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The bilayer perovskite La$_3$Ni$_2$O$_7$ has recently been found to enter a superconducting state under hydrostatic pressure at temperatures as high as 80 K. The onset of superconductivity is observed concurrent with a structural transition…

Superconductivity · Physics 2024-04-15 Luke C. Rhodes , Peter Wahl

The interaction of coexisting structural instabilities in multiferroic materials gives rise to intriguing coupling phenomena and extraordinarily rich phase diagrams, both in bulk materials and strained thin films. Here we investigate the…

We report X-ray structural studies of the metal-insulator phase transition in bismuth ferrite, BiFeO3, both as a function of temperature and of pressure (931 oC at atmospheric pressure and ca. 45 GPa at ambient temperature). Based on the…

Materials Science · Physics 2009-02-05 S. A. T. Redfern , J. N. Walsh , S. M. Clark , G. Catalan , J. F. Scott

Bismuthate superconductor Ba(1-x)K(x)BiO3 (x=0.27-0.49, Tc=25-32K) grown by an electrolysis technique was studied by electron diffraction and high-resolution electron microscopy. The crystalline structure thereof has been found to be…

Superconductivity · Physics 2009-11-10 L. A. Klinkova , M. Uchida , Y. Matsui , V. I. Nikolaichik , N. V. Barkovskii

At room temperature, bismuth undergoes several structural transitions with increasing pressure before taking on a body-centered cubic (bcc) phase at approximately 8 GPa. The bcc structure is stable to the highest measured pressure and its…

Materials Science · Physics 2023-06-28 Daniel J. Campbell , Daniel T. Sneed , Earl F. O'Bannon , Per Söderlind , Zsolt Jenei

Under pressure many rare earths and actinide metals transform to a-U structure or its lower symmetry distorted forms. We have reinterpreted the diffraction data of Dabos et al for Pu (reference 4) and find that a Am IV type distorted a-U…

Materials Science · Physics 2009-11-10 S. K. Sikka

Group I/II materials exhibit unexpected structural phase transitions at high pressures, providing potential insight into the origins of elemental superconductivity. We present here a computational study of elemental barium and binary…

Materials Science · Physics 2012-07-16 Joshua A. Taillon , William W. Tipton , Richard G. Hennig

Measurements on resistivity and magnetic susceptibility have been carried out for Bi single crystals under pressures up to 10.5GPa. The temperature dependent resistivity shows a semimetallic behavior at ambient and low pressures (below…

Superconductivity · Physics 2017-01-25 Yufeng Li , Enyu Wang , Xiyu Zhu , Hai-Hu Wen

Several experiments conducted over decades have revealed that the perovskite-structured BaCeO3 goes through a series of temperature-induced structural phase transitions. However, it has been frequently observed that the number of phases and…

In this work, we investigate calcium titanate (CaTiO3 - CTO) using X-ray diffraction and Raman spectroscopy up to 60 and 55 GPa respectively. Both experiments show that the orthorhombic Pnma structure remains stable up to the highest…

Pressure-induced phase transitions of multiferroic BiFeO3 have been investigated using synchrotron radiation X-ray diffraction with diamond anvil cell technique at room temperature. Present experimental data clearly show that rhombohedral…

Materials Science · Physics 2013-08-30 Zhang XiaoLi , Wu Ye , Zhang Qian , Dong JunCai , Wu Xiang , Liu Jing , Wu ZiYu , Chen DongLiang

We present a study of the effect of very high pressure on the orthorhombic perovskite GdMnO3 by Raman spectroscopy and synchrotron x-ray diffraction up to 53.2 GPa. The experimental results yield a structural and insulator-to-metal phase…

Strongly Correlated Electrons · Physics 2011-11-22 J. Agostinho Moreira , A. Almeida , J. Oliveira , V. H. Rodrigues , M. M. R. Costa , P. B. Tavares , P. Bouvier , M. Guennou , J. Kreisel

This work reports on the pressure dependence of the octahedra tilts and mean Fe-O bond lengths in RFeO3 (R=Nd, Sm, Eu, Gd, Tb and Dy), determined through synchrotron X-ray diffraction and Raman scattering, and their role on the pressure…

Ferroelectricity in perovskites is known to be suppressed by a moderate hydrostatic pressure. The notion that a polar instability should reappear in a higher pressure regime is well accepted theoretically but experiments have failed so far…

The crystal structure of the layered, perovskite-related LaTiO_3.41 (La_5Ti_5O_{17+\delta}) has been studied by synchrotron powder x-ray diffraction under hydrostatic pressure up to 27 GPa (T = 295 K). The ambient-pressure phase was found…

Strongly Correlated Electrons · Physics 2007-05-23 I. Loa , K. Syassen , X. Wang , F. Lichtenberg , M. Hanfland , C. A. Kuntscher

High-pressure can transform the structures and compositions of materials either by changing the relative strengths of bonds or by altering the oxidation states of atoms. Both effects cause unconventional compositions in novel compounds that…

Tellurium trioxide, TeO3, is the only example of a trioxide adopting at ambient conditions the VF3-type structure (a distorted variant of the cubic ReO3 structure). Here we present a combined experimental (Raman scattering) and theoretical…

Materials Science · Physics 2021-11-01 Dominik Kurzydłowski , Mikhail A. Kuzovnikov , Marek Tkacz

Thermoelectric (Bi1-x Sbx)2Te3 (BST-x) compounds with x=0.2, 0.7 and 0.9 have been studied using synchrotron angle-dispersive powder x-ray diffraction in a diamond anvil cell up to 25 GPa (at room temperature). The results clearly indicate…

We study the structural evolution of Sr$_3$Ir$_2$O$_7$ as a function of pressure using x-ray diffraction. At a pressure of 54 GPa at room temperature, we observe a first-order structural phase transition, associated with a change from…

We have conducted a detailed high-pressure (HP) investigation on $Eu-$doped $BaTiO_3$ using angle-resolved x-ray diffraction, Raman spectroscopy, dielectric permittivity and dc resistance measurements. The x-ray diffraction data analysis…

Materials Science · Physics 2023-04-04 Mrinmay Sahu , Bishnupada Ghosh , Bobby Joseph , Goutam Dev Mukherjee