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The traditional picture of solid-solid phase transformations assumes an ordered parent phase transforms into an ordered daughter phase via a single unique pathway. Zirconium and its prototypical phase transition from hexagonal close-packed…

The prototypical $\alpha\to\omega$ phase transition in zirconium is an ideal test-bed for our understanding of polymorphism under extreme loading conditions. After half a century of study, a consensus had emerged that the transition is…

Materials Science · Physics 2024-04-30 P. G. Heighway , S. Singh , M. G. Gorman , D. McGonegle , J. H. Eggert , R. F. Smith

We study the relaxation dynamics and intersystem-crossing to the metastable state in laser-pumped tetra and hexa-coordinated nickel porphyrins. We use a ligand-field model which takes into account the crystal field created by the porphyrin…

Strongly Correlated Electrons · Physics 2015-11-29 Javier Fernandez-Rodriguez , Jun Chang , Arthur J. Fedro , Michel van Veenendaal

We have performed a detailed x-ray diffraction structural study of Zr under pressure and unambiguously identify the existence of a first-order isostructural bcc-to-bcc phase transition near 58 GPa. First-principles quantum molecular…

By means of density-functional calculations, we systematically investigated 24 transition metals for possible metastable phases in body-centered tetragonal structure (bct), including face-centered cubic (fcc) and body-centered cubic (bcc)…

Under high pressure conditions, Zr undergoes a phase transformation from its ambient equilibrium hexagonal close packed $\alpha$ phase to hexagonal $\omega$ phase. Upon returning to ambient conditions, the material displays hysteretic…

The thermodynamic stable phase of cerium metal in the intermediate pressure regime (5.0--13.0 GPa) is studied in detail by the newly developed local-density approximation (LDA)+ Gutzwiller method, which can include the strong correlation…

Strongly Correlated Electrons · Physics 2015-04-08 Ming-Feng Tian , Xiaoyu Deng , Zhong Fang , Xi Dai

As titanium is a highly utilized metal for structural light-weighting, its phases, transformation pathways (transition states), and structures have scientific and industrial importance. Impurities, pressure, and temperature control the…

Materials Science · Physics 2017-11-28 N. A. Zarkevich , D. D. Johnson

This study examines the phase transitions occurring during linear heating of the Zr15Nb alloy through a comprehensive, multi-technique methodology comprising in-situ high-energy synchrotron X-ray diffraction (HEXRD), electrical resistance…

We present a computational study of the dynamic behavior of a Ziff-Gulari-Barshad model of CO oxidation with CO desorption on a catalytic surface. Our results provide further evidence that below a critical desorption rate the model exhibits…

Materials Science · Physics 2007-05-23 E. Machado , G. M. Buendia , P. A. Rikvold , R. M. Ziff

The high-pressure phase stability of the metastable tetragonal zirconia is still under debate. The transition dynamics of shocked Y2O3 (3 mol%) stabilized tetragonal zirconia ceramics under laser-shock compression has been directly studied…

Discontinuous quantum phase transitions and the associated metastability play central roles in diverse areas of physics ranging from ferromagnetism to false vacuum decay in the early universe. Using strongly-interacting ultracold atoms in…

Quantum Gases · Physics 2022-04-26 Bo Song , Shovan Dutta , Shaurya Bhave , Jr-Chiun Yu , Edward Carter , Nigel Cooper , Ulrich Schneider

We present a review on the study of metastable silicon, primarily focusing mainly on the aspects of liquid-liquid transition, critical point and phase behaviour, structural and dynamic properties of liquid phase as well as crystal…

Materials Science · Physics 2021-09-01 Vishwas V. Vasisht , Srikanth Sastry

Metastable phases present a promising route to expand the functionality of complex materials. Of particular interest are light-induced metastable phases that are inaccessible under equilibrium conditions, as they often host new, emergent…

We have studied non-equilibrium phase transitions in the vortex lattice in superconducting MgB2, where metastable states are observed in connection with an intrinsically continuous rotation transition. Using small-angle neutron scattering…

Superconductivity · Physics 2019-04-18 E. R. Louden , C. Rastovski , L. DeBeer-Schmitt , C. D. Dewhurst , N. D. Zhigadlo , M. R. Eskildsen

We investigate the phase behavior of a single-component system in 3 dimensions with spherically-symmetric, pairwise-additive, soft-core interactions with an attractive well at a long distance, a repulsive soft-core shoulder at an…

Soft Condensed Matter · Physics 2009-11-07 G. Franzese , G. Malescio , A. Skibinsky , S. V. Buldyrev , H. E. Stanley

We report a simple technique for the synthesis of uniaxially textured, metastable hexagonal close-packed-like uranium thin films with thicknesses between 175-2800 \r{A}. The initial structure and texture of the layers have been studied via…

Materials Science · Physics 2022-10-11 Rebecca Nicholls , Chris Bell , Johann Bouchet , Ross Springell , Gerard H. Lander

The evaluation of phase stabilities of unstable elemental phases is a long-standing problem in the computational assessment of phase diagrams. Here we tackle this problem by explicitly calculating phase diagrams of intermetallic systems…

Materials Science · Physics 2016-09-20 Shmuel Barzilai , Cormac Toher , Stefano Curtarolo , Ohad Levy

We develop a statistical physics theory for solid-solid phase transitions in which a metamaterial undergoes longitudinal contraction in response to increase in external tension. Such transitions, which are forbidden in thermodynamic…

Statistical Mechanics · Physics 2013-05-16 Zachary G. Nicolaou , Adilson E. Motter

We present diffusion Monte Carlo (DMC) results on a new metastable, superfluid phase above the crystal ground state in two-dimensional 4He at densities > 0.065 1/A^2. The state is anisotropic with hexatic orbital order. This implies that…

Other Condensed Matter · Physics 2009-11-13 V. Apaja , M. Saarela
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