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Quantum magnets based on honeycomb lattices with low-coordination number offer a viable ground to realize exotic emergent quantum excitations and phenomena arising from the interplay between competing magnetic interactions, spin…

Strongly Correlated Electrons · Physics 2024-11-14 J. Khatua , M. Gomilsek , Kwang-Yong Choi , P. Khuntia

Honeycomb iridates are thought to have strongly spin-anisotropic exchange interactions that could lead to an extraordinary state of matter known as the Kitaev quantum spin liquid. The realization of this state requires almost perfectly…

Recently, there have been contrary claims of Kitaev spin-liquid behaviour and ordered behavior in the honeycomb compound Ag$_3$LiIr$_2$O$_6$ based on various experimental signatures. Our investigations on this system reveal a…

In quantum magnetism spin dimers are typically associated with spin-singlet states. To date, $triplet$ $dimerization$ has not been observed in any 3D or quasi-2D material. With this in mind we here discuss the electronic structure of the…

The origin of the spin liquid state in Tb$_2$Ti$_2$O$_7$ has challenged experimentalists and theorists alike for nearly 20 years. To improve our understanding of the exotic magnetism in Tb$_2$Ti$_2$O$_7$, we have synthesized a chemical…

We explore the potential experimental realization of the mixed-spin Kitaev model in materials such as Zr$_{0.5}$Ru$_{0.5}$Cl$_3$, where spin-1/2 and spin-3/2 ions occupy distinct sublattices of a honeycomb lattice. By developing a…

Strongly Correlated Electrons · Physics 2025-05-09 Willian Natori , Yang Yang , Hui-Ke Jin , Johannes Knolle , Natalia B. Perkins

In the quest to find quantum spin liquids, layered cobalt oxides Na2Co2TeO6 and Na3Co2SbO6 have been proposed as promising candidates for approximating the Kitaev honeycomb model. Yet, their suitability has been thrown into question due to…

Strongly Correlated Electrons · Physics 2024-04-25 Ping Miao , Xianghong Jin , Weiliang Yao , Yue Chen , Akihiro Koda , Zhenhong Tan , Wu Xie , Wenhai Ji , Takashi Kamiyama , Yuan Li

Frustration in magnetic interactions can give rise to disordered ground states with subtle and beautiful properties. The spin ices Ho2Ti2O7 and Dy2Ti2O7 exemplify this phenomenon, displaying a classical spin liquid state, with…

Strongly Correlated Electrons · Physics 2017-12-11 Mathieu Taillefumier , Owen Benton , Han Yan , L. D. C. Jaubert , Nic Shannon

The nature of magnetic correlation at low temperature in two-dimensional artificial magnetic honeycomb lattice is a strongly debated issue. While theoretical researches suggest that the system will develop a novel zero entropy spin solid…

Mesoscale and Nanoscale Physics · Physics 2018-02-20 A. Glavic , B. Summers , A. Dahal , R. J. Kline , W. Van Herck , A. Sukhov , A. Ernst , D. K. Singh

The 5d-electron honeycomb compound H$_3$LiIr$_2$O$_3$ [K. Kitagawa $et$ $al.$, Nature 554, 341-345 (2018)] exhibits an apparent quantum spin liquid (QSL) state. In this intercalated spin-orbital compound, a remarkable pile up of low-energy…

Strongly Correlated Electrons · Physics 2019-02-07 Johannes Knolle , Roderich Moessner , Natalia B. Perkins

The three-dimensional frustrated spin lattice in MgCrGaO4, where Cr3+ ions occupy a pyrochlore-like network, exemplifies a quantum magnet with competing interactions, macroscopic degeneracy, and exotic low-energy excitations. Using…

Strongly Correlated Electrons · Physics 2026-03-17 U. Jena , S. Kundu , Suheon Lee , Q. Faure , F. Damay , S. Rols , Adam Berlie , S. Petit , Kwang-Yong Choi , P. Khuntia

The search for Kitaev's quantum spin liquid (KQSL) state in real materials has recently expanded with the prediction that honeycomb lattices of divalent, high-spin cobalt ions could host the dominant bond-dependent exchange interactions…

Quantum spin liquid involves fractionalized quasipariticles such as spinons and visons. They are expressed as itinerant Majorana fermions and $Z_2$ fluxes in the Kitaev model with bond-dependent exchange interactions on a honeycomb spin…

Strongly Correlated Electrons · Physics 2020-02-05 Y. Nagai , T. Jinno , Y. Yoshitake , J. Nasu , Y. Motome , M. Itoh , Y. Shimizu

Quantum spin liquids are materials that feature quantum entangled spin correlations and avoid magnetic long-range order at T = 0 K. Particularly interesting are two-dimensional honeycomb spin lattices where a plethora of exotic quantum spin…

Strongly Correlated Electrons · Physics 2020-11-20 C. Wessler , B. Roessli , K. W. Krämer , B. Delley , O. Waldmann , L. Keller , D. Cheptiakov , H. B. Braun , M. Kenzelmann

The family of edge-sharing tri-coordinated iridates and ruthenates has emerged in recent years as a major platform for Kitaev spin liquid physics, where spins fractionalize into emergent magnetic fluxes and Majorana fermions with Dirac-like…

The possible emergence of a spin liquid phase in the half-filled Hubbard model on the honeycomb lattice; a simple model of graphene, is studied using the variational cluster approximation. We found that the critical interaction strength of…

Strongly Correlated Electrons · Physics 2017-02-24 Atsushi Yamada

The complexity of the antiferromagnetic orders observed in the honeycomb iridates is a double-edged sword in the search for a quantum spin-liquid ground state: both attesting that the magnetic interactions provide many of the necessary…

Strongly Correlated Electrons · Physics 2019-02-22 K. A. Modic , B. J. Ramshaw , Nicholas P. Breznay , James G. Analytis , Ross D. McDonald , Arkady Shekhter

Two-dimensional high-spin bipartite honeycomb networks, where anisotropy, competing exchange interactions, and spin fluctuations interplay, provide an alternative platform to test theoretical models that distinguish between classical and…

Strongly Correlated Electrons · Physics 2026-05-05 M. Barik , Q. Faure , F. Damay , J. P. Embs , S. Petit , P. Khuntia

Quantum spin liquids have been at the forefront of correlated electron research ever since their original proposal in 1973, and the realization that they belong to the broader class of intrinsic topological orders, along with the fractional…

Strongly Correlated Electrons · Physics 2018-04-26 Ioannis Rousochatzakis , Yuriy Sizyuk , Natalia B. Perkins

We have studied the spin liquid Tb$\_2$Sn$\_2$O$\_7$ by neutron diffraction and specific heat measurements. Below about 2 K, the magnetic correlations change from antiferromagnetic to ferromagnetic. Magnetic order settles in two steps, with…

Strongly Correlated Electrons · Physics 2009-11-11 I. Mirebeau , A. Apeteri , J. Rodriguez-Carvajal , P. Bonville , A. Forget , D. Colson , V. Glazkov , J. P. Sanchez , O. Isnard , E. Suard