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We report polarization of a dense nuclear-spin ensemble in diamond and its dependence on magnetic field and temperature. The polarization method is based on the transfer of electron spin polarization of negatively charged nitrogen vacancy…

Quantum Physics · Physics 2013-04-01 Ran Fischer , Andrey Jarmola , Pauli Kehayias , Dmitry Budker

Dynamic Nuclear Polarization (DNP) has revolutionized the field of solid-state NMR spectroscopy by significantly enhancing the sensitivity of nuclear magnetic resonance experiments. Conventionally, cross effect DNP relies on biradicals to…

Chemical Physics · Physics 2023-09-28 Amaria Javed , Asif Equbal

We demonstrate time reversal of nuclear spin dynamics in highly magnetized dilute liquid 3He-4He mixtures through effective inversion of long-range dipolar interactions. These experiments, which involve using magic sandwich NMR pulse…

Other Condensed Matter · Physics 2007-10-10 Michael E. Hayden , Emmanuel Baudin , Geneviève Tastevin , Pierre-Jean Nacher

We report optically detected nuclear magnetic resonance (ODNMR) measurements on small ensembles of nuclear spins in single GaAs quantum dots. Using ODNMR we make direct measurements of the inhomogeneous Knight field from a photo-excited…

Mesoscale and Nanoscale Physics · Physics 2015-05-18 M. N. Makhonin , E. A. Chekhovich , P. Senellart , A. Lemaitre , M. S. Skolnick , A. I. Tartakovskii

Single electron spins coupled to multiple nuclear spins provide promising multi-qubit registers for quantum sensing and quantum networks. The obtainable level of control is determined by how well the electron spin can be selectively coupled…

Isolated nuclear spins offer a promising building block for quantum information processing systems, but their weak interactions often impede preparation, control, and detection. Hyperfine coupling to a proximal electronic spin can enhance…

Quantum Physics · Physics 2013-05-29 Benjamin Smeltzer , Jean McIntyre , Lilian Childress

Methods for achieving quantum control and detection of individual nuclear spins by single electrons of solid-state defects play a central role for quantum information processing and nano-scale nuclear magnetic resonance (NMR). However, with…

Quantum Physics · Physics 2017-03-06 Zhen-Yu Wang , Jorge Casanova , Martin B. Plenio

Nuclear spins in semiconductors are leading candidates for quantum technologies, including quantum computation, communication, and sensing. Nuclear spins in diamond are particularly attractive due to their extremely long coherence lifetime.…

Recently, there have been significant developments to detect nuclear spins with an nitrogen vacancy (NV) center in diamond. However, due to the nature of the short range dipole-dipole interaction, it takes a long time to detect distant…

Quantum Physics · Physics 2021-08-11 Hideaki Hakoshima , Yuichiro Matsuzaki , Toyofumi Ishikawa

Spin-labeling of molecules with paramagnetic ions is an important approach for determining molecular structure, however current ensemble techniques lack the sensitivity to detect few isolated spins. In this Letter, we demonstrate…

Mesoscale and Nanoscale Physics · Physics 2014-12-03 Matthew Pelliccione , Bryan A. Myers , Laetitia Pascal , Ananda Das , Ania C. Bleszynski Jayich

We experimentally resolve several weakly coupled nuclear spins in diamond using a series of novelly designed dynamical decoupling controls. Some nuclear spin signals, hidden by decoherence under ordinary dynamical decoupling controls, are…

Here we propose and analyse in detail protocols that can achieve rapid hyperpolarization of 13C nuclear spins in randomly oriented ensembles of nanodiamonds at room temperature. Our protocols exploit a combination of optical polarization of…

Quantum Physics · Physics 2015-11-25 Q. Chen , I. Schwarz , F. Jelezko , A. Retzker , M. B. Plenio

We observe nuclear magnetic resonance (NMR) in the fractional quantum Hall regime at Landau level filling factor $\nu=2/3$ from simultaneous measurement of longitudinal resistance and photoluminescence (PL). The dynamic nuclear spin…

Mesoscale and Nanoscale Physics · Physics 2016-08-11 K. Akiba , K. Nagase , Y. Hirayama

Nuclear spin ensembles in diamond are promising candidates for quantum sensing applications, including rotation sensing. Here we perform a characterization of the optically detected nuclear-spin transitions associated with the 14N nuclear…

Pulsed Dynamic Nuclear Polarization (DNP) is currently receiving substantial interest as a means to enhance the sensitivity of nuclear magnetic resonance (NMR) and magnetic resonance imaging (MRI) by orders of magnitude. It has also…

One of the most remarkable properties of the nitrogen-vacancy (NV) center in diamond is that optical illumination initializes its electronic spin almost completely, a feature that can be exploited to polarize other spin species in their…

The Cosmic Axion Spin Precession Experiment (CASPEr) seeks to measure oscillating torques on nuclear spins caused by axion or axion-like-particle (ALP) dark matter via nuclear magnetic resonance (NMR) techniques. A sample spin-polarized…

Nuclear spins with hyperfine coupling to single electron spins are highly valuable quantum bits. In this work we probe and characterise the particularly rich nuclear spin environment around single silicon vacancy color-centers (V2) in…

We show that atomic alignment presents a reliable way to study topology of astrophysical magnetic fields. The effect of atomic alignment arises from modulation of the relative population of the sublevels of atomic ground state pumped by…

Astrophysics · Physics 2008-11-26 Huirong Yan , A. Lazarian

A magnetometer using spin-polarized K and $^3$He atoms occupying the same volume is used to search for anomalous nuclear spin-dependent forces generated by a separate $^3$He spin source. We measure changes in the $^3$He spin precession…

Atomic Physics · Physics 2010-01-11 G. Vasilakis , J. M. Brown , T. W. Kornack , M. V. Romalis