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Photoemission orbital tomography provides direct access from laboratory measurements to the real-space molecular orbitals of well-ordered organic semiconductor layers. Specifically, the application of phase retrieval algorithms to…

Materials Science · Physics 2024-04-29 Thi Lan Dinh , G. S. Matthijs Jansen , D. Russell Luke , Wiebke Bennecke , Stefan Mathias

Electronic wave functions of planar molecules can be reconstructed via inverse Fourier transform of angle-resolved photoelectron spectroscopy (ARPES) data, provided the phase of the electron wave in the detector plane is known. Since the…

Other Condensed Matter · Physics 2016-09-23 Pavel Kliuiev , Tatiana Latychevskaia , Juerg Osterwalder , Matthias Hengsberger , Luca Castiglioni

Conventional photoemission orbital tomography based on Fourier iterative method enables us to extract a projected two-dimensional (2D) molecular orbital from a 2D photoelectron momentum map (PMM) of planar $\pi$-conjugated molecules in a…

Materials Science · Physics 2024-03-01 Misa Nozaki , Takehisa Konishi

High harmonic generation in the interaction of femtosecond lasers with atoms and molecules opens the path to molecular orbital tomography and to probe the electronic dynamics with attosecond-{\AA}ngstr\"{o}m resolutions. Molecular orbital…

A method for photoacoustic tomography is presented that uses circular integrals of the acoustic wave for the reconstruction of a three-dimensional image. Image reconstruction is a two-step process: In the first step data from a stack of…

Numerical Analysis · Mathematics 2009-12-06 G. Zangerl , O. Scherzer , M. Haltmeier

We demonstrate to image asymmetric molecular orbitals via high-order harmonic generation in a one-color inhomogeneous field. Due to the broken inversion symmetry of the inhomogeneous field in space, the returning electrons with energy in a…

Optics · Physics 2018-03-14 Hua Yuan , Lixin He , Feng Wang , Baoning Wang , Xiaosong Zhu , Pengfei Lan , Peixiang Lu

With angle resolved photoemission experiments and \emph{ab-initio} electronic structure calculations, the pentacene monolayers on Ag(110) and Cu(110) are compared and contrasted allowing the molecular orientation and an unambiguous…

Photoelectron spectroscopy in intense laser fields has proven to be a powerful tool for providing detailed insights into molecular structure. The ionizing molecular orbital, however, has not been reconstructed from the photoelectron…

Atomic Physics · Physics 2023-04-14 XuanYang Lai , RenPing Sun , ShaoGang Yu , YanLan Wang , Wei Quan , André Staudte , XiaoJun Liu

We present energy-resolved photoelectron momentum maps for orbital tomography that have been collected with a novel and efficient time-of-flight momentum microscopy setup. This setup is combined with a 0.5 MHz table-top femtosecond…

Photoemission orbital tomography (POT) from photoelectron momentum maps (PMMs) has enabled detailed analysis of the shape and energy of molecular orbitals in the adsorbed state. This study proposes a new POT method based on the PhaseLift.…

Materials Science · Physics 2025-06-03 Kaori Niki , Rena Asano , Ryuji Sakanoue , Manabu Hagiwara , Kazushi Mimura

We propose a new method to overcome the nodal plane problem for the tomographic reconstruction of molecular orbitals with twofold mirror antisymmetry in the length form based on high-order harmonic generation. It is shown that, by carrying…

Chemical Physics · Physics 2013-04-30 Xiaosong Zhu , Meiyan Qin , Yang Li , Qingbin Zhang , Zhizhan Xu , Peixiang Lu

This paper provides a tutorial of iterative phase retrieval algorithms based on the Gerchberg-Saxton (GS) algorithm applied in digital holography. In addition, a novel GS-based algorithm that allows reconstruction of 3D samples is…

Optics · Physics 2019-11-19 Tatiana Latychevskaia

The use of plane wave approximation in molecular orbital tomography via high-order harmonic generation has been questioned since it was proposed, owing to the fact that it ignores the essential property of the continuum wave function. To…

Atomic Physics · Physics 2015-06-18 Yang Li , Xiaosong Zhu , Pengfei Lan , Qingbin Zhang , Meiyan Qin , Peixiang Lu

Inverse boundary value problems for the radiative transport equation play important roles in optics-based medical imaging techniques such as diffuse optical tomography (DOT) and fluorescence optical tomography (FOT). Despite the rapid…

Numerical Analysis · Mathematics 2015-06-19 Tian Ding , Kui Ren

A unified method for three-dimensional reconstruction of objects from transmission images collected at multiple illumination directions is described. The method may be applicable to experimental conditions relevant to absorption-based,…

Medical Physics · Physics 2022-12-07 Timur E. Gureyev , Hamish G. Brown , Harry M. Quiney , Leslie J. Allen

Reconstructing 3D distributions from their 2D projections is a ubiquitous problem in various scientific fields, particularly so in observational astronomy. In this work, we present a new approach to solving this problem: a Vienna…

Instrumentation and Methods for Astrophysics · Physics 2020-01-22 B. Hasenberger , J. Alves

Doppler tomography is a method to compute the emissivity distribution within the co-rotating frames of binary stars from observations of their emission line profiles at multiple orbital phases. A key assumption of the method as it is…

Solar and Stellar Astrophysics · Physics 2021-12-08 T. R. Marsh

We consider the imaging problem of the reconstruction of a three-dimensional object via optical diffraction tomography under the assumptions of the Born approximation. Our focus lies in the situation that a rigid object performs an…

Numerical Analysis · Mathematics 2024-07-11 Robert Beinert , Michael Quellmalz

Optical molecular tomographic imaging is to reconstruct the concentration distribution of photon-molecular probes in a small animal from measured photon fluence rates. The localization and quantification of molecular probes is related to…

Biological Physics · Physics 2017-07-18 Wenxiang Cong , Xavier Intes , Ge Wang

I propose an iterative expectation maximization algorithm for reconstructing a quantum optical ensemble from a set of balanced homodyne measurements performed on an optical state. The algorithm applies directly to the acquired data,…

Quantum Physics · Physics 2009-11-10 A. I. Lvovsky
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