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Quantum emitters located in proximity to a metal nanostructure individually transfer their energy via near-field excitation of surface plasmons. The energy transfer process increases the spontaneous emission (SE) rate due to…

We study cooperative effects in energy transfer (ET) from an ensemble of donors to an acceptor near a plasmonic nanostructure. We demonstrate that in cooperative regime ET takes place from plasmonic superradiant and subradiant states rather…

Mesoscale and Nanoscale Physics · Physics 2019-04-15 Vitaliy N. Pustovit , Augustine M. Urbas , Tigran V. Shahbazyan

We develop a theory of cooperative emission of light by an ensemble of emitters, such as fluorescing molecules or semiconductor quantum dots, located near a metal nanostructure supporting surface plasmon. The primary mechanism of…

Mesoscale and Nanoscale Physics · Physics 2015-05-14 Vitaliy N. Pustovit , Tigran V. Shahbazyan

We present a model for exciton-plasmon coupling based on an energy exchange mechanism between quantum emitters (QE) and localized surface plasmons in metal-dielectric structures. Plasmonic correlations between QEs give rise to a collective…

Mesoscale and Nanoscale Physics · Physics 2020-11-12 Tigran V. Shahbazyan

We develop a theory for spontaneous decay of a quantum emitter (QE) situated near metal-dielectric structure supporting localized surface plasmons. If plasmon resonance is tuned close to the QE emission frequency, the emission is enhanced…

Mesoscale and Nanoscale Physics · Physics 2022-10-19 Tigran V. Shahbazyan

Rate of single-photon generation by quantum emitters (QEs) can be enhanced by placing a QE inside a resonant structure. This structure can represent an all-dielectric micro-resonator or waveguide and thus be characterized by ultra-low loss…

Mesoscale and Nanoscale Physics · Physics 2017-01-25 Sergey I. Bozhevolnyi , Jacob B. Khurgin

We develop a unified theory of plasmon-assisted resonance energy transfer (RET) between molecules near a metal nanostructure that maintains energy balance between transfer, dissipation, and radiation. We show that in a wide range of…

Mesoscale and Nanoscale Physics · Physics 2015-05-19 Vitaliy N. Pustovit , Tigran V. Shahbazyan

We show that a single quantum emitter can efficiently couple to the tunable plasmons of a highly doped single-wall carbon nanotube (SWCNT). Plasmons in these quasi-one-dimensional carbon structures exhibit deep subwavelength confinement…

Mesoscale and Nanoscale Physics · Physics 2015-10-28 Luis Martin-Moreno , F. Javier Garcia de Abajo , Francisco J. Garcia-Vidal

The Purcell effect - the modification of the spontaneous emission rate in presence of resonant cavities or other resonant objects - is a fundamental effect of quantum electrodynamics. However, a change of the emission rate caused by…

Plasmonic superradiance originates from the plasmon mediated strong correlation that builds up between dipolar emitters coupled to a metal nanoparticle. This leads to a fast burst of emission so that plasmonic superradiance constitutes…

Quantum Physics · Physics 2019-08-07 H. Varguet , S. Guérin , H. R. Jauslin , G.

Cavity-embedded quantum emitters show strong modifications of free space radiation properties such as an enhanced decay known as the Purcell effect. The central parameter is the cooperativity $C$, the ratio of the square of the coherent…

Quantum Physics · Physics 2019-05-01 David Plankensteiner , Christian Sommer , Michael Reitz , Helmut Ritsch , Claudiu Genes

A surrounding electromagnetic environment can engineer spontaneous emissions from quantum emitters through the Purcell effect. For instance, a plasmonic antenna can efficiently confine an electromagnetic field and enhance the fluorescent…

Optics · Physics 2021-12-22 Jingyi Zhao , Weidong Zhang , Te Wen , Lulu Ye , Hai Lin , Jinglin Tang , Qihuang Gong , Guowei Lu

We obtain the local density of states (LDOS) for any nanoplasmonic system in the frequency range dominated by a localized surface plasmon. By including the Ohmic losses in a consistent way, we show that the plasmon LDOS is proportional to…

Mesoscale and Nanoscale Physics · Physics 2016-11-10 Tigran V. Shahbazyan

Using large-scale, real-time quantum dynamics calculations, we present a detailed analysis of electronic excitation transfer (EET) mechanisms in a multi-particle plasmonic nanoantenna system. Specifically, we utilize real-time,…

Mesoscale and Nanoscale Physics · Physics 2018-03-06 Niranjan V. Ilawe , M. Belén Oviedo , Bryan M. Wong

Plasmon resonant arrays or meta-surfaces shape both the incoming optical field and the local density of states for emission processes. They provide large regions of enhanced emission from emitters and greater design flexibility than single…

The quantum network model with real variables is usually used to describe the excitation energy transfer (EET) in the Fenna-Matthews-Olson(FMO) complexes. In this paper we add the quantum phase factors to the hopping terms and find that the…

Molecular Networks · Quantitative Biology 2015-03-20 Bao-quan Ai , Shi-Liang Zhu

Exciton-surface plasmon coupling is at the heart of the most elementary light-matter interactions and is a result of not only an intrinsic property of the emitter but that of emitter-environment interaction. Thus, change of electromagnetic…

Optics · Physics 2022-03-11 J. S. Duan

The present work deals with a theoretical research on the emission and radiation properties of a dipole emitter source close to a dimer graphene plasmonic antenna. Modification of the radiation and the quantum efficiencies resulting from…

Optics · Physics 2018-10-17 Mauro Cuevas

We identify a new mechanism for cooperative emission of light by an ensemble of N dipoles near a metal nanostructure supporting a surface plasmon.The cross-talk between emitters due to virtual plasmon exchange leads to a formation of three…

Materials Science · Physics 2015-05-13 Vitaliy N. Pustovit , Tigran V. Shahbazyan

We present a combined experimental and simulation study of a single self-assembled InGaAs quantum dot coupled to a nearby ($\sim 25nm$) plasmonic antenna. Micro-photoluminescence spectroscopy shows a $\sim 2.4\times$ increase of intensity,…

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