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Related papers: An Expanded Gas-Grain Model for Interstellar Glyci…

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A new chemical model is presented that simulates fully-coupled gas-phase, grain-surface and bulk-ice chemistry in hot cores. Glycine (NH2CH2COOH), the simplest amino acid, and related molecules such as glycinal, propionic acid and propanal,…

Astrophysics of Galaxies · Physics 2015-06-12 Robin T. Garrod

We present an extended version of the 2-phase gas-grain code NAUTILUS to the 3-phase modelling of gas and grain chemistry of cold cores. In this model, both the mantle and the surface are considered as chemically active. We also take into…

Astrophysics of Galaxies · Physics 2016-04-19 Maxime Ruaud , Valentine Wakelam , Franck Hersant

Aminoacetonitrile (AAN), also known as glycinenitrile, has been suggested as a possible precursor of glycine and adenine in the interstellar medium. Here we present the chemical modeling of AAN and its isomers in hot cores using the…

Astrophysics of Galaxies · Physics 2024-08-22 Xia Zhang , Donghui Quan , Xiaohu Li , Jarken Esimbek , Fangfang Li , Yan Zhou , Dalei Li

Gas-phase processes were long thought to be the key formation mechanisms for complex organic molecules in star-forming regions. However, recent experimental and theoretical evidence has cast doubt on the efficiency of such processes.…

Astrophysics · Physics 2009-11-13 Robin T. Garrod , Susanna L. Widicus Weaver , Eric Herbst

Ice is ubiquitous in the interstellar medium. We model the formation of the main constituents of interstellar ices, including H2O, CO2 , CO, and CH3 OH. We strive to understand what physical or chemical parameters influence the final…

Astrophysics of Galaxies · Physics 2023-07-26 A. Clément , A. Taillard , V. Wakelam , P. Gratier , J. -C. Loison , E. Dartois , F. Dulieu , J. A. Noble , M. Chabot

Icy interstellar dust grains are a source of complex organic molecule (COM) production, although their formation mechanisms are debated. Laboratory experiments show that atomic C deposited onto interstellar ice analogs can react with…

Astrophysics of Galaxies · Physics 2025-10-27 Sydney A. Willis , Serge A. Krasnokutski , Nathaniel J. Morin , Robin T. Garrod

The detection of the amino acid glycine and its amine precursor methylamine on the comet 67P/Churyumov-Gerasimenko by the Rosetta mission provides strong evidence for a cosmic origin of prebiotics on Earth. How and when such complex organic…

Instrumentation and Methods for Astrophysics · Physics 2020-11-17 S. Ioppolo , G. Fedoseev , K. -J. Chuang , H. M. Cuppen , A. R. Clements , M. Jin , R. T. Garrod , D. Qasim , V. Kofman , E. F. van Dishoeck , H. Linnartz

Shocks are a crucial probe for understanding the ongoing chemistry within ices on interstellar dust grains where many complex organic molecules (COMs) are believed to be formed. However, previous work has been limited to the initial…

The first hydrostatic core (FHSC) phase is a brief stage in the protostellar evolution that is difficult to detect. Our goal is to characterize the chemical evolution of gas and dust during the formation of the FHSC. Moreover, we are…

Protoplanetary disks are the target of many chemical studies (both observational and theoretical) as they contain the building material for planets. Their large vertical and radial gradients in density and temperature make them challenging…

Astrophysics of Galaxies · Physics 2016-10-07 V. Wakelam , M. Ruaud , F. Hersant , A. Dutrey , D. Semenov , L. Majumdar , S. Guilloteau

A new, more comprehensive model of gas-grain chemistry in hot molecular cores is presented, in which nondiffusive reaction processes on dust-grain surfaces and in ice mantles are implemented alongside traditional diffusive surface/bulk-ice…

Astrophysics of Galaxies · Physics 2022-02-23 Robin T. Garrod , Mihwa Jin , Kayla A. Matis , Dylan Jones , Eric R. Willis , Eric Herbst

Syn-glycolamide, a glycine isomer, has recently been detected in the G+0.693-0.027 molecular cloud. Investigations on its formation in the interstellar medium could offer insights into synthetic routes leading to glycine in prebiotic…

Astrophysics of Galaxies · Physics 2025-04-25 Jessica Perrero , Silvia Alessandrini , Hexu Ye , Cristina Puzzarini , Albert Rimola

In the interstellar medium (ISM), the formation of complex organic molecules (COMs) is largely facilitated by surface reactions. However, in cold dark clouds, thermal desorption of COMs is inefficient because of the lack of thermal energy…

Astrophysics of Galaxies · Physics 2022-09-07 Alec Paulive , Joshua T. Carder , Eric Herbst

Our automated reaction discovery program, AutoMeKin, has been utilized to investigate the formation of glycolonitrile (HOCH$_{2}$CN) in the gas phase under the low temperatures of the interstellar medium (ISM). The feasibility of a proposed…

Grain surface chemistry is key to the composition of protoplanetary disks around young stars. The temperature of grains depends on their size. We evaluate the impact of this temperature dependence on the disk chemistry. We model a…

Astrophysics of Galaxies · Physics 2021-10-13 S. Gavino , A. Dutrey , V. Wakelam , S. Guilloteau , J. Kobus , S. Wolf , W. Iqbal , E. Di Folco , E. Chapillon , V. Piétu

The observational detection of some metastable isomers in the interstellar medium with abundances comparable to those of the most stable isomer, or even when the stable isomer is not detected, highlights the importance of non-equilibrium…

Amino acids are the essential keys that contribute to the study of the formation of life. The simplest amino acid, glycine (NH$_{2}$CH$_{2}$COOH), has been searched for a long time in the interstellar medium, but all surveys of glycine have…

Astrophysics of Galaxies · Physics 2022-09-05 Arijit Manna , Sabyasachi Pal

Molecular oxygen has been the subject of many observational searches as chemical models predicted it to be a reservoir of oxygen. Although it has been detected in two regions of the interstellar medium, its rarity is a challenge for…

Astrophysics of Galaxies · Physics 2019-06-04 V. Wakelam , M. Ruaud , P. Gratier , I. A. Bonnell

The observed gas-phase molecular inventory of hot cores is believed to be significantly impacted by the products of chemistry in interstellar ices. In this study, we report the construction of a full macroscopic Monte Carlo model of both…

Astrophysics of Galaxies · Physics 2015-06-12 A. I. Vasyunin , E. Herbst

AIM: We have recently developed a microscopic Monte Carlo approach to study surface chemistry on interstellar grains and the morphology of ice mantles. The method is designed to eliminate the problems inherent in the rate-equation formalism…

Astrophysics · Physics 2009-11-13 Q. Chang , H. M. Cuppen , E. Herbst
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