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Quantum mechanics/molecular mechanics (QM/MM) hybrid models allow one to address chemical phenomena in complex molecular environments. Whereas this modeling approach can cope with a large system size at moderate computational costs, the…

Computational Physics · Physics 2023-01-10 Katja-Sophia Csizi , Markus Reiher

The predictions of the geometric collective model (GCM) for different sets of Hamiltonian parameter values are related by analytic scaling relations. For the quartic truncated form of the GCM -- which describes harmonic oscillator, rotor,…

Nuclear Theory · Physics 2007-05-23 M. A. Caprio

The scaling of the viscosity of polymer melts is investigated with regard to the molecular weight. We present a generalization of the Rubinstein-Duke model, which takes constraint releases into account and calculate the effects on the…

Statistical Mechanics · Physics 2009-11-07 Matthias Paessens , Gunter M. Schuetz

A simple application of classical density functional theory is derived and applied to a system of polymers grafted to a plane. The system is assumed to have symmetry in directions parallel to the grafting plane hence it being a…

Soft Condensed Matter · Physics 2016-12-02 Luke Kristopher Davis

Soft membranes are commonly employed in shape-morphing applications, where the material is programmed to achieve a target shape upon activation by an external trigger, and as coating layers that alter the surface characteristics of bulk…

Soft Condensed Matter · Physics 2016-02-05 Alessandro Lucantonio , Luciano Teresi , Antonio DeSimone

A series of aspects of the quantum gravity predict a modification in the Heisenberg uncertainty principle to the generalized uncertainty principle (GUP). In the present work, using the momentum space representation, we study the behavior of…

High Energy Physics - Theory · Physics 2018-08-01 Bing-Qian Wang , Zheng-Wen Long , Chao-Yun Long , Shu-Rui Wu

Molecular dynamics simulation methods are used to study the folding of polymer chains into packed cubic states. The polymer model, based on a chain of linked sites moving in the continuum, includes both excluded volume and torsional…

Soft Condensed Matter · Physics 2009-11-10 D. C. Rapaport

Spherical symmetry is ubiquitous in nature. It's therefore unfortunate that spherical system simulations are so hard, and require complete spheres with millions of interacting particles. Here we introduce an approach to model spherical…

Materials Science · Physics 2011-10-07 Pekka Koskinen , Oleg O. Kit

The statistical-physical study of granular matter is essential to understand, from a fundamental point of view, the many different phenomena emerging in these classical many-body systems. Under rapid-flow conditions, granular materials…

Soft Condensed Matter · Physics 2023-10-23 Alberto Megías

In this paper we study the shape characteristics of star-like polymers in various solvent quality using a mesoscopic level of modeling. The dissipative particle dynamics simulations are performed for the homogeneous and four different…

Soft Condensed Matter · Physics 2020-03-24 O. Kalyuzhnyi , J. M. Ilnytskyi , Yu. Holovatch , C. von Ferber

The success of the Materials Genome Initiative has led to opportunities for data-driven approaches for materials discovery. The recent development of Polymer Genome (PG), which is a machine learning (ML) based data-driven informatics…

Computational Physics · Physics 2019-08-08 Manav Ramprasad , Chiho Kim

Vitrimer is an emerging class of sustainable polymers with self-healing capabilities enabled by dynamic covalent adaptive networks. However, their limited molecular diversity constrains their property space and potential applications.…

We analyze structural and conformational properties in a simulated bead-spring model of a non-entangled, supercooled polymer melt. We explore the statics of the model via various structure factors, involving not only the monomers, but also…

Soft Condensed Matter · Physics 2009-11-10 Martin Aichele , Song-Ho Chong , Jörg Baschnagel , Matthias Fuchs

Synthetic polymers are versatile and widely used materials. Similar to small organic molecules, a large chemical space of such materials is hypothetically accessible. Computational property prediction and virtual screening can accelerate…

Machine Learning · Computer Science 2022-10-13 Matteo Aldeghi , Connor W. Coley

We present a quantum mechanical / molecular mechanics (QM/MM) to tackle chemical reactions with substantial molecular reorganization. For this, molecular dynamics simulations with smoothly switched interaction models are used to suggest…

Soft Condensed Matter · Physics 2020-11-06 Robert H. Meißner , Julian Konrad , Benjamin Boll , Bodo Fiedler , Dirk Zahn

The specific heat is a central property of condensed matter systems including polymers and oligomers in their condensed phases. Yet, predictions of this quantity from molecular simulations and successful comparisons to experimental data are…

Soft Condensed Matter · Physics 2021-06-30 Hongyu Gao , Tobias P. W. Menzel , Martin H. Mueser , Debashish Mukherji

The family of Mat\'ern kernels are often used in spatial statistics, function approximation and Gaussian process methods in machine learning. One reason for their popularity is the presence of a smoothness parameter that controls, for…

Statistics Theory · Mathematics 2025-06-06 Moritz Korte-Stapff , Toni Karvonen , Eric Moulines

The miscibility in several polymer blend mixtures (polymethylmethacrylate/polystyrene, (1,4-cis) polyisoprene/polystyrene, and polymethylmethacrylate/polyoxyethylene) has been investigated using Molecular Dynamics simulations for atomistic…

Chemical Physics · Physics 2009-05-29 Amirhossein Ahmadi , Juan J. Freire

For optimal processing and design of entangled polymeric materials it is important to establish a rigorous link between the detailed molecular composition of the polymer and the viscoelastic properties of the macroscopic melt. We review…

Soft Condensed Matter · Physics 2015-05-27 J. T. Padding , W. J. Briels

Knitting is an effective technique for producing complex three-dimensional surfaces owing to the inherent flexibility of interlooped yarns and recent advances in manufacturing providing better control of local stitch patterns. Fully…

Numerical Analysis · Mathematics 2022-06-20 Sumudu Herath , Xiao Xiao , Fehmi Cirak
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