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We theoretically study resonance responses of flat surfaces and sharp edges of the nanostructures that support excitations of phonon-polaritons in mid-infrared range. We focus on two materials: silicon carbide that has a nearly isotropic…

Optics · Physics 2017-09-20 Viktoriia E. Babicheva

Monolayer hexagonal boron nitride (hBN) has recently become the focus of intense research as a material to host quantum emitters. Although it is well known that such emission is associated with point defects, so far no conclusive…

The advent of monochromated electron energy-loss spectroscopy has enabled atomic-resolution vibrational spectroscopy, which triggered interest in spatially localized or quasi-localized vibrational modes in materials. Here we report the…

Materials Science · Physics 2023-10-13 De-Liang Bao , Mingquan Xu , Ao-Wen Li , Gang Su , Wu Zhou , Sokrates T. Pantelides

Hyperbolic phonon polaritons (HPhPs) in orthorhombic-phase molybdenum trioxide ($\alpha$-MoO3) show in-plane hyperbolicity, great wavelength compression and ultra-long lifetime, therefore holding great potential in nanophotonic…

Materials Science · Physics 2020-11-25 Weikang Dong , Ruishi Qi , Tiansheng Liu , Yi Li , Ning Li , Ze Hua , Zirui Gao , Shuyuan Zhang , Kaihui Liu , Jiandong Guo , Peng Gao

Van der Waals heterostructures assembled from layers of 2D materials have attracted considerable interest due to their novel optical and electrical properties. Here we report a scattering-type scanning near field optical microscopy study of…

We investigate optical nonlinearities that are induced and enhanced due to the strong phonon resonance in hexagonal boron nitride. We predict and observe large sub-picosecond duration signals due to four-wave mixing (FWM) during resonant…

Phonon polaritons (PhPs),light coupled to lattice vibrations,with in-plane hyperbolic dispersion exhibit ray-like propagation with large wavevectors and enhanced density of optical states along certain directions on a surface. As such, they…

We propose to use optical antennas made out of natural hyperbolic material hexagonal boron nitride (hBN), and we demonstrate that this medium is a promising alternative to plasmonic and all-dielectric materials for realizing efficient…

Optics · Physics 2017-06-23 Viktoriia E. Babicheva

Hexagonal boron nitride (h-BN), one of the hallmark van der Waals (vdW) layered crystals with an ensemble of attractive physical properties, is playing increasingly important roles in exploring two-dimensional (2D) electronics, photonics,…

Mesoscale and Nanoscale Physics · Physics 2020-01-07 Yanan Wang , Jaesung Lee , Xu-Qian Zheng , Yong Xie , Philip X. -L. Feng

Hexagonal boron nitride (hBN)-long-known as a thermally stable ceramic-is now available as atomically smooth, single-crystalline flakes, revolutionizing its use in optoelectronics. For nanophotonics, these flakes offer strong…

Heterostructures of van der Waals bonded layered materials offer unique means to tailor dielectric screening with atomic-layer precision, opening a fertile field of fundamental research. The optical analyses used so far have relied on…

Hexagonal boron nitride is a wide bandgap semiconductor with a very high thermal and chemical stability often used in devices operating under extreme conditions. The growth of high-purity crystals has recently revealed the potential of this…

Materials Science · Physics 2016-05-04 G. Cassabois , P. Valvin , B. Gil

Aligned, densely-packed carbon nanotube metamaterials prepared using vacuum filtration are an emerging infrared nanophotonic material. We report multiple hyperbolic plasmon resonances, together spanning the mid-infrared, in individual…

Van-der-Waals materials have been shown to support numerous exotic polaritonic phenomena originating from their layered structures and associated vibrational and electronic properties. This includes emergent polaritonic phenomena, including…

Boron nitride exhibits diverse crystal structures, predominantly a layered arrangement with strong intraplanar covalent bonds and weak interplanar van der Waals bonds. While commonly referred to as hexagonal BN (hBN), the sp$^2$-bonded BN…

We report three-dimensional (3D) structure determination of a twisted hexagonal boron nitride (h-BN) heterointerface from a single-view data set using multislice ptychography. We identify the buried heterointerface between two twisted h-BN…

Extreme confinement of electromagnetic energy by phonon polaritons holds the promise of strong and new forms of control over the dynamics of matter. To bring such control to the atomic-scale limit, it is important to consider phonon…

Mesoscale and Nanoscale Physics · Physics 2019-05-01 Nicholas Rivera , Thomas Christensen , Prineha Narang

Polaritons travelling along a hyperbolic medium's surface have recently sparked significant interest in nanophotonics for the unprecedented manipulation ability on light at the nanoscale in a planar way, promising potential nano-optical…

Bismuth nanostructures are appealing for sustainable color generation and sunlight harvesting, thanks to their non-toxicity and their tunable visible-to-near infrared interband plasmon resonances. However, owing to their broad and…

Stacking mismatches in hexagonal boron nitride (h-BN) nanostructures affect their photonic, mechanical, and thermal properties. To access information about the stacked configuration of layered ensembles, highly sophisticated techniques like…

Materials Science · Physics 2021-03-03 Luigi Cigarini , Michal Novotný , František Karlický
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