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In this work, we introduce the platform of plasmonic Doppler grating (PDG) to experimentally investigate the enhancement effect of plasmonic gratings in the input and output beams of nonlinear surface-enhanced coherent anti-Stokes Raman…

Surface plasmon resonance (SPR) has been widely utilized to improve the absorption performance in the photosensors. Graphene has emerged as a promising plasmonic material, which supports tunable SPR and shows significant flexibility over…

Optics · Physics 2018-09-11 Shuyuan Xiao , Tao Wang , Xiaoyun Jiang , Boyun Wang , Chen Xu

A quantum-mechanical model to calculate the electron energy-loss spectra (EELS) for the system of a closely located metallic nanoshell and a molecule has been developed. At the resonance between the molecular excitation and plasmon modes in…

Atomic Physics · Physics 2014-10-07 I. Yu. Goliney , Ye. V. Onykienko

We perform local nanoscale studies of the surface and interface structure of hydrogen intercalated graphene on 4H-SiC(1000). In particular, we show that intercalation of the interfacial layer results in the formation of quasi-free standing…

Materials Science · Physics 2018-04-27 Christos Melios , Steve Spencer , Alex Shard , Wlodek Strupinski , S. Ravi P. Silva , Olga Kazakova

Creating plasmonic nanoparticles on a tapered optical fiber tip enables a remote SERS sensing probe, ideal for challenging sampling scenarios like biological tissue, specific cells, on-site environmental monitoring, and deep brain…

Broadening of the Raman scattering (RS) spectra was studied in monolayer graphene samples irradiated with various dose of ions followed by annealing of radiation damage at different temperatures. It is shown that the width {\Gamma} (full…

Mesoscale and Nanoscale Physics · Physics 2019-12-13 I. Shlimak , A. Butenko , E. Kogan , M. Kaveh

Resonant dielectric nanoparticles (RDNs) made of materials with large positive dielectric permittivity, such as Si, GaP, GaAs, have become a powerful platform for modern light science, enabling various fascinating applications in…

Optics · Physics 2017-10-30 Alex Krasnok , Martin Caldarola , Nicolas Bonod , Andrea Alú

We examine SERS from two perspectives: as a phenomenon described by the Laplace Equation (the electrostatic or Rayleigh limit) and by the Helmholtz Equation (electrodynamic or Mie limit). We formulate the problem in terms of the scalar…

Optics · Physics 2011-09-14 E. J. Adles , S. Franzen , D. E. Aspnes

Micro-ring resonators (MRRs) "trap" incoming light, and therefore, have been shown to achieve extremely high local intensities of light. Thus, they can be used to facilitate highly non-linear optical signals. By embedding materials that…

Mesoscale and Nanoscale Physics · Physics 2024-09-04 A. Sharma , Y. Li , M. K. Prasad , W. L. Ho , S. T. Chu , I. V. Borzenets

Nanogaps are ubiquitous across science, confining molecules and thus changing chemistries which influence many areas such as catalysis, corrosion, photochemistry, and sensing. However in ambient conditions, it is unclear how water solvates…

Due to their high circulating intensities, ultra-high quality factor dielectric whispering-gallery mode resonators have enabled the development of low threshold Raman microlasers. Subsequently, other Raman-related phenomena, such as…

Accurate detection and analysis of traces of persistent organic pollutants in water is important in many areas, including environmental monitoring and food quality control, due to their long environmental stability and potential…

Machine Learning · Computer Science 2024-02-02 Vishnu Jayaprakash , Jae Bem You , Chiranjeevi Kanike , Jinfeng Liu , Christopher McCallum , Xuehua Zhang

We provide the theoretical framework to understand the phenomenology and statistics of single-molecule (SM) signals arising in Surface-Enhanced Raman Scattering (SERS) under the presence of so-called electromagnetic hot-spots (HS's). We…

Chemical Physics · Physics 2009-11-13 E. C. Le Ru , P. G. Etchegoin , M. Meyer

A mechanism for additional enhancement of SERS in the nanoparticle-on-mirror scheme is proposed. This new mechanism is based on the use of a substrate made of material with a near-minus-one permittivity. The setup involves a plasmonic…

Optics · Physics 2026-05-11 Alexey P. Vinogradov , Evgeny S. Andrianov

Accurate design of labelled oligo probes for the detection of miRNA biomarkers by Surface Enhanced Raman Scattering (SERS) may improve the exploitation of the plasmonic enhancement. This work, thus, critically investigates the role of probe…

The physical processes associated with propagation of a high-power (power > critical power for self-focusing) laser beam in water include nonlinear focusing, stimulated Raman scattering (SRS), optical breakdown and plasma formation. The…

Surface-enhanced coherent anti-Stokes Raman scattering (SE-CARS) takes advantage of surface plasmon resonances supported on metallic nanostructures to amplify the coherent Raman response of target molecules. While these metallic antennas…

Optics · Physics 2022-09-07 Shamsul Abedin , Yong Li , Abid Anjum Sifat , Khokan Roy , Eric Olaf Potma

The synthesis of polyynes during their formation by pulsed laser ablation in liquid (i.e. acetonitrile) has been analyzed by in-situ surface-enhanced Raman spectroscopy (SERS). A polyethylene pellet, functionalized with silver nanoparticles…

Recent advancements in nanotechnology have led to the development of surface-enhanced Raman spectroscopy (SERS) based rapid and low-cost technologies for ultra-sensitive label-free detection and identification of molecular analytes. Herein,…

Characterizing a monolayer of biological molecules has been a major challenge. We demonstrate nanophotonic wave-guide enhanced Raman spectroscopy (NWERS) of monolayers in the near-infrared region, enabling real-time measurements of the…

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