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{\it Ab initio\} calculations have been successfully used for evaluating lattice dynamical properties of solids within the (quasi-)harmonic approximation (i.e., assuming non-interacting phonons with infinite lifetimes), but it remains…

Computational Physics · Physics 2019-11-25 Fei Zhou , Weston Nielson , Yi Xia , Vidvuds Ozolins

First-principles prediction of lattice thermal conductivity $\kappa_L$ of strongly anharmonic crystals is a long-standing challenge in solid state physics. Making use of recent advances in information science, we propose a systematic and…

Materials Science · Physics 2015-11-17 Fei Zhou , Weston Nielson , Yi Xia , Vidvuds Ozolins

This article reviews the current status of lattice-dynamical calculations in crystals, using density-functional perturbation theory, with emphasis on the plane-wave pseudo-potential method. Several specialized topics are treated, including…

Materials Science · Physics 2009-10-31 S. Baroni , S. de Gironcoli , A. Dal Corso , P. Giannozzi

On the basis of the self-consistent phonon theory and the special displacement method, we develop an approach for the treatment of anharmonicity in solids. We show that this approach enables the efficient calculation of…

Materials Science · Physics 2023-08-09 Marios Zacharias , George Volonakis , Feliciano Giustino , Jacky Even

We introduce a new linear response method to study the lattice dynamics of materials with strong correlations. It is based on a combination of dynamical mean field theory of strongly correlated electrons and the local density functional…

Strongly Correlated Electrons · Physics 2009-11-07 S. Y. Savrasov , G. Kotliar

In recent years, the fundamental physics of spin-thermal (i.e., magnon-phonon) interaction has attracted significant experimental and theoretical interests given its potential paradigm-shifting impacts in areas like spin-thermoelectrics,…

Materials Science · Physics 2018-03-14 Xufei Wu , Zeyu Liu , Tengfei Luo

Information over the phonon band structure is crucial to predicting many thermodynamic properties of materials, such as thermal transport coefficients. Highly accurate phonon dispersion curves can be, in principle, calculated in the…

Materials Science · Physics 2020-11-25 Miquel Royo , Konstanze R. Hahn , Massimiliano Stengel

The phonon dispersion relations of crystal lattices can often be well-described with the harmonic approximation. However, when the potential energy landscape exhibits more anharmonicity, for instance, in case of a weakly bonded crystal or…

Materials Science · Physics 2022-01-19 Jonathan Lahnsteiner , Menno Bokdam

Knowledge of lattice anharmonicity is essential to elucidate distinctive thermal properties in crystalline solids. Yet, accurate \textit{ab initio} investigations of lattice anharmonicity encounter difficulties owing to the cumbersome…

Materials Science · Physics 2022-04-13 Zhen Zhang , Dong-Bo Zhang , Tao Sun , Renata M. Wentzcovitch

Phononic properties are commonly studied by calculating force constants using the density functional theory (DFT) simulations. Although DFT simulations offer accurate estimations of phonon dispersion relations or thermal properties, but for…

A simple and accurate method of calculating phonon spectra in mixed semiconductors alloys, on the basis of preliminarily (from first principles) relaxed atomic structure, is proposed and tested for (Zn,Be)Se and (Ga,In)As solid solutions.…

Materials Science · Physics 2008-01-08 Ayoub Nassour , Joseph Hugel , A. V. Postnikov

We apply standard, first-principles calculations to a complete treatment of lattice dynamics in the harmonic approximation. The algorithm makes use of the straightforward ``frozen-phonon'' approach to the calculation of vibrational spectra…

Materials Science · Physics 2007-05-23 Hadley M. Lawler , Eric K. Chang , Eric L. Shirley

An accurate and easily extendable method to deal with lattice dynamics of solids is offered. It is based on first-principles molecular dynamics simulations and provides a consistent way to extract the best possible harmonic - or higher…

Materials Science · Physics 2013-10-14 Olle Hellman , I. A. Abrikosov , S. I. Simak

The existing techniques of account for the phonon dispersion are computationally costly, while its impact on a variety of thermodynamic properties appears negligible. We develop a mathematical formalism, which allows for clear understanding…

Statistical Mechanics · Physics 2014-05-01 Roman Belousov , Mauro Prencipe

Phonon dispersions in <100> silicon nanowires (SiNW) are modeled using a Modified Valence Force Field (MVFF) method based on atomistic force constants. The model replicates the bulk Si phonon dispersion very well. In SiNWs, apart from four…

Mesoscale and Nanoscale Physics · Physics 2015-03-17 Abhijeet Paul , Mathieu Luisier , Gerhard Klimeck

Phonons are quantized vibrations of a crystal lattice that play a crucial role in understanding many properties of solids. Density functional theory (DFT) provides a state-of-the-art computational approach to lattice vibrations from…

We demonstrate how supercell implementations of conventional lattice dynamical calculations can be used to determine the extent and nature of disorder-induced broadening in the phonon dispersion spectrum of disordered crystalline materials.…

Disordered Systems and Neural Networks · Physics 2017-04-26 Alistair R. Overy , Arkadiy Simonov , Philip A. Chater , Matthew G. Tucker , Andrew L. Goodwin

First principles predictions of lattice dynamics are of vital importance for a broad range of topics in materials science and condensed matter physics. The large-scale nature of lattice dynamics calculations and the desire to design novel…

Materials Science · Physics 2023-01-23 Jinliang Ning , James W. Furness , Jianwei Sun

The coherent lattice vibrations significantly impact physical and chemical processes in solids, such as heat transfer, displacive phase transitions, and thermal conductivity. Thus, probing lattice dynamics in real-space and real-time is…

Optics · Physics 2026-05-21 Navdeep Rana

Using a computationally inexpensive frozen phonon approach we have developed a technique which can be used to screen large unit cell materials and systems for enhanced superconducting critical temperatures. The method requires only density…

Superconductivity · Physics 2024-05-07 Oliver A. Dicks , Kateryna Foyevtsova , Ilya Elfimov , Rohit Prasankumar , George Sawatzky
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