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The electronic structure of Y$_{4}$Co$_{3}$ has been studied based on the density functional theory within the local-density approximation. The calculation indicates that Y$_{4}$Co$_{3}$ is very close to ferromagnetic instability. The Fermi…

Strongly Correlated Electrons · Physics 2009-11-11 T. Jeong

Here we present the first large scale investigation of electronic properties and correlated magnetism in Ce-based compounds accompanied by a systematic study of the electronic structure and 4f-hybridization function of a large body of Ce…

We investigated CeNi9In2 compound, which has been considered as a mixed valence (MV) system. Electrical resistivity vs. temperature variation was analysed in terms of the model proposed by Freimuth for systems with unstable 4f shell. At low…

Strongly Correlated Electrons · Physics 2015-04-10 R. Kurleto , P. Starowicz , J. Goraus , S. Baran , Yu. Tyvanchuk , Ya. M. Kalychak , A. Szytuła

The three-dimensional electronic structure and the nature of Ce 4f electrons of the Kondo insulator CeRu4Sn6 are investigated by angle-resolved photoemission spectroscopy, utilizing tunable photon energies. Our results reveal (i) the…

The electronic structure of Ce2 is studied in a valence bond model with two 4f electrons localized at two cerium sites. It is shown that the low-lying energy spectrum of the simplest cerium chemical bond is determined by peculiarities of…

Materials Science · Physics 2015-05-28 A. V. Nikolaev

The electronic structures of SmX (X=N, P, As, Sb, Bi, O, S, Se, Te, Po)compounds are calculated using the self-interaction corrected local-spin density approximation. The Sm ion is described with either five or six localized $f$-electrons…

Strongly Correlated Electrons · Physics 2009-11-10 A. Svane , V. Kanchana , G. Vaitheeswaran , G. Santi , W. M. Temmerman , Z. Szotek , P. Strange , L. Petit

We report an extensive study on the intrinsic bulk electronic structure of the high-temperature superconductor CeFeAsO0.89F0.11 and its parent compound CeFeAsO by soft and hard x-ray photoemission, x-ray absorption and soft-x-ray emission…

The electronic structures of supercells of CeO$_{2-\delta}$ have been calculated within the Density Functional Theory (DFT). The equilibrium properties such as lattice constants, bulk moduli and magnetic moments are well reproduced by the…

Materials Science · Physics 2014-04-02 T. Jarlborg , B. Barbiellini , C. Lane , Yung Jui Wang , R. S. Markiewicz , Zhi Liu , Zahid Hussain , A. Bansil

CaFe2As2 exhibits collapsed tetragonal (cT) structure and varied exotic behavior under pressure at low temperatures that led to debate on linking the structural changes to its exceptional electronic properties like superconductivity,…

Superconductivity · Physics 2017-12-12 Khadiza Ali , Kalobaran Maiti

A transformation between the magnetically ordered CeCoGe$_3$ and heavy fermion CeFeGe$_3$ is isostructural but not isoelectronic, therefore the characterization of the electronic structure of the CeCo$_{1-x}$Fe$_x$Ge$_3$ series is of…

Materials Science · Physics 2025-03-25 P. Skokowski , K. Synoradzki , M. Werwiński , A. Bajorek , G. Chełkowska , T. Toliński

The nature of the elemental cerium phases, undergoing an isostructural volume collapse transition, cannot be understood using conventional solid state concepts. Using the combination of density functional theory and dynamical mean-field…

Strongly Correlated Electrons · Physics 2014-03-18 B. Chakrabarti , M. E. Pezzoli , G. Sordi , K. Haule , G. Kotliar

The electronic properties of Cerium (Ce) and ytterbium (Yb) intermetallic compounds may display a more local or more itinerant character depending on the interplay of the exchange interactions among the $4f$ electrons and the Kondo coupling…

Strongly Correlated Electrons · Physics 2021-05-05 Shin-ichi Kimura , Yong Seung Kwon , Cornelius Krellner , Jörg Sichelschmidt

The electronic structure of the $f$-based superconductor $\mathrm{CeIr_3}$ was studied by photoelectron spectroscopy. The energy distribution of the $\mathrm{Ce}~4f$ states were revealed by the $\mathrm{Ce}~3d-4f$ resonant photoelectron…

Hybridization between localized 4$f$ and itinerant 5$d$6$s$ states in heavy fermion compounds is a well-studied phenomenon and commonly captured by the paradigmatic Anderson model. However, the investigation of additional electronic…

We have calculated the electronic structure of Eu for the bcc, hcp, and fcc crystal structures for volumes near equilibrium up to a calculated 90 GPa pressure using the augmented-plane wave method in the local-density approximation. The…

Superconductivity · Physics 2015-05-18 Lane W. Nixon , D. A. Papaconstantopoulos

Cerium (Ce)-based heavy-fermion materials have a characteristic double-peak structure (mid-IR peak) in the optical conductivity [$\sigma(\omega)$] spectra originating from the strong conduction ($c$)--$f$ electron hybridization. To clarify…

Strongly Correlated Electrons · Physics 2016-10-20 Shin-ichi Kimura , Yong Seung Kwon , Yuji Matsumoto , Haruyoshi Aoki , Osamu Sakai

First-principles based on density functional theory is used to study the phase stability, elastic, magnetic, and electronic properties of cubic (c)-Fe$_4$C. Our results show that c-Fe$_{4}$C has a ferromagnetic (FM) ground state structure…

Materials Science · Physics 2014-08-26 Gul Rahman , Haseen Ullah Jan

We systemically investigate the nature of Ce 4f electrons in structurally layered heavy-fermion compounds CcmMnIn3m+2n (with M =Co, Rh, Ir, and Pt, m=l, 2, n=0 - 2), at low temperature using on-resonance angle-resolved photoemission…

The electronic structure of the ferromagnetic material CeRh$_{3}$B$_{2}$ is studied by means of first-principles calculations with an emphasis on the treatment of localized $4f$ states around Ce. Via the construction of an effective spin…

Materials Science · Physics 2019-03-21 Shotaro Doi , Munehisa Matsumoto

The element Ce exhibits an isostructural $\gamma-\alpha$ phase transition with a 15\% volume change at room temperature. The phase boundary ends in a critical point at 1.5 GPa and 480 K. We describe a model for the equation of state of Ce…

Materials Science · Physics 2018-08-01 C. W. Greeff , S. D. Crockett , K. G. Honnell