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We show how low-energy electronic models derived from the first-principles electronic structure calculations can help to rationalize the magnetic properties of two lacunar spinel compounds GaM4S8 with light (M=V) and heavy (M=Mo)…

Strongly Correlated Electrons · Physics 2020-07-14 S. A. Nikolaev , I. V. Solovyev

Skyrmions are whirl like topological spin objects with high potential for future magnetic data storage. It is a fundamental question, relevant for both basic research and application, if a ferroelectric (FE) polarization can be associated…

Strongly Correlated Electrons · Physics 2015-11-18 E. Ruff , S. Widmann , P. Lunkenheimer , V. Tsurkan , S. Bordács , I. Kézsmárki , A. Loidl

Polar lacunar spinels, such as GaV$_4$S$_8$ and GaV$_4$Se$_8$, were proposed to host skyrmion phases under magnetic field. In this work, we put forward, as a candidate for N\'eel-type skyrmion lattice, the isostructural GaMo$_4$S$_8$, here…

Materials Science · Physics 2019-06-26 Hui-Min Zhang , Jun Chen , Paolo Barone , Kunihiko Yamauchi , Shuai Dong , Silvia Picozzi

The lacunar spinel GaV4S8 exhibits orbital ordering at 44 K and shows a complex magnetic phase diagram below 12.7 K, which includes ferromagnetic and cycloidal spin order. At low but finite external magnetic fields, N\'eel-type skyrmions…

Strongly Correlated Electrons · Physics 2017-12-14 S. Widmann , E. Ruff , A. Günther , H. -A. Krug von Nidda , P. Lunkenheimer , V. Tsurkan , S. Bordács , I. Kézsmárki , A. Loidl

In the present work, we provide results from specific heat, magnetic susceptibility, dielectric constant, ac conductivity, and electrical polarization measurements performed on the lacunar spinel GaV4Se8. With decreasing temperature, we…

Strongly Correlated Electrons · Physics 2017-10-18 E. Ruff , A. Butykai , K. Geirhos , S. Widmann , V. Tsurkan , E. Stefanet , I. Kézsmárki , A. Loidl , P. Lunkenheimer

We report the magnetization and the $^{51}$V NMR measurements in the polar magnet GaV$_4$Se$_8$ in which a magnetic skyrmion lattice appears in the structural domain with the polar axis parallel to the magnetic field. Although we…

Strongly Correlated Electrons · Physics 2024-12-24 Hikaru Takeda , Misaki Ishikawa , Masashi Takigawa , Minoru Yamashita , Yuri Fujima , Taka-hisa Arima

Lacunar spinels with a chemical formula of $AM_4X_8$ form a populous family of narrow-gap semiconductors, which offer a fertile ground to explore correlation and quantum phenomena, including transition between Mott and spin-orbit insulator…

Strongly Correlated Electrons · Physics 2022-05-25 K. Geirhos , S. Reschke , S. Ghara , S. Krohns , P. Lunkenheimer , I. Kézsmárki

By applying Berry-phase theory for the effective half-filled Hubbard model, we derive an analytical expression for the electronic polarization driven by the relativistic spin-orbit (SO) coupling. The model itself is constructed in the…

Materials Science · Physics 2017-06-14 I. V. Solovyev

In the $AB_4Q_8$ lacunar spinels, the electronic structure is described on the basis of inter- and intra-cluster interactions of tetrahedral $B_4$ clusters, and tuning these can lead to myriad fascinating electronic and magnetic ground…

In the lacunar spinel GaV4S8, the interplay of spin, charge, and orbital degrees of freedom produces a rich phase diagram that includes an unusual Neel-type skyrmion phase composed of molecular spins. To provide insight into the…

The orientation of N\'eel-type skyrmions in the lacunar spinels GaV$_4$S$_8$ and GaV$_4$Se$_8$ is tied to the polar axes of their underlying crystal structure through the Dzyaloshinskii-Moriya interaction. In these crystals, the skyrmion…

Strongly Correlated Electrons · Physics 2020-09-04 B. Gross , S. Philipp , K. Geirhos , A. Mehlin , S. Bordács V. Tsurkan , A. Leonov , I. Kézsmárki , M. Poggio

The lacunar spinel GeV4S8 undergoes orbital and ferroelectric ordering at the Jahn-Teller transition around 30 K and exhibits antiferromagnetic order below about 14 K. In addition to this orbitally driven ferroelectricity, lacunar spinels…

Strongly Correlated Electrons · Physics 2017-01-23 S. Widmann , A. Günther , E. Ruff , V. Tsurkan , H. -A. Krug von Nidda , P. Lunkenheimer , A. Loidl

We have carried out neutron diffraction and small angle neutron scattering measurements on a high quality single crystal of the cubic lacunar spinel multiferroic, GaV$_4$S$_8$, as a function of magnetic field and temperature to determine…

We report small-angle neutron scattering studies of the lacunar spinel GaV$_4$S$_8$, which reveal the long-wavelength magnetic states to be cycloidally modulated. This provides direct support for the formation of N\'eel-type skyrmions…

Strongly Correlated Electrons · Physics 2018-01-10 J. S. White , Á. Butykai , R. Cubitt , D. Honecker , C. D. Dewhurst , L. F. Kiss , V. Tsurkan , S. Bordács

GaV$_4$S$_8$ is a multiferroic semiconductor hosting N{\'e}el-type magnetic skyrmions dressed with electric polarization. At T$_s$ = 42K, the compound undergoes a structural phase transition of weakly first-order, from a non-centrosymmetric…

The identification of general principles for stabilizing magnetic skyrmion phases in bulk materials over wide ranges of temperatures is a prerequisite to the development of skyrmion-based spintronic devices. Lacunar spinels with the formula…

Materials Science · Physics 2020-02-12 Daniil A. Kitchaev , Emily C. Schueller , Anton Van der Ven

The double exchange (DE) model is systematically applied for studying the coupling between ferroelectric (FE) and magnetic orders in several prototypical types of multiferroic manganites. The model was constructed for the magnetically…

Strongly Correlated Electrons · Physics 2014-11-26 I. V. Solovyev , S. A. Nikolaev

The magnetic susceptibility and spin-spin correlation of the double-exchange model for doped manganites are investigated through the Monte Carlo calculations on the three-dimensional lattice model. Deviations of the susceptibility from the…

Strongly Correlated Electrons · Physics 2009-10-31 Hongsuk Yi , N. H. Hur , Jaejun Yu

We introduce a microscopic model which unravels the physical mechanisms responsible for the observed phase diagram of the $R$VO$_3$ perovskites. It reveals a nontrivial interplay between superexchange, the orbital-lattice coupling due to…

Strongly Correlated Electrons · Physics 2009-11-13 Peter Horsch , Andrzej M. Oles' , Louis Felix Feiner , Giniyat Khaliullin

Radiative polarization of electrons and positrons through the Sokolov-Ternov effect is important for applications in high-energy physics. Radiative spin-polarization is a manifestation of quantum radiation reaction affecting the…

High Energy Physics - Phenomenology · Physics 2018-08-29 D. Seipt , D. Del Sorbo , C. P. Ridgers , A. G. R. Thomas
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