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Aerosol particles play an important role in the climate system by absorbing and scattering radiation and influencing cloud properties. They are also one of the biggest sources of uncertainty for climate modeling. Many climate models do not…
Calibration of the uncertain Arrhenius diffusion parameters for quantifying mixing rates in Zr-Al nanolaminate foils was performed in a Bayesian setting [Vohra et al., 2014]. The parameters were inferred in a low temperature regime…
In this paper we formulate and analyze an elementary model for the propagation of advancing autoignition fronts in reactive co-flow fuel/oxidizer jets injected into an aqueous environment at high pressure. This work is motivated by the…
We present a density-functional theory based molecular-dynamics study of the structural, dynamical, and electronic properties of liquid methanol under ambient conditions. The calculated radial distribution functions involving the oxygen and…
Because of growing interest in temperature-based sampling methods like replica exchange, this note aims to make some observations and raise some potentially important questions which we have not seen addressed sufficiently in the…
A radio frequency um-jet plasma source is studied using He/O2 mixture. This um-jet can be used for different applications as a source of chemical active species e.g. oxygen atoms, molecular metastables and ozone. Using absolutely-calibrated…
Molecular modelling and simulation of the surface tension of fluids with force fields is discussed. 29 real fluids are studied, including nitrogen, oxygen, carbon dioxide, carbon monoxide, fluorine, chlorine, bromine, iodine, ethane,…
The electron and gas temperature of non-equilibrium argon plasma torch sustained by a focused 24 GHz microwave beam in the external atmosphere of air was measured by optical emission spectroscopy. The excitation temperature of argon atoms…
For a detailed understanding of chemical processes in nature and industry, we need accurate models of chemical reactions in complex environments. While Eyring transition state theory is commonly used for modeling chemical reactions, it is…
We investigated a nonlinear advection-diffusion-reaction equation for a passive scalar field. The purpose is to understand how the compressibility can affect the front dynamics and the bulk burning rate. We study two classes of flows:…
Accurate absorption models for gases at high pressure and temperature support advanced optical combustion diagnostics and aid in the study of harsh planetary atmospheres. Developing and validating absorption models for these applications…
The capabilities of a plug-flow fixed-bed cell for operando studies of heterogeneous catalysts are demonstrated using laboratory-based X-ray absorption spectroscopy (XAS) with a von Hamos spectrometer. The cell operates at temperatures up…
Nuclear magnetic resonance (NMR) experiments are described for two granular-flow systems, the vibrofluidized bed and the gas-fluidized bed. Using pulsed field gradient, magnetic resonance imaging, and hyperpolarized gas NMR, detailed…
We review long-baseline neutrino experiments in which neutrinos are detected after traversing macroscopic distances. Over such distances neutrinos have been found to oscillate among flavor states. Experiments with solar, atmospheric,…
Ultra-lean premixed hydrogen combustion is a possible solution to decarbonize industry, while limiting flame temperatures and thus nitrous oxide emissions. These lean hydrogen/air flames experience strong preferential diffusion effects,…
The new method for aerosol measurement using wide-field stellar photometry was originally developed for B-filter data. The dependence of VAOD (vertical aerosol optical depth) on wavelength can be used to understand the physical…
Moderate or intense low-oxygen dilution (MILD) combustion is achieved by strongly diluting and preheating the reactants through mixing with hot combustion products before ignition. To better understand how fuel/air/product mixing and…
The precise location of the liquid-vapor critical point in aluminum has remained elusive for decades, with reported critical temperatures spanning nearly 4000 K. Here we resolve this long-standing uncertainty by combining deep potential…
Key aerosol properties that shape climate -- such as CCN activity, scattering and absorption, and ice nucleation efficiency -- are difficult to infer from measurements that typically capture only a part of the aerosol state. We develop a…
Upcoming facilities such as the Herschel Space Observatory or ALMA will deliver a wealth of molecular line observations of young stellar objects (YSOs). Based on line fluxes, chemical abundances can then be estimated by radiative transfer…