Related papers: Dynamical decoupling of interacting dipolar spin e…
We establish a testbed system for the development of high-sensitivity Electron Spin Resonance (ESR) techniques for small samples at cryogenic temperatures. Our system consists of a Niobium Nitride thin-film planar superconducting…
We propose a general protocol for on-demand generation of robust entangled states of nuclear and/or electron spins of ultracold $^1\Sigma$ and $^2\Sigma$ polar molecules using electric dipolar interactions. By encoding a spin-1/2 degree of…
We have studied electron spin resonance (ESR) absorption spectra for the nonmagnetically diluted strong-leg spin ladder magnet ({C}$_{7}$H$_{10}$N)$_{2}$Cu$_{(1-x)}$Zn$_{x}$Br$_{4}$ (abbreviated as DIMPY) down to 450 mK. Formation of the…
We study spin relaxation and diffusion in an electron-spin ensemble of nitrogen impurities in diamond at low temperature (0.25-1.2 K) and polarizing magnetic field (80-300 mT). Measurements exploit mode- and temperature-dependent coupling…
Dynamical polarization of nuclear spin ensembles is of central importance for magnetic resonance studies, precision sensing and for applications in quantum information theory. Here we propose a scheme to generate long-lived singlet pairs in…
There are two distinct techniques of proven effectiveness for extending the coherence lifetime of spin qubits in environments of other spins. One is dynamical decoupling, whereby the qubit is subjected to a carefully timed sequence of…
We present a methodology for probing the details of electronic susceptibility through minimally-invasive nuclear magnetic resonance techniques. Specifically, we classify electron-mediated long-range interactions in an ensemble of nuclear…
We experimentally resolve several weakly coupled nuclear spins in diamond using a series of novelly designed dynamical decoupling controls. Some nuclear spin signals, hidden by decoherence under ordinary dynamical decoupling controls, are…
Understanding the thermalization dynamics of quantum many-body systems at the microscopic level is among the central challenges of modern statistical physics. Here we experimentally investigate individual spin dynamics in a two-dimensional…
In dynamic nuclear polarization (DNP) experiments, the compound is driven out-of-equilibrium by microwave (MW) irradiation of the radical electron spins. Their stationary state has been recently probed via electron double resonance (ELDOR)…
Singlet fission, a process that splits a singlet exciton into a biexciton, has promise in quantum information. We report time-resolved electron paramagnetic resonance measurements on a molecule, TIPS-BP1$'$, designed to exhibit strongly…
Dynamical magnetic and nuclear polarization in complex spin systems is discussed on the example of transfer of spin from exciton to the central spin of magnetic impurity in a quantum dot in the presence of a finite number of nuclear spins.…
We present a quantum solution to the electron spin decoherence by a nuclear pair-correlation method for the electron-nuclear spin dynamics under a strong magnetic field and a temperature high for the nuclear spins but low for the electron.…
Here we report the increase of the coherence time T$_2$ of a single electron spin at room temperature by using dynamical decoupling. We show that the Carr-Purcell-Meiboom-Gill (CPMG) pulse sequence can prolong the T$_2$ of a single…
We simulate the coherence of two coupled electron spins interacting with a bath of nuclei using the generalized cluster correlation expansion (gCCE) method. An exchange interaction between the electrons facilitates a family of entangling…
We present pulsed electrically detected magnetic resonance (EDMR) measurements at low magnetic fields using posphorus-doped silicon with natural isotope composition as a model system. Our measurements show that pulsed EDMR experiments, well…
We present a protocol for designing appropriately extended $\pi$ pulses that achieves tunable, thus selective, electron-nuclear spin interactions with low-driving radiation power. Our method is general since it can be applied to different…
The polarisation dynamics of nuclear spins weakly coupled to an NV center is highly sensitive to the parameters of the microwave control and the nuclear Larmor frequency. What is commonly regarded as a challenge, we propose here as a…
The problem of dipole-dipole decoherence of nuclear spins is considered for strongly entangled spin cluster. Our results show that its dynamics can be described as the decoherence due to interaction with a composite bath consisting of fully…
Molecular spins offer promise in emerging quantum technologies such as quantum sensing and computing. At low temperatures, nuclear spin-spin interactions affect electron spin coherence lifetimes through pure dephasing. Nuclear-spin noise…