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Complete and precise characterization of a quantum dynamical process can be achieved via the method of quantum process tomography. Using a source of correlated photons, we have implemented several methods investigating a wide range of…

We present a method designed to efficiently extract optical signals from InGaAs avalanche photodiodes (APDs) operated in gated mode. In particular, our method permits an estimation of the fraction of counts which actually results from the…

Attosecond photoemission or photoionization delays are a unique probe of the structure and the electronic dynamics of matter. However, spectral congestion and spatial delocalization of valence electron wave functions set fundamental limits…

Attosecond transient-absorption spectroscopy (ATAS) is an established method for exploring electron dynamics on the subfemtosecond time-scale. ATAS spectra contain certain ubiquitous features, such as oscillating fringes, light-induced…

Atomic Physics · Physics 2017-08-02 Jørgen Johansen Rørstad , Jens E. Bækhøj , Lars Bojer Madsen

We consider the linear discriminant analysis problem in the high-dimensional settings. In this work, we propose PANDA(PivotAl liNear Discriminant Analysis), a tuning-insensitive method in the sense that it requires very little effort to…

Statistics Theory · Mathematics 2023-09-19 Ethan X. Fang , Yajun Mei , Yuyang Shi , Qunzhi Xu , Tuo Zhao

We develop an analytical model for ultraintense attosecond pulse emission in the highly relativistic laser-plasma interaction. In this model, the attosecond pulse is emitted by a strongly compressed electron layer around the instant when…

Plasma Physics · Physics 2019-01-30 Suo Tang , Naveen Kumar

Transient absorption is a very powerful observable in attosecond experiments on atoms, molecules and solids and is frequently used in experiments employing phase-locked few-cycle infrared and XUV laser pulses derived from high harmonic…

Atomic Physics · Physics 2020-08-26 Lorenz Drescher , Marc J. J. Vrakking , Jochen Mikosch

Tracing ultrafast processes induced by interaction of light with matter is often very challenging. In molecular systems, the initially created electronic coherence becomes damped by the slow nuclear rearrangement on a femtosecond timescale…

Chemical Physics · Physics 2021-09-20 Nikolay V. Golubev , Jiří Vaníček , Alexander I. Kuleff

The characterization of the complex spectral amplitude that is, the spectrum and spectral phase, of single-photon-level light fields is a crucial capability for modern photonic quantum technologies. Since established pulse characterisation…

An essential metric for the quality of a particle-identification experiment is its statistical power to discriminate between signal and background. Pulse shape discrimination (PSD) is a basic method for this purpose in many nuclear,…

Instrumentation and Detectors · Physics 2024-05-17 Shubham Dutta , Sayan Ghosh , Satyaki Bhattacharya , Satyajit Saha

We simulate the transient absorption of attosecond pulses of infrared-laser-dressed atoms by considering a three-level system with the adiabatic approximation. The delay-dependent interference features are investigated from the perspective…

Atomic Physics · Physics 2015-09-23 Wenpu Dong , Yongqiang Li , Xiaowei Wang , Jianmin Yuan , Zengxiu Zhao

Pulse-compression is a correlation-based measurement technique successfully used in many NDE applications to increase the SNR in the presence of huge noise, strong signal attenuation or when high excitation levels must be avoided. In…

Signal Processing · Electrical Eng. & Systems 2024-05-02 Marco Ricci , Rocco Zito , Stefano Laureti

The physics of high harmonics has led to the generation of attosecond pulses and to trains of attosecond pulses. Measurements that confirm the pulse duration are all performed in the far field. All pulse duration measurements tacitly assume…

Optics · Physics 2012-06-15 E. Frumker , G. G. Paulus , H. Niikura , A. Naumov , D. M. Villeneuve , P. B. Corkum

Molecular absorption and photo-electron spectra can be efficiently predicted with real-time time-dependent density-functional theory (TDDFT). We show here how these techniques can be easily extended to study time-resolved pump-probe…

Atomic and Molecular Clusters · Physics 2013-01-10 Umberto De Giovannini , Gustavo Brunetto , Alberto Castro , Jessica Walkenhorst , Angel Rubio

Standard optical pump-probe methods analyze a system's temporal response to a laser pulse within sub-femtoseconds to several nanoseconds, constrained by the optical delay line's length. While resistance is a sensitive detector in various…

Instrumentation and Detectors · Physics 2024-04-26 M. I. Blumenau , A. Yu. Kuntsevich

Anomaly detection methods require high-quality features. In recent years, the anomaly detection community has attempted to obtain better features using advances in deep self-supervised feature learning. Surprisingly, a very promising…

Computer Vision and Pattern Recognition · Computer Science 2021-08-13 Tal Reiss , Niv Cohen , Liron Bergman , Yedid Hoshen

Entangled two-photon absorption (eTPA) has been recognized as a potentially powerful tool for the implementation of ultra-sensitive spectroscopy. Unfortunately, there exists a general agreement in the quantum optics community that…

Quantum Physics · Physics 2025-01-31 Áulide Martínez-Tapia , Roberto de J. León-Montiel

Transient absorption (TA) is the most widespread method to follow ultrafast dynamics in molecules and materials. The related method of TA anisotropy (TAA) reports on the ultrafast reorientation dynamics of transition dipole moments,…

Measured photoionization time delays may exhibit large variations as a function of the emission angles, even for spherically symmetric targets, as shown in recent RABBITT (reconstruction of attosecond beating by interference of two-photon…

Atomic Physics · Physics 2022-12-29 D. I. R. Boll , L. Martini , A. Palacios , O. A. Fojón

The present work focuses on the characterisation of the amount of orbital angular momentum (OAM) encoded in the twisted attosecond pulses via energy- and angle-resolved attosecond streaking in pump-probe setup. It is found that the…

Atomic Physics · Physics 2020-06-03 Irfana N. Ansari , Deependra S. Jadoun , Gopal Dixit