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In vibrational strong coupling (VSC), molecular vibrations strongly interact with the modes of an optical cavity to form hybrid light-matter states known as vibrational polaritons. Experiments show that the kinetics of thermally activated…

Quantum Physics · Physics 2021-05-04 Matthew Du , Jorge A. Campos-Gonzalez-Angulo , Joel Yuen-Zhou

A cloud of cold N two-level atoms driven by a resonant laser beam shows cooperative effects both in the scattered radiation field and in the radiation pressure force acting on the cloud center-of-mass. The induced dipoles synchronize and…

Atomic Physics · Physics 2013-02-05 Tom Bienaime , Romain Bachelard , Nicola Piovella , Robin Kaiser

We investigate the properties of two interacting ultracold polar molecules described as distinguishable quantum rigid rotors, trapped in a one-dimensional harmonic potential. The molecules interact via a multichannel two-body contact…

Atomic Physics · Physics 2018-07-03 Anna Dawid , Maciej Lewenstein , Michał Tomza

Controlling matter-light interactions with cavities is of fundamental importance in modern science and technology. It is exemplified in the strong-coupling regime, where matter-light hybrid modes form, with properties controllable via the…

Mesoscale and Nanoscale Physics · Physics 2021-11-03 Long Zhang , Fengcheng Wu , Shaocong Hou , Zhe Zhang , Yu-Hsun Chou , Kenji Watanabe , Takashi Taniguchi , Stephen R. Forrest , Hui Deng

In 1937 the Jahn-Teller (JT) effect addressed the instability (potential or actual) of non-linear symmetric molecules with degenerate orbital electronic states. In view of the large variety of JT activity that has taken place since then, we…

Other Condensed Matter · Physics 2007-05-23 R. Englman , A. Yahalom

The photochemistry of a molecular ensemble coupled to a resonance cavity and triggered by a femtosecond laser pulse is investigated from a real-time, quantum dynamics perspective with the multi-configuration time-dependent Hartree method.…

Chemical Physics · Physics 2018-06-20 Oriol Vendrell

We experimentally demonstrate optical dipole trapping of a cloud of cold atoms by means of a dynamically coupled mode of a high-finesse cavity. We show that the trap requires a collective action of the atoms, i.e. a single atom would not be…

Quantum Physics · Physics 2021-09-01 A. Dombi , T. W. Clark , F. I. B. Williams , F. Jessen , J. Fortágh , D. Nagy , A. Vukics , P. Domokos

We show that time-resolved x-ray scattering from molecules prepared in a superposition of electronic states moving through an avoided crossing has new features not found in diffraction from the corresponding classical mixed state.…

We study a system of interacting matter quasiparticles strongly coupled to photons inside an optomechanical cavity. The resulting normal modes of the system are represented by hybrid polaritonic quasiparticles, which acquire effective…

Quantum Gases · Physics 2017-02-27 N. Bobrovska , M. Matuszewski , T. C. H. Liew , O. Kyriienko

In this article, we show that the collective light-matter strong coupling regime, where $N$ molecular emitters couple to the photon mode of an optical cavity, can be mapped to a quantum impurity model where the photon is the impurity that…

Quantum Physics · Physics 2023-10-25 Joel Yuen-Zhou , Arghadip Koner

We theoretically investigate the light scattering of the super- and subradiant states which can be prepared by the excitation of a single photon which carries an orbital angular momentum (OAM).\ With this helical phase imprinted on the…

Quantum Physics · Physics 2019-03-06 H. H. Jen , M. -S. Chang , Y. -C. Chen

Recent experiments of chemical reactions in optical cavities have shown great promise to alter and steer chemical reactions but still remain poorly understood theoretically. In particular the origin of resonant effects between the cavity…

Chemical Physics · Physics 2022-12-21 Derek S. Wang , Johannes Flick , Susanne F. Yelin

The interaction between super-intense coherent x-ray light and nuclei is studied theoretically. One of the main difficulties with driving nuclear transitions arises from the very narrow nuclear excited state widths which limit the coupling…

Quantum Physics · Physics 2012-10-03 André Junker , Adriana Pálffy , Christoph H. Keitel

We present a theoretical study of a possibility of superconductivity in a three dimensional molecular conductor in which the interaction between electrons in doubly degenerate molecular orbitals and an {\em intra}molecular vibration mode is…

Superconductivity · Physics 2016-08-31 R. Ramakumar , Sudhakar Yarlagadda

The properties of a system of charged particles on a 2D lattice, subject to an anisotropic Jahn-Teller-type interaction and 3D Coulomb repulsion are investigated. In the mean-field approximation without Coulomb interaction, the system…

Strongly Correlated Electrons · Physics 2008-11-19 T. Mertelj , V. V. Kabanov , D. Mihailovic

Resonant dipole-dipole interaction modifies the energy and decay rate of electronic excitations for finite one dimensional chains of ultracold atoms in an optical lattice. We show that collective excited states of the atomic chain can be…

Quantum Physics · Physics 2012-12-07 Hashem Zoubi , Helmut Ritsch

Interactions between atoms and light in optical cavities provide a means of investigating collective (many-body) quantum physics in controlled environments. Such ensembles of atoms in cavities have been proposed for studying collective…

When molecular transitions strongly couple to photon modes, they form hybrid light-matter modes called polaritons. Collective vibrational strong coupling is a promising avenue for control of chemistry, but this can be deterred by the large…

A light-matter hybrid quasiparticle, called a polariton, is formed when molecules are strongly coupled to an optical cavity. Recent experiments have shown that polariton chemistry can manipulate chemical reactions. Polariton chemistry is a…

Chemical Physics · Physics 2024-01-11 Xinyang Li , Nicholas Lubbers , Sergei Tretiak , Kipton Barros , Yu Zhang

Molecular polaritons, hybrid light-matter states resulting from strong cavity coupling of optical transitions, may provide a new route to guide chemical reactions. However, demonstrations of cavity-modified reactivity in clean benchmark…

Chemical Physics · Physics 2024-08-20 Liying Chen , Ashley P. Fidler , Alexander M. McKillop , Marissa L. Weichman