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Related papers: Hydrogen transfer reactions of interstellar Comple…

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Recent high-resolution and sensitivity ALMA observations have unveiled the carbon isotope ratios ($^{12}$C/$^{13}$C) of Complex Organic Molecules (COMs) in a low-mass protostellar source. To understand the $^{12}$C/$^{13}$C ratios of COMs,…

Solar and Stellar Astrophysics · Physics 2024-06-27 Ryota Ichimura , Hideko Nomura , Kenji Furuya

Oxygen atom addition and insertion reactions may provide a pathway to chemical complexity in ices that are too cold for radicals to diffuse and react. We have studied the ice-phase reactions of photo-produced oxygen atoms with C2…

Earth and Planetary Astrophysics · Physics 2019-04-03 Jennifer B. Bergner , Karin I. Oberg , Mahesh Rajappan

The reactions of carbon atoms with dihydrogen have been investigated in liquid helium droplets at $T$ = 0.37 K. A calorimetric technique was applied to monitor the energy released in the reaction. The barrierless reaction between a single…

Astrophysics of Galaxies · Physics 2016-03-01 S. A. Krasnokutski , M. Kuhn , M. Renzler , C. Jäger , Th. Henning , P. Scheier

This review paper summarizes the state-of-the-art in laboratory based interstellar ice chemistry. The focus is on atom addition reactions, illustrating how water, carbon dioxide and methanol can form in the solid state at astronomically…

Astrophysics of Galaxies · Physics 2015-07-13 Harold Linnartz , Sergio Ioppolo , Gleb Fedoseev

Intermolecular hydrogen transfer free radical reactions are common in the combustion process and in a number of organic chemistry reactions. Therefore, evaluating the pressure and temperature-dependent rate constants of them is of great…

Chemical Physics · Physics 2024-04-01 Yi Sun

Simple and complex organic molecules (COMs) are observed along different phases of star and planet formation and have been successfully identified in prestellar environments such as dark and translucent clouds. Yet the picture of organic…

Interstellar complex organic molecules (iCOMs) can be loosely defined as chemical compounds with at least six atoms in which at least one is carbon. The observations of iCOMs in star-forming regions have shown that they contain an important…

Solar and Stellar Astrophysics · Physics 2019-09-30 Joan Enrique-Romero , Albert Rimola , Cecilia Ceccarelli , Piero Ugliengo , Nadia Balucani , Dimitrios Skouteris

Observational studies reveal that complex organic molecules (COMs) can be found in various objects associated with different star formation stages. The identification of COMs in prestellar cores, i.e., cold environments in which thermally…

Solar and Stellar Astrophysics · Physics 2017-06-28 Gleb Fedoseev , Ko-Ju Chuang , Sergio Ioppolo , Danna Qasim , Ewine F. van Dishoeck , Harold Linnartz

The rates of numerous activated reactions between neutral species increase at low temperatures through quantum mechanical tunneling of light hydrogen atoms. Although tunneling processes involving molecules or heavy atoms are well known in…

Context: Hydrogenation reactions are expected to be among the most important surface reactions on interstellar ices. However, solid state astrochemical laboratory data on reactions of H-atoms with common interstellar ice constituents are…

Astrophysics · Physics 2009-11-13 S. E. Bisschop , G. W. Fuchs , E. F. van Dishoeck , H. Linnartz

Recent laboratory experiments have demonstrated that, even though contribution from other reaction channels cannot be neglected, unsaturated hydrocarbons easily break their multiple C-C bonds to form CO after their interactions with atomic…

Solar and Stellar Astrophysics · Physics 2015-06-15 Angela Occhiogrosso , Serena Viti , Nadia Balucani

Density-functional theory calculations are performed to investigate hydrogen transport in the proton conductor BaSnO$_3$. Structural optimizations in the stable and saddle point configurations for transfer and reorientation allow…

Materials Science · Physics 2014-11-13 Grégory Geneste , Alistar Ottochian , Jessica Hermet , Guilhem Dezanneau

We investigate the role of carbon monoxide ice in the chemical evolution of prestellar cores using astrochemical rate equation models. We constrain the ratios of the binding energies on CO ice and H$_{2}$O ice for a series of adsorbates…

Astrophysics of Galaxies · Physics 2024-08-14 Germán Molpeceres , Kenji Furuya , Yuri Aikawa

We report new computational and experimental evidence of an efficient and astrochemically relevant formation route to formaldehyde (H$_2$CO). This simplest carbonylic compound is central to the formation of complex organics in cold…

Water ice is abundant both astrophysically, for example in molecular clouds, and in planetary systems. The Kuiper belt objects, many satellites of the outer solar system, the nuclei of comets and some planetary rings are all known to be…

Astrophysics · Physics 2009-11-13 Weijun Zheng , David Jewitt , Ralf I. Kaiser

$Aims$: We revisit with new augmented accuracy the theoretical dynamics of basic isotope exchange reactions involved in the $^{12}$C/$^{13}$C, $^{16}$O/$^{18}$O, and $^{14}$N/$^{15}$N balance because these reactions have already been…

Astrophysics of Galaxies · Physics 2015-06-19 Mirjana Mladenović , Evelyne Roueff

We present a combined experimental and theoretical study focussing on the quantum tunneling of atoms in the reaction between CH4 and OH. The importance of this reaction pathway is derived by investigating isotope substituted analogs.…

Astrophysics of Galaxies · Physics 2017-03-15 Thanja Lamberts , Gleb Fedoseev , Johannes Kästner , Sergio Ioppolo , Harold Linnartz

Glycolaldehyde (HOCH2CHO) is the most straightforward sugar detected in the Interstellar Medium (ISM) and participates in the formation pathways of molecules fundamental to life, red such as ribose and derivatives. Although detected in…

Astrophysics of Galaxies · Physics 2023-02-07 Mateus A. M. Paiva , Sergio Pilling , Edgar Mendoza , Breno R. L. Galvão , Heitor A. De Abreu

It is commonly believed that it is unfavourable for adsorbed H atoms on carbonaceous surfaces to form H$_2$ without the help of incident H atoms. Using ring-polymer instanton theory to describe multidimensional tunnelling effects, combined…

Chemical Physics · Physics 2022-04-05 Erxun Han , Wei Fang , Michail Stamatakis , Jeremy O. Richardson , Ji Chen

A prevailing theory for the interstellar production of complex organic molecules (COMs) involves formation on warm dust-grain surfaces, via the diffusion and reaction of radicals produced through grain-surface photodissociation of stable…

Astrophysics of Galaxies · Physics 2020-08-19 Mihwa Jin , Robin T. Garrod