on the itinerant antiferromagnet (AFM) CaCo$_{\mathrm{2}-y}$As$_{2}$ at a temperature of 8 K reveal two orthogonal planes of scattering perpendicular to the Co square lattice in reciprocal space,…

We propose a method for measuring spin Hamiltonians and apply it to the spin-1/2 Heisenberg antiferromagnet Cs2CuCl4, which shows a 2D fractionalized RVB state at low fields. By applying strong fields we fully align the spin moment of…

Strongly Correlated Electrons · Physics 2007-05-23 R. Coldea , D. A. Tennant , K. Habicht , P. Smeibidl , C. Wolters , Z. Tylczynski

For iridates with large spatially extended 5d orbitals, it may be anticipated that distant neighbor interactions would play a crucial role in their ground state properties. From this perspective, we investigate the magnetic structure of…

Materials Science · Physics 2019-09-04 Vijeta Singh , J. J. Pulikkotil

Elastic and inelastic neutron scattering studies have been carried out on the pyrochlore magnet Ho2Ti2O7. Measurements in zero applied magnetic field show that the disordered spin ice ground state of Ho2Ti2O7 is characterized by a pattern…

Strongly Correlated Electrons · Physics 2016-08-05 J. P. Clancy , J. P. C. Ruff , S. R. Dunsiger , Y. Zhao , H. A. Dabkowska , J. S. Gardner , Y. Qiu , J. R. D. Copley , T. Jenkins , B. D. Gaulin