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We study resonance contrast by a two-step pulse observation method to enhance the frequency stability of coherent population trapping (CPT) atomic clocks. The proposed method is a two-step Raman--Ramsey scheme with low intensity during…

Atomic Physics · Physics 2017-03-08 Yuichiro Yano , Shigeyoshi Goka , Masatoshi Kajita

From the interaction between a frequency comb and an atomic qubit, we derive quantum protocols for the determination of the carrier-envelope offset phase, using the qubit coherence as a reference, and without the need of frequency doubling…

Quantum Physics · Physics 2014-03-05 Andrea Cadarso , Jordi Mur-Petit , Juan José García-Ripoll

Increasing coherent interrogation times is central to advancing the precision of optical clocks. Synchronous differential optical clock comparisons have now demonstrated atomic coherence times that far exceed the coherence time of the clock…

We have developed a universal method to form the reference signal for the stabilization of arbitrary atomic clocks based on Ramsey spectroscopy. Our approach uses an interrogation scheme of the atomic system with two different Ramsey…

A train of periodic optical pulses gives an optical frequency "comb" that acts as a precise ruler for light measurement due to its equally spaced frequencies. Today, such pulses last millionths of a billionth of a second (Femtoseconds/fs)…

Optics · Physics 2026-05-22 Tushar Malica

We derive composite pulse sequences that achieve high-fidelity excitation of two-state systems in an optically dense, inhomogeneously broadened ensemble. The composite pulses are resistant to distortions due to the back-action of the medium…

Quantum Physics · Physics 2016-02-24 Gabor Demeter

We describe a possible new technique for precise wavelength calibration of high-resolution astronomical spectrographs using femtosecond-pulsed mode-locked lasers controlled by stable oscillators such as atomic clocks. Such `frequency combs'…

The stability of an optical atomic clock is a critical figure of merit for almost all clock applications. To this end, much optical atomic clock research has focused on reducing clock instability by increasing the atom number, lengthening…

Atomic Physics · Physics 2023-12-21 Xin Zheng , Jonathan Dolde , Shimon Kolkowitz

Achieving high-frequency spectral resolution with quantum sensors, while crucial in fields ranging from physical to biological sciences, is challenging due to their finite coherence time. Here, we introduce a novel protocol that achieves…

Quantum Physics · Physics 2025-04-17 Jungbae Yoon , Keyuan Zhong , Guoqing Wang , Boning Li , Donghun Lee , Paola Cappellaro

We present a novel approach to achieve hyper spectral resolution, high sensitive detection, and high speed data acquisition Stimulated Raman Spectroscopy by employing amplified offset-phase controlled fs-pulse bursts. In this approach, the…

Qubit noise spectroscopy is an important tool for the experimental investigation of open quantum systems. However, conventional techniques for noise spectroscopy are time-consuming, because they require measurements of the noise spectral…

Quantum Physics · Physics 2025-06-24 Kaixin Huang , Demitry Farfurnik , Alireza Seif , Mohammad Hafezi , Yi-Kai Liu

Scattering of ultraintense short laser pulses off relativistic electrons allows one to generate a large number of X- or $\gamma$-ray photons with the expense of the spectral width---temporal pulsing of the laser inevitable leads to…

Plasma Physics · Physics 2019-05-29 Daniel Seipt , Vasily Yu. Kharin , Sergey G. Rykovanov

Interference between multiple distinct paths is a defining property of quantum physics, where "paths" may involve actual physical trajectories, as in interferometry, or transitions between different internal (e.g. spin) states, or both. A…

We propose a set of experiments in which Ramsey-fringe techniques are tailored to probe transitions originating and terminating on the same ground state level. When pulses of resonant radiation, separated by a time delay $% T, $ interact…

Atomic Physics · Physics 2007-05-23 Tycho Sleator , Paul R. Berman , Boris Dubetsky

Ramsey interferometry is a cornerstone technique for precise measurement of time and frequency in modern clocks. The Ramsey experiments are typically done in optically dilute samples of atoms to improve homogeneity and avoid back-action of…

Quantum Physics · Physics 2025-05-20 S. A. Moiseev , K. I. Gerasimov , M. M. Minnegaliev , I. V. Brekotkin , E. S. Moiseev

Ultrafast lasers ($< 500$ fs) have enabled laser-matter interactions at intensities exceeding $10^{18} \rm{Wcm}^{-2}$ with only millijoules of laser energy. However, as pulse durations become shorter, larger spectral bandwidths are…

Nonlinear spectroscopy employs a series of laser pulses to interrogate dynamics in large interacting many-body systems, and has become a highly successful method for experiments in chemical physics. Current quantum optical experiments…

Quantum Physics · Physics 2016-10-19 Frank Schlawin , Manuel Gessner , Shaul Mukamel , Andreas Buchleitner

Femtosecond dual-comb lasers have revolutionized linear Fourier-domain spectroscopy by offering a rapid motion-free, precise and accurate measurement mode with easy registration of the combs beat note in the RF domain. Extensions of this…

Random pulse sequences are a powerful method for qubit noise spectroscopy, enabling efficient reconstruction of sparse noise spectra. Here, we advance this method in two complementary directions. First, we extend the method using a…

Quantum Physics · Physics 2026-01-07 Kaixin Huang , Demitry Farfurnik , Dror Baron , Yi-Kai Liu

Laser treatment has emerged into a cornerstone of industrial manufacturing. This creates the demand to understand in detail the involved physical processes and their dynamics, to control the process, and to keep guard in-situ the laser…

Optics · Physics 2025-12-16 Jörn Bonse