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Topological insulators are insulating in the bulk but possess metallic surface states protected by time-reversal symmetry. Here, we report a detailed electronic transport study in high quality Bi2Se3 topological insulator thin films…

Bi$_2$Se$_3$ is a widely studied 3D topological insulator having potential applications in optics, electronics, and spintronics. When the thickness of these films decrease to less than approximately 6 nm, the top and bottom surface states…

Materials Science · Physics 2024-06-19 Saadia Nasir , Walter J. Smith , Thomas E. Beechem , Stephanie Law

Quality of epitaxial films strongly depends on their structural and chemical match with the substrates: the more closely they match, the better the film quality is. Topological insulators (TI) such as Bi2Se3 thin films are of no exception.…

Materials Science · Physics 2020-06-25 Xiong Yao , Jisoo Moon , Sang-Wook Cheong , Seongshik Oh

Hydrogen is a promising energy carrier and key agent for many industrial chemical processes1. One method for generating hydrogen sustainably is via the hydrogen evolution reaction (HER), in which electrochemical reduction of protons is…

Epitaxial growth of topological insulator Bi2Se3 thin films on nominally flat and vicinal Si(111) substrates is studied. In order to achieve planner growth front and better quality epifilms, a two-step growth method is adopted for the van…

Materials Science · Physics 2015-05-18 H. D. Li , Z. Y. Wang , X. Kan , X. Guo , H. T. He , Z. Wang , J. N. Wang , T. L. Wong , N. Wang , M. H. Xie

We demonstrate the capability of growing high quality ultrathin films of the topological insulators Bi2Se3 and Bi2Te3 using molecular beam epitaxy. Unlike previous growth techniques, which often pin the Fermi energy in the conduction band…

Materials Science · Physics 2014-01-15 J. J. Lee , F. T. Schmitt , R. G. Moore , I. M. Vishik , Y. Ma , Z. X. Shen

Topological semimetals with protected surface states mark a new paradigm of research beyond the early landmarks of band-structure engineering, allowing fabrication of efficient catalyst to harness the rich metallic surface states to…

The discovery of topological insulators (TIs), materials with bulk band gaps and protected cross-gap surface states, in compounds such as Bi2Se3 has generated much interest in identifying topological surface states (TSSs) in other classes…

Using first-principles calculations and Boltzmann theory, we explore the feasibility to maximize the thermoelectric figure of merit (ZT) of topological insulator Bi2Te3 films in the few-quintuple layer regime. We discover that the delicate…

Mesoscale and Nanoscale Physics · Physics 2016-06-09 Jinghua Liang , Long Cheng , Jie Zhang , Huijun Liu , Zhenyu Zhang

Magnetic devices are a leading contender for implementing memory and logic technologies that are nonvolatile, that can scale to high density and high speed, and that do not suffer wear-out. However, widespread applications of magnetic…

Mesoscale and Nanoscale Physics · Physics 2015-06-18 A. R. Mellnik , J. S. Lee , A. Richardella , J. L. Grab , P. J. Mintun , M. H. Fischer , A. Vaezi , A. Manchon , E. -A. Kim , N. Samarth , D. C. Ralph

Thermoelectric (TE) devices have been attracting increasing attention because of their ability to convert heat directly to electricity. To date, improving the TE figure of merit remains the key challenge. The advent of the topological…

Mesoscale and Nanoscale Physics · Physics 2016-08-02 T. H. Wang , H. T. Jeng

Exotic and robust metallic surface states of topological insulators (TIs) have been expected to provide a promising platform for novel surface chemistry and catalysis. However, it is still an unprecedented field how TIs affect the activity…

Computational Physics · Physics 2015-09-09 Jianping Xiao , Liangzhi Kou , Chi-Yung Yam , Thomas Frauenheim , Binghai Yan

Two-dimensional transition metal-dichalcogenides are emerging as efficient and cost-effective electrocatalysts for hydrogen evolution reaction (HER). However, only the edge sites of their trigonal prismatic phase show HER-electrocatalytic…

In the last several years, there has been a wealth of studies to clarify the role of thin layers of electrocatalysts on semiconducting photoelectrodes to the efficiency of the oxygen evolution reaction (OER). It has been shown that the…

Ultrathin topological insulator membranes are building blocks of exotic quantum matter. However, traditional epitaxy of these materials does not facilitate stacking in arbitrary orders, while mechanical exfoliation from bulk crystals is…

Mechanical exfoliation of bulk crystals has been widely used to obtain thin topological insulator (TI) flakes for device fabrication. However, such a process produces only micro-sized flakes that are highly irregular in shape and thickness.…

We employed graphene as a patternable template to protect the intrinsic surface states of thin films of topological insulators (TIs) from environment. Here we find that the graphene provides high-quality interface so that the Shubnikov de…

The integration of quantum materials like topological insulators (TIs) with magnetic insulators (MIs) has important technological implications for spintronics and quantum computing. Here we report excellent crystallinity of c-axis oriented…

Materials Science · Physics 2019-02-12 C. C. Chen , K. H. M. Chen , Y. T. Fanchiang , C. C. Tseng , S. R. Yang , C. N. Wu , M. X. Guo , C. K. Cheng , C. T. Wu , M. Hong , J. Kwo

We study the properties of a thin film of topological insulator material. We treat the coupling between helical states at opposite surfaces of the film in the properly-adapted tunneling approximation, and show that the tunneling matrix…

Mesoscale and Nanoscale Physics · Physics 2018-02-21 Mahmoud M. Asmar , Daniel E. Sheehy , Ilya Vekhter

An electrocatalyst is needed to efficiently lower the reaction barriers to produce hydrogen through the H2 evolution reaction (HER). Recently, two-dimensional transition metal dichalcogenides (2D TMDs), such as the pure 2D monolayer MoTe2…

Materials Science · Physics 2024-04-24 Vikash Kumar , Srimanta Pakhira