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Related papers: The LDA-1/2 method applied to atoms and molecules

200 papers

Many-body perturbation theory methods, such as the $G_0W_0$ approximation, are able to accurately predict quasiparticle (QP) properties of several classes of materials. However, the calculation of the QP band structure of two-dimensional…

Materials Science · Physics 2022-06-23 Alberto Guandalini , Pino D'Amico , Andrea Ferretti , Daniele Varsano

Density functional theory within the local or semilocal density approximations (DFT-LDA/GGA) has become a workhorse in electronic structure theory of solids, being extremely fast and reliable for energetics and structural properties, yet…

A novel hybrid scheme is proposed. The {\it ab initio} LDA calculation is used to construct the Wannier functions and obtain single electron and Coulomb parameters of the multiband Hubbard-type model. In strong correlation regime the…

Strongly Correlated Electrons · Physics 2007-05-23 V. A. Gavrichkov , M. M. Korshunov , S. G. Ovchinnikov , I. A. Nekrasov , Z. V. Pchelkina , V. I. Anisimov

The structural and electronic properties of the wurtzite phase of the InAs and GaAs compounds are, for the first time, studied within the framework of Density Functional Theory (DFT). We used the full-potential linearized augmented plane…

Materials Science · Physics 2007-05-23 Zeila Zanolli , Ulf von Barth

We study the Mott insulating phase of the one-dimensional Hubbard model using a local-density approximation (LDA) that is based on the Bethe Ansatz (BA). Unlike conventional functionals, the BA-LDA has an explicit derivative discontinuity.…

Strongly Correlated Electrons · Physics 2009-11-07 N. A. Lima , L. N. Oliveira , K. Capelle

The outstanding optoelectronics and photovoltaic properties of metal halide perovskites, including high carrier motilities, low carrier recombination rates, and the tunable spectral absorption range are attributed to the unique electronic…

Materials Science · Physics 2020-08-14 Shuxia Tao , Xi Cao , Peter Bobbert

An $\it{ab \,\, initio}$ based fully microscopic approach is applied to study the nonlinear optical response of bulk Tellurium. The structural and electronic properties are calculated from first principles using the shLDA-1/2 method within…

Optics · Physics 2021-08-20 S. C. Liebscher , M. K. Hagen , J. Hader , J. V. Moloney , S. W. Koch

Calculating the quasiparticle (QP) band structure of two-dimensional (2D) materials within the GW self-energy approximation has proven to be a rather demanding computational task. The main reason is the strong $\mathbf{q}$-dependence of the…

Materials Science · Physics 2016-10-12 Filip A. Rasmussen , Per S. Schmidt , Kirsten T. Winther , Kristian S. Thygesen

The electronic structures and optical properties of cubic HfO2 are calculated by means of generalized gradient approximation (GGA) +U approach. Without on-site Coulomb interactions, the band gap of cubic HfO2 is 2.92eV, much lower than the…

Materials Science · Physics 2013-11-26 Jinping Li , Songhe Meng , Lingling Li , Hantao Lu , Takami Tohyama

We discuss a general approach to a realistic theory of the electronic structure in materials containing correlated d- or f- electrons. The main feature of this approach is the taking into account the energy dependence of the electron…

Strongly Correlated Electrons · Physics 2009-10-30 A. I. Lichtenstein , M. I. Katsnelson

Although the GW approximation is recognized as one of the most accurate theories for predicting materials excited states properties, scaling up conventional GW calculations for large systems remains a major challenge. We present a powerful…

Computational Physics · Physics 2018-03-28 Weiwei Gao , Weiyi Xia , Xiang Gao , Peihong Zhang

We examine the influence of the relativistic effects within the linear augmented plane wave method (LAPW) for solids and propose a few alternative ways to accurately take them into account: (1) we introduce new radial dependencies for LAPW…

Materials Science · Physics 2026-04-14 A. V. Nikolaev , U. N. Kurelchuk , E. V. Tkalya

We present a $GW$ space-time algorithm for periodic systems in a Gaussian basis including spin-orbit coupling. We employ lattice summation to compute the irreducible density response and the self-energy, while we employ $k$-point sampling…

We provide a straightforward and efficient procedure to combine LDA+U total energy functional with the full potential linearized augmented plane wave method. A detailed derivation of the LDA+U Kohn-Sham type equations is presented for the…

Strongly Correlated Electrons · Physics 2009-10-31 A. B. Shick , A. I. Liechtenstein , W. E. Pickett

Very recently, in the 2011 version of the Wien2K code, the long standing shortcome of the codes based on Density Functional Theory, namely, its impossibility to account for the experimental band gap value of semiconductors, was overcome.…

Materials Science · Physics 2013-09-10 J. A. Camargo-Martinez , R. Baquero

Combining the density functional theory (DFT) and the Gutzwiller variational approach, a LDA+Gutzwiller method is developed to treat the correlated electron systems from {\it ab-initio}. All variational parameters are self-consistently…

Strongly Correlated Electrons · Physics 2009-11-13 XiaoYu Deng , Xi Dai , Zhong Fang

We calculate the electronic structure of several atoms and small molecules by direct minimization of the Self-Interaction Corrected Local Density Approximation (SIC-LDA) functional. To do this we first derive an expression for the gradient…

Condensed Matter · Physics 2009-10-28 S. Goedecker , C. J. Umrigar

A GW approximation (GWA) method named U+GWA is proposed, where we can start GWA with more localized wave functions obtained by the local spin-density approximation (LSDA)+U method. Then GWA and U+GWA are applied to MnO, NiO, and V$_2$O$_3$…

Strongly Correlated Electrons · Physics 2008-10-18 S. Kobayashi , Y. Nohara , S. Yamamoto , T. Fujiwara

We implemented combination of DMFT and $GW$ in its fully self-consistent way, one shot $GW$ approximation, and quasiparticle self-consistent scheme, and studied how well these combined methods perform on H$_2$ molecule as compared to more…

Strongly Correlated Electrons · Physics 2017-04-12 Juho Lee , Kristjan Haule

The band gap is an important parameter of semiconductor materials that influences several functional properties, in particular optical properties. However, a fast and reliable first-principles prediction of band gaps remains a challenging…