English
Related papers

Related papers: Towards Time-Resolved Atomic Structure Determinati…

200 papers

X-ray standing wave (XSW) excited photoelectron emission was used to measure the site-specific valence band (VB) for 1/2 monolayer (ML) Pt grown on a SrTiO3 (001) surface. The XSW induced modulations in the core level (CL) and VB…

We present here a powerful method providing simultaneous atomic spatial and nanosecond temporal resolution for investigating dynamics and structure on the atomic scale, in general. We reveal the dynamic reorganization of surface (ad)atoms…

Mesoscale and Nanoscale Physics · Physics 2016-08-18 Giulia Serrano , Stefano Tebi , Stefan Wiespointner-Baumgarthuber , Stefan Müllegger , Reinhold Koch

Periodical multilayer (ML) structures can be used as generators of X-ray standing waves (XSW) for investigation of objects and processes on solid/liquid and solid/gas interfaces. In this paper, we investigate the specific requirements to…

Materials Science · Physics 2018-03-22 Olga Dikaya , Dmitri Novikov , Alexander Goikhman , Ksenia Maksimova

The development of high-brightness free-electron lasers (FEL) has revolutionised our ability to create and study matter in the high-energy-density (HED) regime. Current diagnostic techniques have been very successful in yielding information…

A natural approach to measure the time of arrival of an atom at a spatial region is to illuminate this region with a laser and detect the first fluorescence photons produced by the excitation of the atom and subsequent decay. We investigate…

Quantum Physics · Physics 2009-11-10 J. A. Damborenea , I. L. Egusquiza , G. C. Hegerfeldt , J. G. Muga

Upon absorbing a photon, the ionized electron sails through the target force field in attoseconds to reach free space. This navigation probes details of the potential landscape that get imprinted into the phase of the ionization amplitude.…

Atomic Physics · Physics 2024-12-12 Sajad Azizi , Mohamed El-Amine Madjet , Zheng Li , Jan M. Rost , Himadri S. Chakraborty

Nanostructures of Titanium oxide (TiO2) are being studied for many promising applications, e.g., solar photovoltaics, solar water splitting for H2 fuel generation etc., due to their excellent photo-catalytic properties. We have synthesized…

Materials Science · Physics 2016-09-30 Gangadhar Das , Manoj Kumar , A. K. Biswas , Ajay Khooha , Puspen Mondal , M. K. Tiwari

A major remaining challenge in the superconducting cuprates is the unambiguous differentiation of the composition and electronic structure of the CuO$_2$ layers and those of the intermediate layers. The large c axis for these materials…

By analyzing ``exact'' theoretical results from solving the time-dependent Schr\"odinger equation of atoms in few-cycle laser pulses, we established the general conclusion that differential elastic scattering and photo-recombination cross…

Atomic Physics · Physics 2008-04-04 Toru Morishita , Anh-Thu Le , Zhangjin Chen , C. D. Lin

Knowledge of the molecular structure is key to understanding the function of participating molecules in photo-induced chemical reactions. Visualizing the nuclear dynamics of a photochemical reaction requires an ultrafast measurement…

Chemical Physics · Physics 2021-12-21 Kasra Amini

Time-resolved X-ray scattering patterns from photoexcited molecules in solution are in many cases anisotropic at the ultrafast time scales accessible at X-ray Free Electron Lasers (XFELs). This anisotropy arises from the interaction of a…

Wavelength stability of free-electron lasers (FELs) is one of the important parameters for various applications. In this paper we describe two different methods to diagnose the wavelength stability of a mid-infrared (MIR) FEL. The first one…

Resonant inelastic x-ray scattering (RIXS) is a widely used spectroscopic technique, providing access to the electronic structure and dynamics of atoms, molecules, and solids. However, RIXS requires a narrow bandwidth x-ray probe to achieve…

We demonstrate X-ray phase contrast microscopy performed at the European X-ray Free-Electron Laser sampled at 1.128 MHz rate. We have applied this method to image stochastic processes induced by an optical laser incident on water-filled…

The low repetition rates and possible shot-to-shot variations in laser-plasma studies place a high value on single-shot diagnostics. For example, white-beam scattering methods based on broadband backlighter x-ray sources are used to…

Plasma Physics · Physics 2014-03-04 O. R. Hoidn , G. T. Seidler

The current state of the art in structural biology is led by NMR, X-ray crystallography and TEM investigations. These powerful tools however all rely on averaging over a large ensemble of molecules. Here, we present an alternative concept…

Atomic and Molecular Clusters · Physics 2015-12-15 Tatiana Latychevskaia , Jean-Nicolas Longchamp , Conrad Escher , Hans-Werner Fink

Superconducting microcircuits and metamaterials are promising candidates for use in new generation cryogenic electronics. Their functionality is largely justified by the macroscopic distribution of electromagnetic fields in arranged unit…

Superconductivity · Physics 2022-02-16 A. A. Leha , A. P. Zhuravel , A. Karpov , A. V. Lukashenko , A. V. Ustinov

Precision measurement of small separations between two atoms or molecules has been of interest since the early days of science. Here, we discuss a scheme which yields spatial information on a system of two identical atoms placed in a…

Quantum Physics · Physics 2007-05-23 Jun-Tao Chang , Joerg Evers , Marlan O. Scully , M. Suhail Zubairy

The development of X-ray free-electron lasers (XFELs) has enabled ultrafast X-ray diffraction (XRD) experiments, which are capable of resolving electronic/vibrational transitions and structural changes in molecules, or capturing molecular…

Chemical Physics · Physics 2024-08-29 Sebastian V. Pios , Jiaji Zhang , Maxim F. Gelin , Hong-Guang Duan , Lipeng Chen

Understanding elementary mechanisms behind solid-state phase transformations and reactions is the key to optimizing desired functional properties of many technologically relevant materials. Recent advances in scanning transmission electron…