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Attractive colloidal dispersions, suspensions of fine particles which aggregate and frequently form a space spanning elastic gel are ubiquitous materials in society with a wide range of applications. The colloidal networks in these…

Fluid Dynamics · Physics 2018-11-14 Zsigmond Varga , Jennifer L. Hofmann , James W. Swan

We study the weak solvability of a quasilinear reaction-diffusion system nonlinearly coupled with an linear elliptic system posed in a domain with distributed microscopic balls in $2D$. The size of these balls are governed by an ODE with…

Analysis of PDEs · Mathematics 2023-11-23 Michael Eden , Christos Nikolopoulos , Adrian Muntean

We investigate the behavior of colloidal suspensions with different volume fractions confined between parallel walls under a range of steady shears. We model the particles using molecular dynamics (MD) with full hydrodynamic interactions…

Soft Condensed Matter · Physics 2014-09-18 Frances E. Mackay , Kyle Pastor , Mikko Karttunen , Colin Denniston

By means of classical density functional theory and its dynamical extension, we consider a colloidal fluid with spherically-symmetric competing interactions, which are well known to exhibit a rich bulk phase behavior. This includes complex…

Soft Condensed Matter · Physics 2018-06-11 Daniel Stopper , Roland Roth

The HNC Ornstein-Zernike integral equations are used to determine the properties of simple models of colloidal solutions where the colloids and ions are immersed in a solvent considered as a dielectric continuum and have a size ratio equal…

Soft Condensed Matter · Physics 2009-11-10 Daniel Leger , Dominique Levesque

As a model for a suspension of hard-sphere like colloidal particles where small nonadsorbing dissolved polymers create a depletion attraction, we introduce an effective colloid-colloid potential closely related to the Asakura-Oosawa model…

Soft Condensed Matter · Physics 2015-10-28 Antonia Statt , Peter Virnau , Kurt Binder

We study swelling and structural properties of ionic microgel suspensions within a comprehensive coarse-grained model that combines the polymeric and colloidal natures of microgels as permeable, compressible, charged spheres governed by…

Soft Condensed Matter · Physics 2018-06-07 Tyler J. Weyer , Alan R. Denton

We have measured equilibrium sedimentation profiles in a colloidal model system with confocal microscopy. By tuning the interactions, we have determined the gravitational length in the limit of hard-sphere-like interactions, and using the…

Soft Condensed Matter · Physics 2009-11-10 C. P. Royall , R. van Roij , A. van Blaaderen

We introduce a model gel system in which colloidal forces, structure, and rheology are measured by balancing the requirements of rheological and microscopy techniques with those of optical tweezers. Sterically stabilized poly(methyl…

Soft Condensed Matter · Physics 2015-06-18 Lilian C. Hsiao , Kathryn A. Whitaker , Michael J. Solomon , Eric M. Furst

The drying of colloidal suspensions leads to complex deposition patterns, accompanied by instabilities such as cracking and delamination. In this study, we experimentally investigate the coupled influence of particle surface charge and…

Soft Condensed Matter · Physics 2026-01-27 A. Madhav Sai Kumar , A. Hari Govindha , Ranajit Mondal , Kirti Chandra Sahu

We study suspensions of colloidal spheres with a constant zeta-potential within Poisson-Boltzmann theory, quantifying the discharging of the spheres with increasing colloid density and decreasing salt concentration. We use the calculated…

Soft Condensed Matter · Physics 2013-10-16 Frank Smallenburg , Niels Boon , Maarten Kater , Marjolein Dijkstra , René van Roij

Colloidal gels constitute an important class of materials found in many contexts and with a wide range of applications. Yet as matter far from equilibrium, gels exhibit a variety of time-dependent behaviours, which can be perplexing, such…

Soft Condensed Matter · Physics 2021-09-22 C. Patrick Royall , Malcolm A. Faers , Sian L. Fussell , James E. Hallett

Thermodynamic properties of charge-stabilised colloidal suspensions are commonly modeled by implementing the mean-field Poisson-Boltzmann (PB) theory within a cell model. This approach models a bulk system by a single macroion, together…

Soft Condensed Matter · Physics 2015-05-18 Alan R. Denton

The phase behavior of charge-stabilized colloidal suspensions is modeled by a combination of response theory for electrostatic interparticle interactions and variational theory for free energies. Integrating out degrees of freedom of the…

Soft Condensed Matter · Physics 2009-11-11 Alan R. Denton

We develop a computational method for modeling electrostatic interactions of arbitrarily-shaped, polarizable objects on colloidal length scales, including colloids/nanoparticles, polymers, and surfactants, dispersed in explicit ion…

Soft Condensed Matter · Physics 2024-06-18 Emily Krucker-Velasquez , James W. Swan , Zachary Sherman

In titration experiments with NaOH we have determined the full phase diagram of charged colloidal spheres in dependence on the particle density n, the particle effective charge Zeff and the concentration of screening electrolyte c using…

Partial pair-correlation functions of colloidal suspensions with continuous polydispersity can be challenging to characterize from optical microscopy or computer simulation data due to inadequate sampling. As a result, it is common to adopt…

Soft Condensed Matter · Physics 2011-10-12 Mark J. Pond , Jeffrey R. Errington , Thomas M. Truskett

Several statistical mechanical theories predict that colloidal suspensions of highly charged macroions and monovalent microions can exhibit unusual thermodynamic phase behavior when strongly deionized. Density-functional, extended…

Soft Condensed Matter · Physics 2009-11-11 A. R. Denton

We present a theory of effective electrostatic interactions in polydisperse suspensions of charged macroions, generalizing to mixtures a theory previously developed for monodisperse suspensions. Combining linear response theory with a…

Soft Condensed Matter · Physics 2013-08-20 Jun Kyung Chung , Alan R. Denton

The structure of the Baxter adhesive hard sphere fluid is examined using computer simulation. The radial distribution function (which exhibits unusual discontinuities due to the particle adhesion) and static structure factor are calculated…

Soft Condensed Matter · Physics 2009-11-10 Mark A. Miller , Daan Frenkel
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