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Ultrafast processes in matter, such as the electron emission following light absorption, can now be studied using ultrashort light pulses of attosecond duration ($10^{-18}$s) in the extreme ultraviolet spectral range. The lack of spectral…

We study orientation and two-center interference effects in attosecond time-resolved photoionization of the H$_2$ molecule. Time resolution of XUV ionization of H$_2$ is gained through the phase retrieval capability of attosecond angular…

Atomic Physics · Physics 2026-03-03 Vladislav V. Serov , Anatoli S. Kheifets

We present angular distributions of photoelectrons of atomic model systems excited by intense linearly polarized laser pulses in the VUV- and XUV-regime. We solve the multi-dimensional time-dependent Schr\"odinger equation for one particle…

Atomic Physics · Physics 2010-03-16 S. Bauch , M. Bonitz

In attosecond streaking, an electron is released by a short xuv pulse into a strong near infrared laser field. When the laser coupling between two states in the target is weak relative to the detuning, the streaking technique, which allows…

Atomic Physics · Physics 2015-05-19 Jan Conrad Baggesen , Lars Bojer Madsen

We use orthogonally polarized two-colour (OTC) laser pulses to separate quantum paths in multiphoton ionization of Ar atoms. Our OTC pulses consist of 400~nm and 800~nm light at a relative intensity ratio of 10:1. We find a hitherto…

We consider tunnel ionization of atomic argon in a femtosecond laser pulse of intensity $10^{21}-10^{22}{\rm W/cm}^2$ aiming to investigate the relativistic dynamics and radiation of photoelectrons released from their parent ions inside the…

Atomic Physics · Physics 2026-02-05 N. V. Makarenko , S. V. Popruzhenko

We theoretically study dissociative ionization of H$_2^+$ exposed to strong linearly polarized few-cycle visible, near-infrared and midinfrared laser pulses. We find rich energy-sharing structures in the combined electron and nuclear…

Atomic Physics · Physics 2016-03-15 Lun Yue , Lars Bojer Madsen

We explore the possibility of retrieving Auger spectra with FEL radiation. Using a laser pulse of 260 eV photon energy, we study the interplay of photo-ionization and Auger processes following the initial formation of a 2p inner-shell hole…

Atomic Physics · Physics 2015-06-19 Alisdair O. G. Wallis , L. Lodi , A. Emmanouilidou

Attosecond interferometry in a two-color field is central to attosecond metrology and spectroscopy. In this technique, a photoelectron wave packet is released when a single photon from an extreme ultraviolet comb is absorbed. The wave…

By analyzing ``exact'' theoretical results from solving the time-dependent Schr\"odinger equation of atoms in few-cycle laser pulses, we established the general conclusion that differential elastic scattering and photo-recombination cross…

Atomic Physics · Physics 2008-04-04 Toru Morishita , Anh-Thu Le , Zhangjin Chen , C. D. Lin

Photoionization by attosecond (as) extreme ultraviolet (xuv) pulses into the laser-dressed continuum of the ionized atom is commonly described in strong-field approximation (SFA), neglecting the Coulomb interaction between the emitted…

Atomic and Molecular Clusters · Physics 2015-05-20 C. -H. Zhang , U. Thumm

Photoelectron spectroscopy is a powerful method that provides insight into the quantum mechanical properties of a wide range of systems. The ionized electron wavefunction carries information on the structure of the bound orbital, the ionic…

We present an experimental study on the photoionization dynamics of non-resonant one-color two-photon single valence ionization of neutral argon atoms. Using 9.3 eV photons produced via high harmonic generation and a 3-D momentum imaging…

Atomic Physics · Physics 2020-08-28 Kirk A. Larsen , Daniel S. Slaughter , Thorsten Weber

Interplay of the angle dependent X-ray reflectivity and absorption with the photoelectron attenuation length in the photoelectron emission process determine the optimal X-ray incidence angle which maximizes the photoelectron signal.…

Instrumentation and Detectors · Physics 2012-12-18 Vladimir N. Strocov

We consider the ionization of neon induced by a femtosecond laser pulse composed of overlapping, linearly polarized bichromatic extreme ultraviolet and infrared fields. In particular, we study the effects of the infrared light on a…

Atomic Physics · Physics 2017-01-25 Nicolas Douguet , Alexei N. Grum-Grzhimailo , Klaus Bartschat

We report on the observation of subcycle interferences of electron wave packets released during the strong field ionization of H$_2$ with cycle-shaped two-color laser fields. With a reaction microscope, channel-resolved photoelectron…

Chemical Physics · Physics 2016-12-08 Xinhua Xie , Stefan Roither , Daniil Kartashov , Li Zhang , Andrius Baltuška , Markus Kitzler

The photoelectron momentum distribution in the strong-field ionization has a variety of structures that reveal the complicated dynamics of this process. Recently, we identified a low-energy interference structure in the case of a…

Atomic Physics · Physics 2022-04-27 Lei Geng , Hao Liang , Liang-You Peng

We investigated the complex index of refraction in the x-ray regime of atoms in laser light. The laser (intensity up to 10^13 W/cm^2, wavelength 800nm) modifies the atomic states but, by assumption, does not excite or ionize the atoms in…

Atomic Physics · Physics 2008-11-18 Christian Buth , Robin Santra

We present a new extension of the UKRmol electron-molecule scattering code suite, which allows one to compute ab initio photoionization and photorecombination amplitudes for complex molecules, resolved both on the molecular alignment…

Chemical Physics · Physics 2014-02-18 Alex G Harvey , Danilo S Brambila , Felipe Morales , Olga Smirnova

The development of attosecond technology has enabled the real-time observation of coherent electron motion in atoms, molecules and condensed phases. Experimentally, it is now possible to generate laser pulses of durations of only a few tens…

Chemical Physics · Physics 2017-05-18 David Ayuso