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We demonstrate that a conditional wavefunction theory enables a unified and efficient treatment of the equilibrium structure and nonadiabatic dynamics of correlated electron-ion systems. The conditional decomposition of the many-body…

Chemical Physics · Physics 2021-07-22 Guillermo Albareda , Kevin Lively , Shunsuke A. Sato , Aaron Kelly , Angel Rubio

We transform the Schr\"odinger wave equation to a nine-parameter Heun-type differential equation. Using our solutions of the latter in [J. Math. Phys. 59 (2018) 113507], we are able to identify the associated potential function, energy…

Quantum Physics · Physics 2020-12-25 A. D. Alhaidari

For a given many-electron molecule, it is possible to define a corresponding one-electron Schr\"odinger equation, using potentials derived from simple atomic densities, whose solution predicts fairly accurate molecular orbitals for single-…

Chemical Physics · Physics 2022-05-16 Fariba Nazari , Jerry L. Whitten

We develop a variational method for interacting surface systems with higher-form global symmetries. As a natural extension of the conventional second-quantized Hamiltonian of interacting bosons, we explicitly construct a second-quantized…

Statistical Mechanics · Physics 2026-02-10 Kiyoharu Kawana

A simple analytic expression of the three-body wave function describing the system $(\alpha\alpha n)$ in the ground state $\frac{3}{2}^-$ of ${}^9\mathrm{Be}$ is obtained. In doing this, it is assumed that the $\alpha$ particles interact…

Nuclear Theory · Physics 2024-08-06 S. A. Rakityansky

In this study, we present analytical solutions of the Schr\"odinger equation with the Multiparameter potential containing the different types of physical potential via the asymptotic iteration method (AIM) by applying a Pekeris-type…

Quantum Physics · Physics 2017-02-02 Ahmet Taş , Ali Havare

We have developed the technique of a quantum wave impedance determination for the sequence of not only constant potentials but also for potentials of forms for which the solution of a Shr\"{o}dinger equation exists at least in terms of…

Quantum Physics · Physics 2020-10-20 O. I. Hryhorchak

Traditional multiconfiguration Hartree-Fock (MCHF) and configuration interaction (CI) methods are based on a single orthonormal orbital basis (OB). For atoms with complicated shell structures, a large OB is needed to saturate all the…

Atomic Physics · Physics 2015-06-12 S. Verdebout , P. Rynkun , P. Jönsson , G. Gaigalas , C. Froese Fischer , M. Godefroid

The Schr\"{o}dinger equation is solved exactly for some well known potentials. Solutions are obtained reducing the Schr\"{o}dinger equation into a second order differential equation by using an appropriate coordinate transformation. The…

Quantum Physics · Physics 2019-12-06 Cevdet Tezcan , Ramazan Sever

This paper presents the first implementation of a coupling between advanced wave function theories and molecular density functional theory (MDFT). This method enables the modeling of solvent effect into quantum mechanical (QM) calculations…

Chemical Physics · Physics 2024-04-12 Maxime Labat , Emmanuel Giner , Guillaume Jeanmairet

A new approximation scheme to the centrifugal term is proposed to obtain the $l\neq 0$ bound-state solutions of the Schr\"{o}dinger equation for an exponential-type potential in the framework of the hypergeometric method. The corresponding…

Quantum Physics · Physics 2015-05-13 Sameer M. Ikhdair , Ramazan Sever

We derive analytic expressions of the recursive solutions to the Schr\"{o}dinger's equation by means of a cutoff potential technique for one-dimensional piecewise constant potentials. These solutions provide a method for accurately…

Quantum Physics · Physics 2015-06-26 Hwasung Lee , Y. J. Lee

A version of the configuration interaction (CI) method is developed which treats highly excited many-electron basis states perturbatively, so that their inclusion does not affect the size of the CI matrix. This removes, at least in…

Atomic Physics · Physics 2017-01-25 V. A. Dzuba , J. Berengut , C. Harabati , V. V. Flambaum

We introduce an energy functional for ground-state electronic structure calculations. Its variables are the natural spin-orbitals of singlet many-body wave functions and their joint occupation probabilities deriving from controlled…

Chemical Physics · Physics 2016-12-04 Ralph Gebauer , Morrel H. Cohen , Roberto Car

The multi-configuration Dirac-Hartree-Fock method was employed to calculate the total and excitation energies, oscillator strengths and hyperfine structure constants for low-lying levels of Sm I. In the first-order perturbation…

Atomic Physics · Physics 2015-09-16 Fuyang Zhou , Yizhi Qu , Jiguang Li , Jianguo Wang

In recent years, an increasing attention has been paid to quantum heterostructures with tailored functionalities, such as heterojunctions and quantum matematerials, in which quantum dynamics of electrons can be described by the…

Numerical Analysis · Mathematics 2024-12-20 Jingrun Chen , Dingjiong Ma , Zhiwen Zhang

Over time, many different theories and approaches have been developed to tackle the many-body problem in quantum chemistry, condensed-matter physics, and nuclear physics. Here we use the helium atom, a real system rather than a model, and…

Atomic Physics · Physics 2019-04-03 Jing Li , N. D. Drummond , Peter Schuck , Valerio Olevano

We introduce the time-dependent restricted active space Configuration Interaction method to solve the time-dependent Schr\"odinger equation for many-electron atoms, and particularly apply it to the treatment of photoionization processes in…

Atomic Physics · Physics 2013-05-30 David Hochstuhl , Michael Bonitz

We present the concept, derivation, and implementation of dynamical configuration interaction, a quantum embedding theory that combines Green's function methodology with the many-body wave function. In a strongly-correlated active space, we…

Chemical Physics · Physics 2019-04-03 Marc Dvorak , Patrick Rinke

The general formulation of a technically advantageous method to find the ground state solution of the Schrodinger equation in configuration space for systems with a number of particles A greater than 4 is presented. The wave function is…

Nuclear Theory · Physics 2009-10-31 Nir Barnea , Winfried Leidemann , Giuseppina Orlandini