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Experimental quest for the hypothetical "quantum spin liquid" state has recently met a few promising candidate materials including organic salts \kappa-(ET)2Cu2(CN)3 and EtMe3Sb[Pd(dmit)2]2, S=1/2 triangular-lattice Heisenberg…
The effects of pressure on a quantum spin liquid are investigated in an organic Mott insulator $\kappa$-(ET)$_2$Ag$_2$(CN)$_3$ with a spin-1/2 triangular lattice. The application of negative chemical pressure to…
Quantum spin liquids (QSLs) represent a novel state where spins are highly entangled but do not order even at zero temperature due to strong quantum fluctuations. Such a state is mostly studied in Heisenberg models defined on geometrically…
We present microscopic magnetic properties of a two dimensional triangular lattice Sc2Ga2CuO7, consisting of single and double triangular Cu planes. A Curie-Weiss temperature theta_CW = --44 K and an antiferromagnetic (AFM) exchange…
Disordered magnetic states known as spin liquids are of paramount importance in both fundamental and applied science. A classical state of this kind was predicted for the Ising antiferromagnetic triangular model more than half a century…
A quantum spin liquid (QSL) is an exotic state in which electron spins are highly entangled, yet keep fluctuating even at zero temperature. Experimental realization of model QSLs has been challenging due to imperfections, such as antisite…
The molecular triangular lattice system, beta'-EtMe3Sb[Pd(dmit)2]2, is considered as a candidate material for the quantum spin liquid (QSL) state, although ongoing debates arise from recent controversial results. Here, the results of…
Quantum spin liquids~(QSLs) represent a unique quantum disordered state of matter that hosts long-range quantum entanglement and fractional excitations. However, structural disorder resulting from site mixing between different types of ions…
Organic salts represent an ideal experimental playground for studying the interplay between magnetic and charge degrees of freedom, which has culminated in the discovery of several spin-liquid candidates, such as…
The existence of a quantum spin liquid (QSL) in which quantum fluctuations of spins are sufficiently strong to preclude spin ordering down to zero temperature was originally proposed theoretically more than 40 years ago, but its…
We investigate the anisotropic triangular lattice that interpolates from decoupled one-dimensional chains to the isotropic triangular lattice and has been suggested to be relevant for various quasi-two-dimensional materials, such as…
A quantum spin liquid (QSL) is a state of matter characterized by fractionalized quasiparticle excitations, quantum entanglement, and a lack of long-range magnetic order. However, QSLs have evaded definitive experimental observation.…
Although magnetically ordered at low temperatures, the spin-1/2 triangular antiferromagnet Cs_2CuCl_4 exhibits remarkable spin dynamics that strongly suggest proximity to a spin liquid phase. Here we address the question of whether a…
A quantum spin liquid (QSL) is an exotic state of matter in which electrons' spins are quantum entangled over long distances, but do not show symmetry-breaking magnetic order in the zero-temperature limit. The observation of QSL states is a…
The quasi-two-dimensional organic charge-transfer salt $\kappa$-(BEDT-TTF)$_2$Cu$_2$(CN)$_3$ is one of the prime candidates for a quantum spin-liquid due the strong spin frustration of its anisotropic triangular lattice in combination with…
The absence of conventional magnetic order together with anomalous low-temperature magnetic heat capacity is often interpreted as evidence for quantum spin liquid ground states in frustrated magnets. Using a recently developed semiclassical…
The layered triangular lattice owing to $1:2$ order of $B$ and $B'$ sites in the triple perovskite $A_3 B B'_2$O$_9$ family provides an enticing domain for exploring the complex phenomena of quantum spin liquids (QSLs). We report a…
A quantum spin liquid (QSL) is a state of matter where unpaired electrons' spins in a solid are quantum entangled, but do not show magnetic order in the zero-temperature limit. Because such a state may be important to the microscopic origin…
A quantum spin liquid (QSL) is a state of matter in which magnetic spins interact strongly, but quantum fluctuations inhibit long-range magnetic order even at zero temperature. A QSL has been predicted to have a host of exotic properties,…
The quantum spin liquid (QSL) is a highly entangled magnetic state characterized by the absence of static magnetism in its ground state. Instead, the spins fluctuate in a highly correlated way down to the lowest temperatures. The QSL is…