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Long-lived oscillations in 2D spectra of chlorophylls are at the heart of an ongoing debate. Their physical origin is either a multi-pigment effect, such as excitonic coherence, or primarily stems from localized vibrations. In the present…

Chemical Physics · Physics 2017-08-31 Václav Perlík , Craig Lincoln , František Šanda , Jürgen Hauer

The study of phonon coupling in doped semiconductors via electrical transport measurements is challenging due to unwanted temperature-induced effects such as dopant ionisation and parallel conduction. Here, we study phonon scattering in 2D…

Mesoscale and Nanoscale Physics · Physics 2025-03-03 Y. Ashlea Alava , K. Kumar , C. Harsas , P. Mehta , P. Hathi , C. Chen , D. A. Ritchie , A. R. Hamilton

Theoretical and numerical calculations of the optical absorption spectra of excitons interacting with longitudinal-optical phonons in quasi-2D polar semiconductors are presented. In II-VI semiconductor quantum wells, exciton binding energy…

Mesoscale and Nanoscale Physics · Physics 2009-11-07 F. J. Rodriguez

The temperature-dependent linewidths of excitons in ZnO quantum wells were studied by measuring absorption spectra from 5 K to room temperature. We deduced experimentally the exciton-longitudinal-optical (LO) phonon coupling strength, which…

Materials Science · Physics 2015-06-25 T. Makino , Y. Segawa , M. Kawasaki

When an electron-hole pair is optically excited in a semiconductor quantum dot the host crystal lattice needs to adapt to the presence of the generated charge distribution. Therefore the coupled exciton-phonon system has to establish a new…

The picosecond dynamics of excitons in colloidal CdSe nanorods are directly measured via their 1s to 2p-like internal transitions by ultra-broadband terahertz spectroscopy. Broadened absorption peaks from both the longitudinal and…

Mesoscale and Nanoscale Physics · Physics 2015-06-17 David G. Cooke , Peter Uhd Jepsen , Jun Yan Lek , Yeng Ming Lam , Fredrik Sy , Marc M. Dignam

Laser control of solids was so far mainly discussed in the context of strong classical nonlinear light-matter coupling in a pump-probe framework. Here we propose a quantum-electrodynamical setting to address the coupling of a…

Superconductivity · Physics 2018-07-02 Michael A. Sentef , Michael Ruggenthaler , Angel Rubio

We study theoretically the radiative recombination of excitons in double quantum dots in the presence of carrier-phonon coupling. We show that the phonon-induced pure dephasing effects and transitions between the exciton states strongly…

Mesoscale and Nanoscale Physics · Physics 2012-01-20 Pawel Karwat , Anna Sitek , Pawel Machnikowski

We systematically study the coupling of longitudinal modes (shells) in a carbon nanotube quantum dot. Inelastic cotunneling spectroscopy is used to probe the excitation spectrum in parallel, perpendicular and rotating magnetic fields. The…

Mesoscale and Nanoscale Physics · Physics 2019-01-23 M. C. Hels , T. S. Jespersen , J. Nygård , K. Grove-Rasmussen

Micro-photoluminescence spectroscopy at variable temperature, excitation intensity and energy was performed on a single InAs/AlAs self-assembled quantum dot. The exciton emission line (zero-phonon line, ZPL) exhibits a broad sideband due to…

Materials Science · Physics 2009-11-13 D. Sarkar , H. P. van der Meulen , J. M. Calleja , J. M. Meyer , R. J. Haug , K. Pierz

We propose a three-pulse coherent ultrafast optical technique that is particularly sensitive to two-exciton correlations. Two Liouville-space pathways for the density matrix contribute to this signal which reveals double quantum coherences…

Mesoscale and Nanoscale Physics · Physics 2009-11-13 Lijun Yang , Shaul Mukamel

Luminescence properties of colloidal quantum dots have found applications in imaging, light-sources, and displays. Despite wide interest, several experimental observations from these quantum dots, such as the short lifetime on the scale of…

Mesoscale and Nanoscale Physics · Physics 2018-06-05 Meenakshi Khosla , Sravya Rao , Shilpi Gupta

We study the transport properties of two double quantum dots in a parallel arrangement at temperatures of a few Kelvin. Thereby, we show that decoherence entailed by the substrate phonons affects the shot noise. For asymmetric coupling…

Mesoscale and Nanoscale Physics · Physics 2008-01-10 Rafael Sánchez , Sigmund Kohler , Peter Hänggi , Gloria Platero

The coupling between a two-level system and its environment leads to decoherence. Within the context of coherent manipulation of electronic or quasiparticle states in nanostructures, it is crucial to understand the sources of decoherence.…

Mesoscale and Nanoscale Physics · Physics 2015-05-27 P. Roulleau , S. Baer , T. Choi , F. Molitor , J. Güttinger , T. Müller , S. Dröscher , K. Ensslin , T. Ihn

Electric dipole radiation can be controlled by coherent optical feedback, as has previously been studied by modulating the photonic environment for point dipoles placed both in optical cavities and near metal mirrors. In experiments…

Mesoscale and Nanoscale Physics · Physics 2020-02-05 Christopher Rogers , Dodd Gray , Nathan Bogdanowicz , Takashi Taniguchi , Kenji Watanabe , Hideo Mabuchi

Resonance Raman scattering, a very effective and sensitive technique for atomically thin semiconducting transition metal dichalcogenide, can be used to observe the phonons from the entire Brillouin zone. In addition to the significance of…

Materials Science · Physics 2023-02-06 Deepu Kumar , Nasaru Khan , Rahul Kumar , Mahesh Kumar , Pradeep Kumar

Addressing the role of quantum coherence in the interplay between the different matter constituents (electrons, phonons and spin) is a critical step towards understanding transition metal oxides and design complex materials with new…

Coupling between electrons and phonons (lattice vibrations) drives the formation of the electron pairs responsible for conventional superconductivity. The lack of direct evidence for electron-phonon coupling in the electron dynamics of the…

Tailoring the properties of correlated oxides is accomplished by chemical doping, pressure, temperature or magnetic field. Photoexcitation is a valid alternative to reach out-of-equilibrium states otherwise inaccessible. Here, we…

Strong electron-electron interactions are known to significantly modify the electron-phonon coupling relative to the predictions of density functional theory, but this effect is challenging to calculate with realistic theories of strongly…

Strongly Correlated Electrons · Physics 2025-07-21 David J. Abramovitch , Jennifer Coulter , Sophie Beck , Andrew Millis