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Second harmonic generation (SHG) extensively employs periodically poled nonlinear crystals through forward quasi-phase-matching to achieve efficient frequency conversion. As poling periods approach sub-micrometers, backward…

Optics · Physics 2024-07-15 Fengyan Yang , Juanjuan Lu , Mohan Shen , Guangcanlan Yang , Hong X. Tang

The stacking configuration of two-dimensional materials critically governs their optical and electronic responses. Monolayer transition-metal dichalcogenides (TMDC) lack inversion symmetry and exhibit exciton-enhanced second-harmonic…

The effective second-harmonic generation (SHG) coefficient is a crucial data that quantifies the efficiency of transforming fundamental frequency light into its second harmonic. With the help of the symmetry of nonlinear optical…

Optimization and Control · Mathematics 2026-02-24 Die Xiao , Yisheng Song

Little is known about the role of weak interlayer coupling in the second harmonic generation (SHG) effects of two-dimensional van der Waals (vdW) systems. In this article, taking homo-bilayer $MoS_2/MoS_2$ and hetero-bilayer $MoS_2/MoSe_2$…

Computational Physics · Physics 2022-02-02 Xiao Jiang , Lei Kang , Bing Huang

The nonlinear process of second harmonic generation (SHG) in monolayer (1L) transition metal dichalcogenides (TMD), like $WS_2$, strongly depends on the polarization state of the excitation light. Combining plasmonic nanostructures with…

Optics · Physics 2021-10-08 Florian Spreyer , Claudia Ruppert , Philip Georgi , Thomas Zentgraf

An optical Second-Harmonic Generation (SHG) allows to probe various structural and symmetry-related properties of materials, since it is sensitive to the inversion symmetry breaking in the system. Here, we investigate the SHG response from…

Mesoscale and Nanoscale Physics · Physics 2019-05-08 M. Vandelli , M. I. Katsnelson , E. A. Stepanov

We theoretically investigate the second harmonic generation (SHG) of topological insulator surface states in a perpendicular magnetic field. Our theory is based on the microscopic expression of the second-order magneto-optical conductivity…

Mesoscale and Nanoscale Physics · Physics 2024-11-27 Kainan Chang , Muhammad Zubair , Jin Luo Cheng , Wang-Kong Tse

The second-order $\chi^{2}$ process underpins many important nonlinear optical applications in the field of classical and quantum optics. Generally, the $\chi^{2}$ process manifests itself only in a non-centrosymmetric dielectric medium via…

Optics · Physics 2022-06-29 Yadong Wang , Daniel Burt , Kunze Lu , Donguk Nam

We report ionic strength-dependent phase shifts in second harmonic generation (SHG) signals from charged interfaces that verify a recent model in which dispersion between the fundamental and second harmonic beams modulates observed signal…

Second-harmonic generation (SHG) is a fundamental tool in modern laser technology, enabling coherent frequency conversion to remote optical bands, serving as the basis for self-referenced femtosecond lasers and quadrature-squeezed light…

Optics · Physics 2025-12-10 Nikolai Kuznetsov , Zihan Li , Tobias J. Kippenberg

We study the second harmonic generation (SHG) in a suspension of small spherical particles confined within a slab, assuming undepleted pump and applying (i) single scattering approximation and (ii) diffusion approximation. In the case (i),…

Optics · Physics 2007-05-23 E. V. Makeev , S. E. Skipetrov

The notion of spontaneous symmetry breaking has been used to describe phase transitions in a variety of physical systems. In crystalline solids, the breaking of certain symmetries, such as mirror symmetry, is difficult to detect…

Materials Science · Physics 2020-07-01 Bryan T. Fichera , Anshul Kogar , Linda Ye , Bilal Gökce , Alfred Zong , Joseph G. Checkelsky , Nuh Gedik

Optical second harmonic generation (SHG) is used as a noninvasive probe of two-dimensional (2D) ferroelectricity in Langmuir-Blodgett (LB) films of copolymer vinylidene fluoride with trifluorethylene. The surface 2D…

Polarized and azimuthal dependencies of optical second harmonics generation (SHG) at the surface of noncentrosymmetric semiconductor crystals have been measured on polished surfaces of ZnSe(100), using a fundamental wavelength of 1.06$\mu…

Optics · Physics 2007-05-23 Xiangyang Song , Arnold Neumann , Rein Maripuu , Kai Siegbahn

Second-harmonic generation (SHG) is a well-known nonlinear spectroscopy method to probe electronic structure, specifically, in transition metal dichalcogenide (TMDC) monolayers. This work investigates the nonlinear dynamics of a strongly…

Stacked atomically thin transition metal dichalcogenides (TMDs) exhibit fundamentally new physical properties compared to those of the individual layers. The twist angle between the layers plays a crucial role in tuning these properties.…

Optical second-harmonic generation (SHG) is studied for the confined geometry of a circular cylindrical waveguide or optical fiber. A model situation of high symmetry is considered where the material with nonlinear susceptibility is…

Optics · Physics 2013-09-17 B. U. Felderhof , G. Marowsky

We analyze second-harmonic generation (SHG) at a thin effectively quadratic nonlinear interface between two linear optical media. We predict multistability of SHG for both plane and localized waves, and also describe two-color localized…

patt-sol · Physics 2007-05-23 Andrey A. Sukhorukov , Yuri S. Kivshar , Ole Bang

This research will examine the computational methods to calculate the nonlinear optical process of second harmonic generation (SHG) that will be hypothesized to be present during lithium ion insertion into silicon nanowires. First it will…

Optics · Physics 2021-10-19 Donald C. Boone

3R-MoS2, a MoS2 polytype with broken inversion symmetry, enables unique light-matter interactions and is promising for linear and nonlinear integrated photonics beyond the monolayer limit. Yet, systematic studies of its thickness-dependent…