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Transitions of many-particle quantum systems between distinct phases at absolute-zero temperature, known as quantum phase transitions, require an exacting treatment of particle correlations. In this work, we present a general…

Quantum Physics · Physics 2022-07-29 Samuel Warren , LeeAnn M. Sager-Smith , David A. Mazziotti

We design two-dimensional (2D) mechanical metamaterials that may be deformed substantially at little or no energy cost. Examples of such deformable structures are assemblies of rigid isosceles triangles hinged in their corners on the…

Mesoscale and Nanoscale Physics · Physics 2018-12-21 Zhibin Gao , Dan Liu , David Tomanek

Density-functional theory (DFT) has revolutionized computer simulations in chemistry and material science. A faithful implementation of the theory requires self-consistent calculations. However, this effort involves repeatedly diagonalizing…

Quantum Physics · Physics 2023-07-17 Taehee Ko , Xiantao Li , Chunhao Wang

Using density functional theory (DFT), we investigate mechanical properties of a few 2D metal-organic frameworks (MOFs) and covalent-organic frameworks (COFs) having Dirac and flat bands. These porous materials have become a subject of…

Materials Science · Physics 2023-03-15 Priyadarshini Kapri , Takuto Kawakami , Mikito Koshino

Within the nuclear DFT approach, we determined the magnetic dipole and electric quadrupole moments for paired nuclear states corresponding to the proton (neutron) quasiparticles blocked in the p11/2- (n13/2+) intruder configurations. We…

Nuclear Theory · Physics 2023-08-22 J. Bonnard , J. Dobaczewski , G. Danneaux , M. Kortelainen

Finding new two-dimensional (2D) materials with novel quantum properties is highly desirable for technological innovations. In this work, we studied a series of metal-organic frameworks (MOFs) with different metal cores and discovered…

Materials Science · Physics 2020-11-17 Jie Li , Ruqian Wu

Density functional theory (DFT) is shown to provide a novel conceptual and computational framework for entanglement in interacting many-body quantum systems. DFT can, in particular, shed light on the intriguing relationship between quantum…

Quantum Physics · Physics 2009-11-11 L. -A. Wu , M. S. Sarandy , D. A. Lidar , L. J. Sham

The advent of bottom-up atomic manipulation heralded a new horizon for attainable information density, as it allowed a bit of information to be represented by a single atom. The discrete spacing between atoms in condensed matter has thus…

Mesoscale and Nanoscale Physics · Physics 2009-11-13 Christopher R. Moon , Laila S. Mattos , Brian K. Foster , Gabriel Zeltzer , Hari C. Manoharan

We perform extensive density functional theory (DFT) calculations to determine the stability and elementary properties of 4249 previously unexplored monolayer crystals. The monolayers comprise the most stable subset (energy within 0.1…

Materials Science · Physics 2024-06-18 Peder Lyngby , Kristian Sommer Thygesen

Multi-dimensional quantum walks can exhibit highly non-trivial topological structure, providing a powerful tool for simulating quantum information and transport systems. We present a flexible implementation of a 2D optical quantum walk on a…

Exotic phenomenon can be achieved in quantum materials by confining electronic states into two dimensions. For example, relativistic fermions are realised in a single layer of carbon atoms, the quantized Hall effect can result from…

In recent decades, scientists have developed the means to engineer synthetic periodic arrays with feature sizes below the wavelength of light. When such features are appropriately structured, electromagnetic radiation can be manipulated in…

Mesoscale and Nanoscale Physics · Physics 2018-11-12 Justin C. W. Song , Nathaniel M. Gabor

The dimensionality of an electronic quantum system is decisive for its properties. In 1D electrons form a Luttinger liquid and in 2D they exhibit the quantum Hall effect. However, very little is known about the behavior of electrons in…

Mesoscale and Nanoscale Physics · Physics 2021-02-23 S. N. Kempkes , M. R. Slot , S. E. Freeney , S. J. M. Zevenhuizen , D. Vanmaekelbergh , I. Swart , C. Morais Smith

Progress towards the energy breakthroughs needed to combat climate change can be significantly accelerated through the efficient simulation of atomic systems. Simulation techniques based on first principles, such as Density Functional…

Machine Learning · Computer Science 2021-06-18 Muhammed Shuaibi , Adeesh Kolluru , Abhishek Das , Aditya Grover , Anuroop Sriram , Zachary Ulissi , C. Lawrence Zitnick

A quantitative and predictive theory of quantum light-matter interactions in ultra thin materials involves several fundamental challenges. Any realistic model must simultaneously account for the ultra-confined plasmonic modes and their…

In this work, we investigate the electronic and magnetic properties of single-layer pentahexoctite, a two-dimensional carbon allotrope patterned by pentagons, hexagons, and octagons. Using density functional theory (DFT) calculations…

Mesoscale and Nanoscale Physics · Physics 2024-05-30 Sejoong Kim

In the near future, material and drug design may be aided by quantum computer assisted simulations. These have the potential to target chemical systems intractable by the most powerful classical computers. However, the resources offered by…

We present a comprehensive first-principles study of the electronic structure of 51 semiconducting monolayer transition metal dichalcogenides and -oxides in the 2H and 1T hexagonal phases. The quasiparticle (QP) band structures with…

Materials Science · Physics 2015-06-10 Filip Anselm Rasmussen , Kristian Sommer Thygesen

Systematically studying the crystal, magnetic, and electronic structures of PuGa3 with density functional theory (DFT) reveals the entanglement of the three types of structure. Magnetic structure affects the energy more strongly than…

Materials Science · Physics 2013-07-03 Sven P. Rudin

Atoms deposited on two-dimensional (2D) electronic materials, such as graphene, can exhibit unconventional many-body correlations, not accessible in other settings. All of these are driven by van der Waals forces: between the atoms…

Mesoscale and Nanoscale Physics · Physics 2022-01-13 Adrian Del Maestro , Carlos Wexler , Juan M. Vanegas , Taras Lakoba , Valeri N. Kotov