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We examine a mechanism by which excitons undergo ultrafast relaxation in common monolayer transition metal dichalcogenides. It is shown that at densities $\approx$ 1$\times$ 10$^{11}$ cm$^{-2}$ and temperatures $ \le 60$ K, excitons in well…

Mesoscale and Nanoscale Physics · Physics 2016-06-29 A. Thilagam

We perform coherent nonlinear spectroscopy of excitons in single-layers of MoSe$_2$ and WSe$_2$ encapsulated between thin films of hexagonal boron nitride. Employing four-wave mixing microscopy we identify virtually disorder free areas,…

The Bose-Einstein condensation of excitons continues to garner immense attention as a prototypical example for observing emergent properties from many-body quantum effects. In particular, Titanium Diselenide (TiSe$_2$) is a promising…

Materials Science · Physics 2019-12-06 Chao Lian , Zulfikhar A. Ali , Bryan M. Wong

Manipulation of intrinsic electron degrees of freedom, such as charge and spin, gives rise to electronics and spintronics, respectively. Electrons in monolayer materials with a honeycomb lattice structure, such as the Transition-Metal…

Strongly Correlated Electrons · Physics 2018-11-27 E. C. Marino , Leandro O. Nascimento , Van Sérgio Alves , N. Menezes , C. Morais Smith

Monolayers of transition-metal dichalcogenides (TMDs) are characterized by an extraordinarily strong Coulomb interaction giving rise to tightly bound excitons with binding energies of hundreds of meV. Excitons dominate the optical response…

Materials Science · Physics 2018-05-30 Samuel Brem , Gunnar Berghaeuser , Malte Selig , Ermin Malic

Conventional methods to measure the dispersion relations of collective spin excitations involve probing bulk samples with particles such as neutrons, photons or electrons, which carry a well-defined momentum. Open-ended finite-size spin…

Mesoscale and Nanoscale Physics · Physics 2025-02-20 J. C. G. Henriques , Chenxiao Zhao , G. Catarina , Pascal Ruffieux , Roman Fasel , J. Fernández-Rossier

Transition metal dichalcogenides (TMDs) exhibit a remarkable exciton physics including optically accessible (bright) as well as spin- and momentum-forbidden (dark) excitonic states. So far the dark exciton landscape has not been revealed…

We present a minimalistic equilateral triangular lattice model, from which we derive electron and exciton band structures for semiconducting transition-metal dichalcogenides. With explicit consideration of the exchange interaction, this…

Mesoscale and Nanoscale Physics · Physics 2026-05-12 Daniel Gunlycke , Frank Tseng

We study the screened dynamics of the nonequilibrium excitonic consensate forming in a bulk WSe$_{2}$ when illuminated by coherent light resonant with the lowest-energy exciton. Intervalley scattering causes electron migration from the…

Mesoscale and Nanoscale Physics · Physics 2021-06-16 E. Perfetto , G. Stefanucci

We investigate excitons in stacked transition metal dichalcogenide (TMDC) layers under perpendicularly applied electric field, herein MoSe$_2$/WSe$_2$ van der Waals heterostructures. Band structures are obtained with density functional…

Mesoscale and Nanoscale Physics · Physics 2018-09-19 A. Chaves , J. G. Azadani , V. Ongun Özçelik , R. Grassi , T. Low

Moir\'{e} twist angle underpins the interlayer interaction of excitons in twisted van der Waals hetero- and homo-structures. The influence of twist angle on the excitonic absorption of twisted bilayer tungsten diselenide (WSe$_{2}$) has…

Microcavity electron-hole-photon systems in two-dimensions are long anticipated to exhibit a crossover from Bose-Einstein condensate (BEC) to Bardeen-Cooper-Schrieffer (BCS) superfluid, when carrier density is tuned to reach the Mott…

Quantum Gases · Physics 2020-02-05 Hui Hu , Xia-Ji Liu

We study the effects of strain on exciton dynamics in transition metal dichalcogenide (TMD) nanoribbons. Using the Bethe-Salpeter formalism, we derive the exciton dispersion relation in strained TMDs and demonstrate that strain-induced…

Mesoscale and Nanoscale Physics · Physics 2026-01-19 Shiva Heidari , Shervin Parsi , Pouyan Ghaemi

The high-quality structures containing semiconducting transition metal dichalcogenides (S-TMDs) monolayer (MLs) required for optical and electrical studies are achieved by their encapsulation in hexagonal BN (hBN) flakes. To examine the…

Mesoscale and Nanoscale Physics · Physics 2023-08-14 A. O. Slobodeniuk , M. R. Molas

Moir\'e superlattices of transition-metal dichalcogenide bilayers host strong Coulomb interactions residing in narrow electron bands, leading to correlated insulating states at fractional carrier doping densities, known as generalized…

Optical properties of transition metal dichalcogenides monolayers are controlled by the Wannier-Mott excitons forming a series of $1s$, $2s$, $2p$,... hydrogen-like states. We develop the theory of the excited excitonic states energy…

Mesoscale and Nanoscale Physics · Physics 2017-02-01 M. M. Glazov , L. E. Golub , G. Wang , X. Marie , T. Amand , B. Urbaszek

Excitons are electron-hole (e-h) pair quasiparticles, which may form a Bose-Einstein condensate (BEC) and collapse into the phase coherent state at low temperature. However, because of ephemeral strength of pairing, a clear evidence for BEC…

Mesoscale and Nanoscale Physics · Physics 2017-11-03 Min-Kyu Joo , Youngjo Jin , Byoung Hee Moon , Hyun Kim , Sanghyub Lee , Young Hee Lee

We demonstrate that, in monolayers (MLs) of semiconducting transition metal dichalcogenides, the $s$-type Rydberg series of excitonic states follows a simple energy ladder: $\epsilon_n=-Ry^*/(n+\delta)^2$, $n$=1,2,\ldots, in which $Ry^*$ is…

Mesoscale and Nanoscale Physics · Physics 2019-09-26 M. R. Molas , A. O. Slobodeniuk , K. Nogajewski , M. Bartos , Ł. Bala , A. Babiński , K. Watanabe , T. Taniguchi , C. Faugeras , M. Potemski

We develop a low energy effective field theory of a mixture of two species of pseudospin-1/2 atoms with interspecies spin-exchange, in addition to density-density interaction. This approach is beyond the single orbital-mode approximation.…

Quantum Gases · Physics 2013-03-01 Li Ge , Yu Shi

We report on the direct mapping of electron transfer in the momentum space of bulk MoS$_2$ by means of time- and angle-resolved two-photon photoemission with a high-harmonic probe. For this purpose, we have combined a high-repetition rate…

Mesoscale and Nanoscale Physics · Physics 2016-10-20 Robert Wallauer , Johannes Reimann , Nico Armbrust , Jens Güdde , Ulrich Höfer