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In interstellar environment, fullerene species readily react with large molecules (e.g., PAHs and their derivatives) in the gas phase, which may be the formation route of carbon dust grains in space. In this work, the gas-phase ion-molecule…

Astrophysics of Galaxies · Physics 2024-05-28 Yin Wu , Xiaoyi Hu , Junfeng Zhen , Xuejuan Yang

The infrared (IR) emission of polycyclic aromatic hydrocarbons (PAHs) permeates our universe; astronomers have detected the IR signatures of PAHs around many interstellar objects. The IR emission of interstellar PAHs differs from their…

Astrophysics of Galaxies · Physics 2018-10-05 Cameron J. Mackie , Tao Chen , Alessandra Candian , Timothy J. Lee , Alexander G. G. M. Tielens

We present a charge distribution based model that computes the infrared spectrum of polycyclic aromatic hydrocarbon (PAH) molecules using recent measurements or quantum chemical calculations of specific PAHs. The model is applied to a…

Astrophysics of Galaxies · Physics 2022-06-15 Ameek Sidhu , A. G. G. M. Tielens , Els Peeters , Jan Cami

H2 formation in metal-free gas occurs via the intermediate H- or H2+ ions. Destruction of these ions by photodissociation therefore serves to suppress H2 formation. In this paper, I highlight the fact that several processes that occur in…

Astrophysics · Physics 2008-11-26 S. C. O. Glover

We have studied molecular hydrogen emission in a sample of 21 YSOs using spectra obtained with the Infrared Space Observatory (ISO). H2 emission was detected in 12 sources and can be explained as arising in either a shock, caused by the…

Astrophysics · Physics 2007-05-23 M. E. van den Ancker , P. R. Wesselius , A. G. G. M. Tielens

We present a new method to decompose the emission features of polycyclic aromatic hydrocarbons (PAHs) from mid-infrared spectra using theoretical PAH templates in conjunction with modified blackbody components for the dust continuum and an…

Astrophysics of Galaxies · Physics 2018-06-26 Yanxia Xie , Luis C. Ho , Aigen Li , Jinyi Shangguan

We present the detection and analysis of molecular hydrogen emission toward ten interstellar regions in the Large Magellanic Cloud. We examined low-resolution infrared spectral maps of twelve regions obtained with the Spitzer infrared…

The mid-infrared (IR; 5-15~$\mu$m) spectrum of a wide variety of astronomical objects exhibits a set of broad emission features at 6.2, 7.7, 8.6, 11.3 and 12.7 $\mu$m. About 30 years ago it was proposed that these signatures are due to…

Astrophysics of Galaxies · Physics 2014-07-02 Marissa J. F. Rosenberg , Olivier Berné , Christiaan Boersma

The formation of interstellar water has been commonly accepted to occur on the surfaces of icy dust grains in dark molecular clouds at low temperatures (10-20 K), involving hydrogenation reactions of oxygen allotropes. As a result of the…

Astrophysics of Galaxies · Physics 2014-10-22 Thanja Lamberts , Herma Cuppen , Gleb Fedoseev , Sergio Ioppolo , Ko-Ju Chuang , Harold Linnartz

We present subarcsecond-resolution ALMA mosaics of the Orion Bar PDR in [CI] 609um, C2H (4-3), and C18O (3-2) emission lines complemented by JWST images of H2 and aromatic infrared band (AIB) emission. The rim of the Bar shows very…

A first-principle theoretical approach to study the process of radiative electron attachment is developed and applied to the negative molecular ions CN$^-$, C$_4$H$^-$, and C$_2$H$^-$. Among these anions, the first two have already been…

Molecular fragmentation leading to the formation of negatively and positively charged hydrogen ions in 7-keV OH$^+$ + Ar collisions is investigated experimentally. The most striking finding is that negative and positive hydrogen ions are…

Cosmic Rays (CR) process the matter of the Interstellar Medium. Such energetic processing not only modifies the interstellar matter but also injects chemical species in the gas phase. In this work, we study the effect of the CR on the…

Astrophysics of Galaxies · Physics 2017-09-25 Marin Chabot , Karine Béroff , Emmanuel Dartois , Thomas Pino , Marie Godard

The fullerene C$_{60}$, one of the largest molecules identified in the interstellar medium (ISM), has been proposed to form top-down through the photo-chemical processing of large (more than 60 C-atoms) polycyclic aromatic hydrocarbon (PAH)…

Instrumentation and Methods for Astrophysics · Physics 2019-02-20 Weiwei Zhang , Yubing Si , Junfeng Zhen , Tao Chen , Harold Linnartz , Alexander G. G. M. Tielens

For star-forming galaxies, we investigate a global relation between polycyclic aromatic hydrocarbon (PAH) emission luminosity at 3.3 um, L_PAH3.3, and infrared (8-1000 um) luminosity, L_IR, to understand how the PAH 3.3 um feature relates…

Cosmology and Nongalactic Astrophysics · Physics 2015-06-16 Rika Yamada , Shinki Oyabu , Hidehiro Kaneda , Mitsuyoshi Yamagishi , Daisuke Ishihara , Ji Hoon Kim , Myungshin Im

We examine the annihilation of positrons on polycyclic aromatic hydrocarbon (PAH) molecules in interstellar medium conditions. We estimate the annihilation rates of positrons on PAHs by a semi-empirical approach. We show that PAHs can play…

High Energy Astrophysical Phenomena · Physics 2015-05-14 N. Guessoum , P. Jean , W. Gillard

Irradiation of isolated water molecules by few-cycle pulses of intense infrared laser light can give rise to ultrafast rearrangement resulting in formation of the H2+ ion. Such unimolecular reactions occur on the potential energy surface of…

Chemical Physics · Physics 2015-06-03 Manish Garg , Ashwani K. Tiwari , Deepak Mathur

The UV photoreactivity of polycyclic aromatic hydrocarbons (PAHs) in porous amorphous solid water has long been known to form both oxygenated photoproducts and photofragments. The aim of this study was to examine the influence of the ice…

Earth and Planetary Astrophysics · Physics 2020-11-25 J. A. Noble , E. Michoulier , C. Aupetit , J. Mascetti

The infrared signature of polycyclic aromatic hydrocarbons (PAHs) are present in many protostellar disks and these speciesare thought to play an important role in heating of the gas in the photosphere. We aim to consider PAH cluster…

Earth and Planetary Astrophysics · Physics 2021-09-01 K. Lange , C. Dominik , A. G. G. M. Tielens

The interaction of polycyclic aromatic hydrocarbons (PAHs) with vacuum ultraviolet (VUV) photons triggers the emission of the well-known aromatic infrared bands (AIBs) but other mechanisms such as fragmentation can be involved in this…

Astrophysics of Galaxies · Physics 2021-08-12 Alexandre Marciniak , Christine Joblin , Giacomo Mulas , Venkat Rao Mundlapati , Anthony Bonnamy