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The effect of magnetic STM-tip on electronic, magnetic and electronic transport properties through the molecule junction STM-tip-Co/CoPc/Co(111), has been investigated by mean of ab initio electronic structure calculations. The spin…

Quantum Physics · Physics 2025-02-25 Ali Jaafar , Tarek Khalil

We present a generalized extension of the recently developed electron/hole-transfer Dynamically-weighted State-Averaged Constrained CASSCF (eDSC/hDSC) method to model charge transfer in the presence of spin-orbit coupling (SOC) for systems…

Chemical Physics · Physics 2026-02-13 Alok Kumar , Zhen Tao , Joseph E. Subotnik , Tian Qiu

The control of spins and spin to charge conversion in organics requires understanding the molecular spin-orbit coupling (SOC), and a means to tune its strength. However, quantifying SOC strengths indirectly through spin relaxation effects…

We study the electronic transport through a spin-1 molecule in which mechanical stretching produces a magnetic anisotropy. In this type of device, a vibron mode along the stretching axis will couple naturally to the molecular spin. We…

Strongly Correlated Electrons · Physics 2012-07-31 David A. Ruiz-Tijerina , Pablo S. Cornaglia , C. A. Balseiro , Sergio E. Ulloa

In contrast to the static operations of conventional semiconductor devices, the dynamic conformational freedom in molecular devices opens up the possibility of using molecules as new types of devices such as a molecular conformational…

Mesoscale and Nanoscale Physics · Physics 2009-07-02 Daijiro Nozaki , Gianaurelio Cuniberti

We present a theoretical model of spin transitions in stacks of molecular layers. Our model captures the already established physics of these systems (thermal hysteretic transitions and crossovers) and suggests a way towards in situ control…

Strongly Correlated Electrons · Physics 2019-12-25 O. I. Utesov , S. Burdin , P. Rosa , M. Gonidec , L. Poggini , S. V. Andreev

Molecular spintronics devices (MSDs) are highly promising candidates for enabling quantum computation and revolutionizing computer logic and memory. An advanced MSD will require the placement of magnetic molecules between the two…

Mesoscale and Nanoscale Physics · Physics 2019-12-04 Pawan Tyagi , Christopher D Angelo , Collin Baker

Materials with spin-crossover (SCO) properties hold great potentials in information storage and therefore have received a lot of concerns in the recent decades. The hysteresis phenomena accompanying SCO is attributed to the intermolecular…

Chemical Physics · Physics 2022-10-11 Hong-zhou Ye , Chong Sun , Hong Jiang

The recent experimental realization of spin-orbit coupling for ultracold atomic gases provides a powerful platform for exploring many interesting quantum phenomena. In these studies, spin represents spin vector (spin-1/2 or spin-1) and…

Quantum Gases · Physics 2017-11-15 Xi-Wang Luo , Kuei Sun , Chuanwei Zhang

Spin-orbit coupling (SOC) is pivotal for various fundamental spin-dependent phenomena in solids and their technological applications. In semiconductors, these phenomena have been so far studied in relatively weak electron-electron…

Mesoscale and Nanoscale Physics · Physics 2021-06-09 D. Maryenko , M. Kawamura , A. Ernst , V. K. Dugaev , E. Ya. Sherman , M. Kriener , M. S. Bahramy , Y. Kozuka , M. Kawasaki

Among the different types of switchable molecular compounds, sublimable Fe(II) SCO molecules provide a suitable platform to develop smart devices that respond to external stimuli. Here we report the synthesis, crystallographic structure and…

Magnetic switching of a single-molecule magnet (SMM) due to spin-polarized current is investigated theoretically. The charge transfer between the electrodes takes place via the lowest unoccupied molecular orbital (LUMO) of the SMM.…

Mesoscale and Nanoscale Physics · Physics 2007-08-29 Maciej Misiorny , Józef Barnas

The change of conductance of single molecule junctions in response to various external stimuli is the fundamental mechanism for single-molecule electronic devices with multiple functionalities. We propose a concept that the conductance of…

Mesoscale and Nanoscale Physics · Physics 2014-12-04 Chengbo Zhu , Xiaolin Wang

Control over quantum systems is typically achieved by time-dependent electric or magnetic fields. Alternatively, electronic spins can be controlled by spin-polarized currents. Here we demonstrate coherent driving of a single spin by a…

Mesoscale and Nanoscale Physics · Physics 2024-06-26 Stepan Kovarik , Richard Schlitz , Aishwarya Vishwakarma , Dominic Ruckert , Pietro Gambardella , Sebastian Stepanow

The interplay between chirality and magnetism has been a source of fascination among scientists for over a century. In recent years, chirality-induced spin selectivity (CISS) has attracted renewed interest. It has been observed that…

Mesoscale and Nanoscale Physics · Physics 2024-08-07 Mohammad Reza Safari , Frank Matthes , Claus M. Schneider , Karl-Heinz Ernst , Daniel E. Bürgler

Spin-orbit coupling (SOC), the intrinsic interaction between a particle spin and its motion, is responsible for various important phenomena, ranging from atomic fine structure to topological condensed matter physics. The recent experimental…

Quantum Gases · Physics 2013-07-05 Yongping Zhang , Gang Chen , Chuanwei Zhang

Molecular bridges covalently bonded to two ferromagnetic electrodes can transform ferromagnetic materials and produce intriguing spin transport characteristics. This paper discusses the impact of molecule induced strong coupling on spin…

Materials Science · Physics 2019-12-04 Pawan Tyagi , Edward Friebe

Polar molecules in selected quantum states can be guided, decelerated, and trapped using electric fields created by microstructured electrodes on a chip. Here we explore how transitions between two of these quantum states can be induced…

Atomic Physics · Physics 2015-03-17 Gabriele Santambrogio , Samuel A. Meek , Mark J. Abel , Liam M. Duffy , Gerard Meijer

Spin-crossover complexes exhibit two stable configurations with distinct spin states. The investigation of these molecules using low-temperature scanning tunneling microscopy has opened new perspectives for understanding the associated…

Mesoscale and Nanoscale Physics · Physics 2026-01-05 Jonas Fußangel , Björn Sothmann , Sven Johannsen , Sascha Ossinger , Felix Tuczek , Richard Berndt , Jürgen König , Manuel Gruber

Spin-orbit (SO) interaction critically influences electron spin dynamics and spin transport in bulk semiconductors and semiconductor microstructures. This interaction couples electron spin to dc and ac electric fields. Spin coupling to ac…

Mesoscale and Nanoscale Physics · Physics 2009-11-10 Emmanuel I. Rashba
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