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We use dynamic nuclear polarization (DNP) enhanced nuclear magnetic resonance (NMR) at liquid helium temperatures to directly detect hydrogen attached to the surface of silicon microparticles. The proton NMR spectrum from a dry sample of…

Materials Science · Physics 2017-06-08 Mallory L. Guy , Kipp J. van Schooten , Lihuang Zhu , Chandrasekhar Ramanathan

Polarization transfers are crucial building blocks in magnetic resonance experiments, i.e., they can be used to polarize insensitive nuclei and correlate nuclear spins in multidimensional NMR spectroscopy. The polarization can be…

Chemical Physics · Physics 2022-08-24 Zhenfeng Pang , Sheetal Jain , Chen Yang , Xueqian Kong , Kong Ooi Tan

Polarizing nuclear spins is of fundamental importance in biology, chemistry and physics. Methods for hyperpolarizing 13C nuclei from free electrons in bulk, usually demand operation at cryogenic temperatures. Room-temperature approaches…

We present dynamic nuclear polarization (DNP) in the simplest pseudospin quantum Hall ferromagnet (QHF) of an InSb two-dimensional electron gas with a large g factor using tilted magnetic fields. The DNP-induced amplitude change of a…

Mesoscale and Nanoscale Physics · Physics 2015-05-18 H. W. Liu , K. F. Yang , T. D. Mishima , M. B. Santos , Y. Hirayama

Quantum sensors using solid-state spin defects excel in the detection of radiofrequency (RF) fields, serving various purposes in communication, ranging, and sensing. For this purpose, pulsed dynamical decoupling (PDD) protocols are…

Photonic analog to digital conversion offers promise to overcome the signal-to-noise ratio (SNR) and sample rate trade-off in conventional analog to digital converters (ADCs), critical for modern digital communications and signal analysis.…

Signal Processing · Electrical Eng. & Systems 2019-09-09 Callum Deakin , Zhixin Liu

Frequency comb spectroscopy has significantly advanced molecular spectroscopy across scientific research and diverse applications. Among its key performance metrics especially for time-resolved studies, sensitivity and measurement speed are…

CMOS-compatible Kerr microcombs have drawn substantial interest as mass-manufacturable, compact alternatives to bulk frequency combs. This could enable deployment of many comb-reliant applications previously confined to laboratories.…

The increasing demand for multi-wavelength optical sources to support dense wavelength-division multiplexing (DWDM) channels has driven the development of compact and reconfigurable multi-wavelength fiber lasers. Here, we demonstrate a…

Optics · Physics 2026-04-14 Subrata Manna , Amala Jose , K. Nithyanandan

Optically addressable molecular triplet spins provide a chemically tunable platform for quantum application, but their coherence is often limited by interactions with surrounding spin baths. Here we demonstrate controlled suppression of…

We demonstrate dual-comb spectroscopy based on difference frequency generation of frequency-agile near-infrared frequency combs, produced with the help of electro-optic modulators. The combs have a remarkably flat intensity distribution and…

Microwave photonic (MWP) transversal signal processors offer a compelling solution for realizing versatile high-speed information processing by combining the advantages of reconfigurable electrical digital signal processing and…

Signal Processing · Electrical Eng. & Systems 2023-09-15 Yang Sun , Jiayang Wu , Yang Li , Xingyuan Xu , Guanghui Ren , Mengxi Tan , Sai Tak Chu , Brent E. Little , Roberto Morandotti , Arnan Mitchell , David J. Moss

Solid-state NMR spectroscopy is a powerful technique for the characterization of the atomic-level structure and dynamics of materials. Nevertheless, the use of this technique is often limited by its lack of sensitivity, which can prevent…

The ability to optically initialize the electronic spin of the nitrogen-vacancy (NV) center in diamond has long been considered a valuable resource to enhance the polarization of neighboring nuclei, but efficient polarization transfer to…

Mesoscale and Nanoscale Physics · Physics 2018-08-01 F. Shagieva , S. Zaiser , P. Neumann , D. B. R. Dasari , R. Stöhr , A. Denisenko , R. Reuter , C. A. Meriles , J. Wrachtrup

Optical microcombs generated in high-Q microresonators are promising chip-scale light sources for applications ranging from optical communications to spectroscopy and metrology. However, thermo-optic instabilities remain a major obstacle to…

Dynamic nuclear polarization (DNP) is an out-of-equilibrium method for generating non-thermal spin polarization which provides large signal enhancements in modern diagnostic methods based on nuclear magnetic resonance. A particular instance…

Optical frequency combs enable state-of-the-art applications including frequency metrology, optical clocks, astronomical measurements, and sensing. Recent demonstrations of microresonator-based Kerr frequency combs or microcombs pave the…

We consider the dynamic nuclear spin polarization (DNP) using two electrons in a double quantum dot in presence of external magnetic field and spin-orbit interaction, in various schemes of periodically repeated sweeps through the S-T+…

Mesoscale and Nanoscale Physics · Physics 2015-06-17 Izhar Neder , Mark S. Rudner , Bertrand I. Halperin

Mid-infrared microscopy is an important tool for biological analyses, allowing a direct probe of molecular bonds in their low energy landscape. In addition to the label-free extraction of spectroscopic information, the application of…

Dual-comb spectroscopy is a powerful technique for real-time, broadband optical sampling of molecular spectra which requires no moving components. Recent developments with microresonator-based platforms have enabled frequency combs at the…