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CaV$_2$O$_4$ is a spin-1 antiferromagnet, where the magnetic vanadium ions are arranged on quasi-one-dimensional (1D) zig-zag chains with potentially frustrated antiferromagnetic exchange interactions. High temperature susceptibility and…

We perform ultrasound velocity measurements on a single crystal of nearly-metallic spinel Co$_{1.21}$V$_{1.79}$O$_4$ which exhibits a ferrimagnetic phase transition at $T_C \sim$ 165 K. The experiments reveal a variety of elastic anomalies…

Strongly Correlated Electrons · Physics 2017-07-26 Tadataka Watanabe , Shogo Yamada , Rui Koborinai , Takuro Katsufuji

Ultrasound velocity measurements of the orbital-degenerate frustrated spinel MgV$_2$O$_4$ are performed in the high-purity single crystal which exhibits successive structural and antiferromagnetic phase transitions, and in the…

Strongly Correlated Electrons · Physics 2014-09-23 Tadataka Watanabe , Takashi Ishikawa , Shigeo Hara , A. T. M. Nazmul Islam , Elisa M. Wheeler , Bella Lake

Simultaneous control of structural and physical properties via applied electrical current poses a key, new research topic and technological significance. Studying the spin-orbit-coupled antiferromagnet Ca2RuO4, with 3% Mn doping to weaken…

Strongly Correlated Electrons · Physics 2019-12-18 Hengdi Zhao , Bing Hu , Feng Ye , Christina Hoffmann , Itamar Kimchi , Gang Cao

The ferrimagnetic spinel $\mathrm{CoV_2O_4}$ has been a topic of intense recent interest, both as a frustrated insulator with unquenched orbital degeneracy and as a near-itinerant magnet which can be driven metallic with moderate applied…

Strongly Correlated Electrons · Physics 2016-02-03 D. Reig-i-Plessis , D. Casavant , V. O. Garlea , A. A. Aczel , M. Feygenson , J. Neuefeind , H. D. Zhou , S. E. Nagler , G. J. MacDougall

We present our theoretical and numerical results on thermodynamic properties and the microscopic mechanism of two successive transitions in vanadium spinel oxides $A$V$_2$O$_4$ ($A$=Zn, Mg, or Cd) obtained by Monte Carlo calculations of an…

Strongly Correlated Electrons · Physics 2007-05-23 Yukitoshi Motome , Hirokazu Tsunetsugu

Ultrasound velocity measurements were performed on a single crystal of spin-frustrated ferrite spinel ZnFe$_2$O$_4$ from 300 K down to 2 K. In this cubic crystal, all the symmetrically-independent elastic moduli exhibit softening with a…

Strongly Correlated Electrons · Physics 2015-11-26 Tadataka Watanabe , Shota Takita , Keisuke Tomiyasu , Kazuya Kamazawa

Motivated by the quasi-1D antiferromagnet CaV$_2$O$_4$, we explore spin-orbital systems in which the spin modes are gapped but orbitals are near a macroscopically degenerate classical transition. Within a simplified model we show that…

Strongly Correlated Electrons · Physics 2015-05-27 Eran Sela , R. G. Pereira

We have theoretically studied successive transitions in vanadium spinel oxides with (t_2g)^2 electron configuration. These compounds show a structural transition at ~ 50K and an antiferromagnetic transition at ~ 40K. Since threefold t_2g…

Strongly Correlated Electrons · Physics 2009-11-11 Yukitoshi Motome , Hirokazu Tsunetsugu

Recently, competing electronic instabilities, including superconductivity and density-wave-like order, have been discovered in vanadium-based kagome metals AV3Sb5 (A = K, Rb, Cs) with a nontrivial band topology. This finding stimulates wide…

We report the successful growth of high-quality single crystals of \ACVO, a quasi-one-dimensional zigzag chain compound containing Co$^{2+}$ ions, using the optical floating zone method. The crystal growth was stabilized under high-pressure…

Strongly Correlated Electrons · Physics 2025-08-15 Anzar Ali , Guratinder Kaur , Arvind Maurya , Isha , Kathrin Küster , Ulrich Starke , Pascal Puphal , Arvind Kumar Yogi , Masahiko Isobe

Our powder inelastic neutron scattering data indicate that \zvo is a system of spin chains that are three dimensionally tangled in the cubic phase above 50 K due to randomly occupied $t_{2g}$ orbitals of V$^{3+}$ ($3d^2$) ions. Below 50 K…

Strongly Correlated Electrons · Physics 2009-11-10 S. -H. Lee , D. Louca , H. Ueda , S. Park , T. J. Sato , M. Isobe , Y. Ueda , S. Rosenkranz , P. Zschack , J. Iniguez , R. Osborn

The compound CaV2O4 contains V^{+3} cations with spin S = 1 and has an orthorhombic structure at room temperature containing zigzag chains of V atoms running along the c-axis. We have grown single crystals of CaV2O4 and report…

We propose a scenario for the two phase transitions in $A$V$_2$O$_4$ ($A$=Zn, Mg, Cd), based on an effective spin-orbital model on the pyrochlore lattice. At high temperatures, spin correlations are strongly frustrated due to the lattice…

Strongly Correlated Electrons · Physics 2007-05-23 Hirokazu Tsunetsugu , Yukitoshi Motome

We use variable-temperature x-ray thermal diffuse scattering and inelastic scattering to investigate the lattice dynamics in single crystals of multiferroic CaMn7O12 which undergo a series of orbital and magnetic transitions at low…

Strongly Correlated Electrons · Physics 2016-11-24 S. M. Souliou , Y. Li , X. Du , M. Le Tacon , A. Bosak

The spin density wave instabilities in the quasi-one-dimensional metal (TMTSF)_2ClO_4 are studied in the framework a matrix random phase approximation for intra-band and inter-band order parameters. Depending on the anion ordering potential…

Strongly Correlated Electrons · Physics 2009-11-07 D. Zanchi , A. Bjelis

We present our theoretical results on the mechanism of two transitions in vanadium spinel oxides $A$V$_2$O$_4$ ($A$=Zn, Mg, or Cd) in which magnetic V cations constitute a geometrically-frustrated pyrochlore structure. We have derived an…

Strongly Correlated Electrons · Physics 2007-05-23 Yukitoshi Motome , Hirokazu Tsunetsugu

We report a thorough study of Y$_{0.7}$La$_{0.3}$VO$_3$ single crystals by measuring magnetic properties, specific heat, thermal conductivity, x-ray and neutron diffraction with the motivation of revealing the lattice response to the…

Strongly Correlated Electrons · Physics 2019-12-04 J. -Q. Yan , W. Tian , H. B. Cao , S. Chi , F. Ye , A. Llobet , Q. Chen , J. Ma , Y. Ren , J. -G. Cheng , J. -S. Zhou , M. A. McGuire , R. J. McQueeney

Spin-state ordering - a periodic pattern of ions with different spin-state configurations along a crystal lattice - is a rare phenomenon, and its possible interrelation with other electronic degrees of freedom remains little explored. Here…

Strongly Correlated Electrons · Physics 2024-03-27 E. Granado , C. W. Galdino , B. D. Moreno , G. King , D. C. Freitas

Motivated by recent interest in quasi-one-dimensional compound CaV2O4, we study the ground states of a spin-orbital chain characterized by an Ising-like orbital Hamiltonian and frustrated interactions between S=1 spins. The on-site…

Strongly Correlated Electrons · Physics 2010-07-13 Gia-Wei Chern , Natalia Perkins
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