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The magnetic structure and spin-wave excitations in the quasi-square-lattice layered perovskite compound La$_5$Mo$_4$O$_{16}$ were studied by a combination of neutron diffraction and inelastic neutron scattering techniques using…

Strongly Correlated Electrons · Physics 2017-06-07 K. Iida , R. Kajimoto , Y. Mizuno , K. Kamazawa , Y. Inamura , A. Hoshikawa , Y. Yoshida , T. Matsukawa , T. Ishigaki , Y. Kawamura , S. Ibuka , T. Yokoo , S. Itoh , T. Katsufuji

An inelastic neutron scattering study was performed on a Zn-substituted spin-1/2 Heisenberg 2-leg ladder compound Sr(Cu1-xZnx)2O3 (x < 0.04) to investigate nonmagnetic impurity effects on the quantum spin system with a large spin gap of…

Condensed Matter · Physics 2009-10-30 M. Azuma , M. Takano , R. S. Eccleston

We study dynamical properties of the anisotropic triangular quantum antiferromagnet Cs_2CuCl_4. Inelastic neutron scattering measurements have established that the dynamical spin correlations cannot be understood within a linear spin wave…

Strongly Correlated Electrons · Physics 2007-05-23 Martin Y. Veillette , Andrew J. A. James , Fabian H. L. Essler

We performed inelastic neutron scattering experiments on Cu$_2$$^{114}$Cd$^{11}$B$_2$O$_6$ powder. The magnetic excitations at low temperatures are similar to those of the interacting spin-1/2 tetramers in the ordered state. The weak…

Strongly Correlated Electrons · Physics 2015-12-09 Masashi Hase , Kenji Nakajima , Seiko Ohira-Kawamura , Yukinobu Kawakita , Tatsuya Kikuchi , Masashige Matsumoto

We present inelastic neutron scattering measurements and first principles calculations examining the intermetallic marcasite CrSb2. The observed spin wave dispersion implies that the magnetic interactions are strongly one-dimensional with…

Strongly Correlated Electrons · Physics 2015-06-03 M. B. Stone , M. D. Lumsden , S. E. Nagler , D. J. Singh , J. He , B. C. Sales , D. Mandrus

Here we present inelastic neutron scattering measurements from the frustrated, quantum spin-1/2 chain material linarite, PbCuSO_4(OH)_2. Time of flight data, taken at 0.5K and zero applied magnetic field reveals low-energy dispersive spin…

We present and analyze Raman spectra of the Mott insulator Ca$_2$RuO$_4$, whose quasi-two-dimensional antiferromagnetic order has been described as a condensate of low-lying spin-orbit excitons with angular momentum $J_{eff}=1$. In the…

Transformation of Coulomb interaction terms to the pseudo-orbital basis constituted by $J=1/2$ and $3/2$ states arising from spin-orbit coupling provides a versatile tool. This formalism is applied to investigate magnetic anisotropy effects…

Strongly Correlated Electrons · Physics 2019-03-11 Shubhajyoti Mohapatra , Avinash Singh

Magnetic excitations in a Ni$_4$ magnetic molecule were investigated by inelastic neutron scattering and bulk susceptibility ($\chi_\text{bulk}$) techniques. The magnetic excitation spectrum obtained from the inelastic neutron scattering…

Strongly Correlated Electrons · Physics 2015-06-04 K. Iida , S. -H. Lee , T. Onimaru , K. Matsubayashi , T. J. Sato

We use polarized inelastic neutron scattering (INS) to study spin excitations of optimally hole-doped superconductor Ba$_{0.67}$K$_{0.33}$Fe$_2$As$_{2}$ ($T_c=38$ K). In the normal state, the imaginary part of the dynamic susceptibility,…

Neutron scattering is used to investigate the single-ion spin and orbital excitations below the Mott-Hubbard gap in CoO. Three excitations are reported at 0.870 $\pm$ 0.009 eV, 1.84 $\pm$ 0.03, and 2.30 $\pm$ 0.15 eV. These were…

Strongly Correlated Electrons · Physics 2015-06-17 R. A. Cowley , W. J. L. Buyers , C. Stock , Z. Yamani , C. Frost , J. W. Taylor , D. Prabhakaran

The antiferromagnetic structure of Sr3Ir2O7, the bilayer analogue of a spin-orbital Mott insulator Sr2IrO4, was revealed by resonant magnetic x-ray diffraction. Contrasting intensities of the magnetic diffraction at the Ir LIII and LII…

Strongly Correlated Electrons · Physics 2015-06-05 Shigeki Fujiyama , K. Ohashi , H. Ohsumi , K. Sugimoto , T. Takayama , T. Komesu , M. Takata , T. Arima , H. Takagi

Sr$_{2}$IrO$_{4}$ has often been described via a simple, one-band pseudo-spin 1/2 model, subject to electron-electron interactions, on a square lattice, fostering analogies with cuprate superconductors, believed to be well described by a…

The magnon disp ersion in Ca2RuO4 has been determined by inelastic neutron scattering on single crytals containing 1% of Ti. The dispersion is well described by a conventional Heisenberg model suggesting a local moment model with nearest…

Strongly Correlated Electrons · Physics 2015-12-16 S. Kunkemöller , D. Khomskii , P. Steffens , A. Piovano , A. Nugroho , M. Braden

We report magnetic and thermodynamic properties of a $4d^1$ (Mo$^{5+}$) magnetic insulator MoOPO$_4$ single crystal, which realizes a $J_1$-$J_2$ Heisenberg spin-$1/2$ model on a stacked square lattice. The specific-heat measurements show a…

I propose the emergence of the spin-orbital-coupled vector chirality in a non-frustrated Mott insulator with the strong spin-orbit coupling due to $ab$-plane's inversion-symmetry (IS) breaking. I derive the superexchange interactions for a…

Strongly Correlated Electrons · Physics 2016-11-10 Naoya Arakawa

We have measured the doping and temperature dependence of lattice vibrations and magnetic excitations in the prototypical doped spin-orbit Mott insulator Sr$_{2-x}$La$_x$IrO$_4$ (x=0, 0.015, and 0.10). Our findings show that the…

Strongly Correlated Electrons · Physics 2017-09-27 H. Gretarsson , J. Sauceda , N. H. Sung , M. Höppner , M. Minola , B. J. Kim , B. Keimer , M. Le Tacon

Inelastic neutron scattering performed at a spallation source is used to make absolute measurements of the dynamic susceptibility of insulating La2CuO4 and superconducting La2-xSrxCuO4 over the energy range 15<EN<350 meV. The effect of Sr…

Superconductivity · Physics 2009-10-28 S. M. Hayden , G. Aeppli , H. A. Mook , T. G. Perring , T. E. Mason , S-W. Cheong , Z. Fisk

We have explored the magnetic excitation spectrum of the S=1/2 square lattice Heisenberg antiferromagnet, K2V3O8 using both triple-axis and time-of-flight inelastic neutron scattering. The long-wavelength spin waves are consistent with the…

Strongly Correlated Electrons · Physics 2015-06-25 M. D. Lumsden , S. E. Nagler , B. C. Sales , D. A. Tennant , D. F. McMorrow , S. -H. Lee , S. Park

In this short note, we report on the first inelastic neutron scattering (INS) study on high-energy magnetic excitations in Sr$_3$Ir$_2$O$_7$. We observed excitations between $\sim$80 meV and $\sim$180 meV. The peak position of the…

Strongly Correlated Electrons · Physics 2021-01-12 Masaki Fujita , Kazuhiko Ikeuchi , Ryoichi Kajimoto , Mitsutaka Nakamura