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We investigate a two-level atom in the field of a strong laser pulse. The resulting time-dependent polarization is the source of a radiation the frequency components of which are essentially harmonics of the driving field's carrier…

Quantum Physics · Physics 2016-09-13 Ákos Gombkötő , Attila Czirják , Sándor Varró , Péter Földi

Optical second-harmonic generation is demonstrated to be a sensitive probe of the buried interface between the lattice matched semiconductors gallium phosphide and silicon with (001) orientation. Rotational anisotropy measurements of SHG…

Mesoscale and Nanoscale Physics · Physics 2020-10-29 K. Brixius , A. Beyer , J. Güdde , M. Dürr , W. Stolz , K. Volz , U. Höfer

Second and third harmonic generation in the opaque region of a GaAs wafer is experimentally observed both in transmission and reflection. These harmonic components can propagate through an opaque material as long as the pump is tuned to a…

Optics · Physics 2019-05-13 L. Rodriguez , J. Trull , M. Scalora , R. Vilaseca , C. Cojocaru

We derive an expression for the effective second-harmonic coefficient of a dilute suspension of coated spherical particles. It is assumed that the coating material, but not the core or the host, has a nonlinear susceptibility for…

Disordered Systems and Neural Networks · Physics 2009-11-10 P. M. Hui , C. Xu , D. Stroud

Second harmonic generation (SHG) extensively employs periodically poled nonlinear crystals through forward quasi-phase-matching to achieve efficient frequency conversion. As poling periods approach sub-micrometers, backward…

Optics · Physics 2024-07-15 Fengyan Yang , Juanjuan Lu , Mohan Shen , Guangcanlan Yang , Hong X. Tang

Efficient nonlinear wave mixing is of paramount importance for a wide range of applications. However, weak optical nonlinearities pose significant challenges for accessing nonlinear light-matter interaction in compact systems. Here, we…

Strong light-matter coupling gives rise to polaritons -- quasiparticles that combine both photonic and material characteristics. Here, we show that polar nanocrystals exhibit structure- and environment-dependent Raman scattering, enabled by…

We present a new theoretical approach to the study of second and third harmonic generation from metallic nanostructures and nanocavities filled with a nonlinear material, in the ultrashort pulse regime. We model the metal as a two-component…

Localized electromagnetic modes and negligible Ohmic losses dictate the growing interest in subwavelength all-dielectric nanoparticles. Although an exhaustive volume of study dealt with interaction of all-dielectric nanostructures with…

The nonlinear forcing terms for the wave equation in general curvilinear coordinates are derived based on a hyperelastic material. The expressions for the nonlinear part of the first Piola-Kirchhoff stress are specialized for axisymmetric…

Classical Physics · Physics 2012-09-20 Yang Liu , Ehsan Khajeh , Cliff J. Lissenden , Joseph L. Rose

Simultaneous Kerr comb formation and second-harmonic generation with on-chip microresonators can greatly facilitate comb self-referencing for optical clocks and frequency metrology. Moreover, the presence of both second- and third-order…

There is an active demand to develop efficient nanoscale nonlinear sources for applications in photonic circuitry, quantum optics and biosensing. To this end, plasmonic systems have been utilized to boost the nonlinear signal generation,…

Optics · Physics 2019-06-26 Feng Wang , Manoj Manjare , Robert Lemasters , Chentao Li , Hayk Harutyunyan

Second-harmonic generation (SHG) is a quintessential probe of inversion symmetry breaking in condensed matter. While perturbative $\chi^{(2)}$ processes are well-documented, the nonperturbative regime under intense driving remains largely…

Strongly Correlated Electrons · Physics 2026-04-08 Keisuke Kitayama , Masao Ogata

Hyperbolic plasmonic metamaterials provide numerous opportunities for designing unusual linear and nonlinear optical properties. We show that the modal overlap of fundamental and second-harmonic light in an anisotropic plasmonic…

We show that second harmonic generation can be enhanced by Fano resonant coupling of asymmetric plasmonic metal nanostructures. We develop a theoretical model examining the effects of electromagnetic interaction between two metal…

Parametric oscillation is a fundamental concept that underlies nonlinear wave-matter interactions, leading to generation or amplification of new frequency components. Using a temporal modulation generated by the heterodyne interference of a…

Optics · Physics 2020-01-10 Xuexue Guo , Xingjie Ni

We investigate high-harmonic generation in graphene heterostructures consisting of metallic nanoribbons separated from a graphene sheet by either a few-nanometer layer of aluminum oxide or an atomic monolayer of hexagonal boron nitride. The…

We use ultrafast laser pulses to experimentally demonstrate that the second-order optical response of bulk single crystals of the topological insulator Bi$_2$Se$_3$ is sensitive to its surface electrons. By performing surface doping…

Materials Science · Physics 2011-02-02 D. Hsieh , J. W. McIver , D. H. Torchinsky , D. R. Gardner , Y. S. Lee , N. Gedik

Chip-scale nonlinear optics enables strong light-matter interactions within compact devices, serving as a fundamental platform for multifunctional integrated photonics from classical optical signal processing to quantum information…

We study theoretically optical response of WS2 monolayer located near periodic metal nanostructured arrays in two and three dimensions. The emphasis of simulations is on the strong coupling regime of excitons supported by WS2 and surface…

Mesoscale and Nanoscale Physics · Physics 2018-04-04 Maxim Sukharev , Ruth Pachter