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Reliable predictions of the static and dynamic properties of a nucleus require a fully microscopic description of both ground and excited states of this complicated many-body quantum system. Predictive calculations are key to understanding…

Nuclear Theory · Physics 2022-10-19 Emanuel V. Chimanski , Eun Jin In , Jutta E. Escher , Sophie Péru , Walid Younes

Using the Dirac equation, we study corrections to electron binding energies and hyperfine splittings of atomic hydrogen and hydrogen-like ions due to finite nuclear size (FNS) effects, relativistic QED radiative corrections and nuclear…

Atomic Physics · Physics 2023-06-06 Igor Kuzmenko , Tetyana Kuzmenko , Y. Avishai , Y. B. Band

We present fully numerical electronic structure calculations on diatomic molecules exposed to an external magnetic field at the unrestricted Hartree-Fock limit, using a modified version of a recently developed finite element program,…

Chemical Physics · Physics 2020-02-12 Susi Lehtola , Maria Dimitrova , Dage Sundholm

Neutral uranium (U I) is a very difficult atom for theoretical calculations due to a large number of valence electrons, six, strong valence-valence and valence-core correlations, high density of states, and relativistic effects.…

Atomic Physics · Physics 2020-10-14 Igor M. Savukov

We present calculations of the hyperfine coupling constants for all the heteronuclear alkali-metal diatomic molecules at the equilibrium geometry of the electronic ground state. These constants are important in developing methods to control…

Atomic Physics · Physics 2017-11-01 J. Aldegunde , J. M. Hutson

A simple approximation within the framework of the hybrid methods for the calculation of the electronic structure of solids is presented. By considering only the diagonal elements of the perturbation operator (Hartree-Fock exchange minus…

Materials Science · Physics 2012-01-31 Fabien Tran

Nuclear structure corrections of orders $Z\alpha\, E_F$ and $(Z\alpha)^2 E_F$ are calculated for the hyperfine splitting of the muonic deuterium. The obtained results disagree with previous calculations and lead to a $5\,\sigma$…

Atomic Physics · Physics 2019-01-02 Marcin Kalinowski , Krzysztof Pachucki , Vladimir A. Yerokhin

Calculation of statistical properties of nuclei in a finite-temperature mean-field theory requires projection onto good particle number, since the theory is formulated in the grand canonical ensemble. This projection is usually carried out…

Nuclear Theory · Physics 2018-01-23 P. Fanto , Y. Alhassid , G. F. Bertsch

Density functional theory (DFT) provides a theoretical framework for efficient and fairly accurate calculations of the electronic structure of molecules and crystals. The main features of density functional theory are described and DFT…

Chemical Physics · Physics 2012-06-12 Hauke Paulsen , Alfred Xaver Trautwein

We study the low temperature transport characteristics of a disordered metal in the presence of electron-electron interactions. We compare Hartree-Fock and dynamical mean field theory (DMFT) calculations to investigate the scattering…

Strongly Correlated Electrons · Physics 2011-09-20 E. C. Andrade , E. Miranda , V. Dobrosavljevic

The self-energy of the Dirac Brueckner-Hartree-Fock calculation in nuclear matter is parametrized by introducing density-dependent coupling constants of isoscalar mesons in the relativistic Hartree-Fock (RHF) approach where isoscalar meson…

Nuclear Theory · Physics 2009-10-28 Hua-lin Shi , Bao-qiu Chen , Zhong-yu Ma

Empirical fitting of parameters in approximate density functionals is common. Such fits conflate errors in the self-consistent density with errors in the energy functional, but density-corrected DFT (DC-DFT) separates these two. We…

Chemical Physics · Physics 2020-12-02 Suhwan Song , Stefan Vuckovic , Eunji Sim , Kieron Burke

In this manuscript we provide an outline of the numerical methods used in implementing the density constrained time-dependent Hartree-Fock (DC-TDHF) method and provide a few examples of its application to nuclear fusion. In this approach,…

Nuclear Theory · Physics 2015-02-16 V. E. Oberacker , A. S. Umar

Advances in laser spectroscopy of superheavy ($Z>100$) elements enabled determination of the nuclear moments of the heaviest nuclei, which requires high-precision atomic calculations of the relevant hyperfine structure (HFS) constants.…

Atomic Physics · Physics 2018-12-05 S. G. Porsev , M. S. Safronova , U. I. Safronova , V. A. Dzuba , V. V. Flambaum

An algorithm for the calculation of hyperfine structure and spectra of diatomic molecules based on the variational nuclear motion is presented. Hyperfine coupling terms considered are Fermi-contact, nuclear spin-electron spin dipole-dipole,…

Chemical Physics · Physics 2022-02-15 Qianwei Qu , Sergei N. Yurchenko , Jonathan Tennyson

The largest uncertainty in calculations of hydrogen ground-state hyperfine splitting comes from corrections due to proton stucture. We review these corrections, with special mention of the inelastic, or polarizability, corrections which…

High Energy Physics - Phenomenology · Physics 2007-05-23 Carl E. Carlson

Condensed Fermi systems with an odd number of particles can be described by means of polarizing external fields having a time-odd character. We illustrate how this works for Fermi gases and atomic nuclei treated by density functional theory…

Superconductivity · Physics 2009-09-20 George Bertsch , Jacek Dobaczewski , Witold Nazarewicz , Junchen Pei

Relativistic Hartree-Fock-Bogoliubov (RHFB) theory with density-dependent meson-nucleon couplings is presented. The integro-differential RHFB equations are solved by expanding the different components of the quasi-particle spinors in the…

Nuclear Theory · Physics 2010-04-06 Wen Hui Long , Peter Ring , Nguyen Van Giai , Jie Meng

Several pairing schemes currently used to describe superfluid nuclei through Hartree-Fock-Bogolyubov (HFB) calculations are briefly reviewed. We put a particular emphasis on the regularization recipes used in connection with zero-range…

Nuclear Theory · Physics 2007-05-23 T. Duguet , K. Bennaceur , P. Bonche

We formulate a new scheme of the Hartree-Fock-Bogoliubov mean-field theory applicable to weakly bound and pair correlated deformed nuclei using the coordinate-space Green's function technique. On the basis of a coupled-channel…

Nuclear Theory · Physics 2009-08-20 Hiroshi Oba , Masayuki Matsuo