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Two-dimensional (2D) materials with remarkable second-harmonic generation (SHG) hold promise for future on-chip nonlinear optics. Relevant materials with both giant SHG response and environmental stability are long-sought targets. Here, we…

Light-matter interactions in crystals are powerful tools that seamlessly allow both functionalities of sizeable bandgap modulation and non-invasive spectroscopy. While we often assume that the border between the two regimes of modulation…

Raman spectroscopy and Second Harmonic Generation (SHG) are complementary, non-destructive techniques that provide rich and distinct insights into the structural and electronic properties of materials. Raman spectroscopy offers detailed…

Optics · Physics 2026-04-30 Volodymyr Multian , Luigi Bonacina , Jérémie Teyssier

Quadratic optical parametric processes form the foundation for a variety of applications related to classical and quantum frequency conversion, which have attracted significant interest recently in on-chip implementation. These processes…

Optics · Physics 2018-09-19 Rui Luo , Yang He , Hanxiao Liang , Mingxiao Li , Qiang Lin

We report a strong nonlinear optical response of 2D MoSe$_2$ nanoflakes (NFs) through spatial self-phase modulation (SSPM) and cross-phase modulation (XPM) induced by nonlocal coherent light-matter interactions. The coherent interaction of…

We study experimentally parametric amplification in the continuous regime using a transverse-degenerate type-II Optical Parametric Oscillator operated below threshold. We demonstrate that this device is able to amplify either in the phase…

Quantum Physics · Physics 2009-11-11 S. Gigan , L. Lopez , V. Delaubert , N. Treps , C. Fabre , A. Maitre

The second-order nonlinear optical susceptibility $\Pi^{(2)}$ for second harmonic generation is calculated for gapped graphene. The linear and second-order nonlinear plasmon excitations are investigated in context of second harmonic…

Mesoscale and Nanoscale Physics · Physics 2015-06-17 Godfrey Gumbs , Yonatan Abranyos , Upali Aparajita , Oleksiy Roslyak

Spatial self-phase modulation (SSPM) is the optical nonlinear process and is a result of spatially varying refractive index profile along the line of propagation in a medium. SSPM is proved to be a method to demonstrate different photonic…

By combining analytical and numerical approaches, we study resonantly enhanced second-harmonic generation (SHG) by individual high-index dielectric nanoparticles made of centrosymmetric materials. Considering both bulk and surface…

Optics · Physics 2018-01-08 Daria Smirnova , Alexander I. Smirnov , Yuri S. Kivshar

A compact and broadband polarimetric imaging platform is presented, based on second-harmonic generation (SHG) in nonlinear flat-optics. The system employs periodic all-dielectric AlGaAs gratings to induce polarization-dependent SH emission,…

Nonlinear optical processes in whispering gallery mode (WGM) microresonators have attracted much attention. Owing to the strong confinement of light in a small volume, a WGM microresonator can dramatically boost the strength of light field,…

Optics · Physics 2015-12-29 Jintian Lin , Yingxin Xu , Jielei Ni , Min Wang , Zhiwei Fang , Lingling Qiao , Wei Fang , Ya Cheng

We demonstrate and explore an all-optical technique for direct monitoring the orientation dynamics of gas phase molecular ensembles. The technique termed 'MOISH' utilizes the transiently lifted inversion symmetry of polar gas media and…

Chemical Physics · Physics 2022-10-12 Amit Beer , Ran Damari , Yun Chen , Sharly Fleischer

Advanced photonic materials showing two-photon absorption (2PA) have been widely explored to develop three-dimensional imaging, micro and nanofabrication, all-optical switching, lithography on a nanoscale and many other enabling…

High complexity, dense integrated nanophotonic circuits possessing strong nonlinearities are desirable for a breadth of applications in classical and quantum optics. In this work, we study natural phase matching via modal engineering in…

Optics · Physics 2018-05-30 Jia-Yang Chen. Yong Meng Sua , Heng Fan , Yu-ping Huang

Rhombohedrally stacked transition metal dichalcogenides such as 3R-MoS$_2$ offer an exceptional platform for nonlinear optics, naturally forming Fabry-P\'erot (FP) microcavities due to their giant dielectric contrast with the surrounding…

Plasmonic metasurfaces have emerged as a promising platform for enhancing a range of nonlinear optical processes, offering compact geometry and flexibility in light manipulation. Second order nonlinear processes, like second harmonic…

Nonlinear optical frequency conversion, where optical fields interact with a nonlinear medium to generate new frequencies, is a key phenomenon in modern photonic systems. However, a major challenge with these techniques lies in the…

Materials Science · Physics 2024-12-05 Simone Grillo , Elena Cannuccia , Maurizia Palummo , Olivia Pulci , Claudio Attaccalite

Metasurfaces, composed of subwavelength scattering elements, have demonstrated remarkable control over the transmitted amplitude, phase, and polarization of light. However, manipulating the amplitude upon transmission has required loss if a…

Current advances in nonlinear optics have made it possible to perform a homodyne-like tomography of an unknown state without highly efficient detectors or a strong local oscillator. Thereby, a new experimental direction has been opened into…

Quantum Physics · Physics 2023-10-31 Éva Rácz , László Ruppert , Radim Filip

We have investigated second harmonic generation (SHG) from Ag-coated LiNbO3 (LN) core-shell nanocuboids and found that giant SHG can occur via deliberately designed double plasmonic resonances. By controlling the aspect ratio, we can tune…

Optics · Physics 2014-11-19 Ming-Liang Ren , Si-Yuan Liu , Ben-Li Wang , Bao-Qin Chen , Jiafang Li , Zhi-Yuan Li