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A combined experimental and theoretical investigation of the electronic structure of the archetypal oxide heterointerface system LaAlO3 on SrTiO3 is presented. High-resolution, hard x-ray photoemission is used to uncover the occupation of…

Bi2Se3 and Bi2Te3 are layered compounds of technological importance, being excellent thermoelectric materials as well as topological insulators. We report density functional theory calculations of the atomic, electronic and thermoelectric…

Materials Science · Physics 2013-08-08 Xin Luo , Michael B. Sullivan , Su Ying Quek

An electro-optic modulator offers the function of modulating the propagation of light in a material with electric field and enables seamless connection between electronics-based computing and photonics-based communication. The search for…

Materials Science · Physics 2022-05-11 Yang Liu , Guodong Ren , Tengfei Cao , Rohan Mishra , Jayakanth Ravichandran

The anisotropic optical properties of multiferroic BiFeO$_3$ thin films have been determined with Mueller matrix ellipsometry at room-temperature. The full dielectric tensors of tetragonal-like and rhombohedral-like BiFeO$_3$ phases…

Materials Science · Physics 2015-08-26 Daniel Schmidt , Lu You , Xiao Chi , Junling Wang , Andrivo Rusydi

Using atomic-force microscopy (AFM) and wide-band (0.02-8.5 eV) spectroscopic ellipsometry techniques we investigated morphology and optical properties of Cd3As2 films grown by non-reactive rf magnetron sputtering on two types of oriented…

Materials Science · Physics 2023-01-16 Natalia Kovaleva , Ladislav Fekete , Dagmar Chvostova , Andrei Muratov

Properties of complex oxide thin films can be tuned over a range of values as a function of mismatch, composition, orientation, and structure. Here, we report a strategy for growing structured epitaxial thermoelectric thin films leading to…

Materials Science · Physics 2013-10-08 D. Pravarthana , O. I. Lebedev , D. Chateigner , S. Hebert , P. A. Salvador , W. Prellier

LaAlO3-Ba0.5Sr0.5TiO3 (LAO-BST) thin films, with different LAO contents, were deposited on Pt/Ti/SiO2/Si and (100) LaAlO3 substrate, via a pulsed laser deposition (PLD). Phase composition and microstructure of the LAO-BST thin films were…

Materials Science · Physics 2007-05-23 L. B. Kong , L. Yan , K. B. Chong , C. Y. Tan , L. F. Chen , C. K. Ong

Surface Acoustic Waves on piezoelectric substrates can be used to investigate the dynamic conductivity of thin films in a non-contact and very sensitive way, especially at low conductivities. Here, we report on such surface acoustic wave…

Statistical Mechanics · Physics 2007-05-23 Andreas Heinrich , Andreas L. Hoerner , Achim Wixforth , Bernd Stritzker

Thin films of pure and self-deficient calcium titanites i.e., CaTiO$_3$, Ca$_{1-\alpha}$TiO$_3$, CaTi$_{1-\beta}$O$_3$ and CaTiO$_{3-\gamma}$ have been deposited on ITO substrate using dip coating method. X-ray diffraction and Scanning…

Materials Science · Physics 2023-02-14 Shashi Pandey , Alok Shukla , Anurag Tripathi

Using density-functional-theory (DFT) calculations with the HSE06 hybrid functional, we accurately evaluate the critical thickness of LaAlO3 film for the intrinsic doping in LaAlO3/SrTiO3 (LAO/STO) heterstructures. The calculated critical…

Materials Science · Physics 2018-04-13 Yun Li , Xinyuan Wei , Jaejun Yu

We develop a phenomenological thermodynamic theory of ferroelectric BaTiO3 (BT) thin films epitaxially grown on cubic substrates using the Landau-Devonshire eight-order potential. The constructed "misfit-temperature" phase diagram is…

Materials Science · Physics 2007-06-24 V. B. Shirokov , Yu. I. Yuzyuk , B. Dkhil , V. V. Lemanov

The quasi 2D electron system (q2DES) that forms at the interface between LaAlO3 and SrTiO3 has attracted much attention from the oxide electronics community. One of its hallmark features is the existence of a critical LaAlO3 thickness of 4…

Materials Science · Physics 2017-08-31 D. C. Vaz , E. Lesne , H. Naganuma , E. Jacquet , J. Santamaria , A. Barthelemy , M. Bibes

The presence of oxygen vacancy, as well as ordering of vacancies plays an important role in determining the electronic, ionic and thermal transport properties of many transition metal oxide materials. Controlling the concentration of oxygen…

Mesoscale and Nanoscale Physics · Physics 2018-12-05 Xue Rui , Robert Klie

Ferroelastic domain walls (DWs) underpin key functionalities in complex oxides. In free-standing ferroic thin films, where elastic interactions are highly thickness dependent, understanding DW behaviour across length scales and external…

The structural, magnetic and dielectric properties have been investigated in 3$d$-5$d$ based double perovskite Sr$_2$FeIrO$_6$ thin films deposited by pulse laser deposition technique. To understand the effect of strain, epitaxial films are…

Strongly Correlated Electrons · Physics 2020-12-02 K. C. Kharkwal , Roshan Kumar Patel , K. Asokan , A. K. Pramanik

We report the epitaxial growth of BiFeO3 by pulsed electron deposition and the resulting crystal quality, magnetic and nanoscale switching properties. X-ray diffraction shows high quality single phase, epitaxial (001) oriented films grown…

Materials Science · Physics 2015-06-12 Hongxue Liu , Ryan Comes , Yonghang Pei , Jiwei Lu , Stuart Wolf

We present a theoretical study of electron-phonon scattering effects in thin films made of a strong topological insulator. Phonons are modelled by isotropic elastic continuum theory with stress-free boundary conditions, and the interaction…

Mesoscale and Nanoscale Physics · Physics 2012-01-26 Sébastien Giraud , Arijit Kundu , Reinhold Egger

We study the dielectric function of CuBr$_\mathrm{x}$I$_{1-\mathrm{x}}$ thin film alloys using spectroscopic ellipsometry in the spectral range between 0.7 eV to 6.4 eV, in combination with first-principles calculations based on density…

A unique polymorph of binary tungsten trioxide, the epsilon phase of WO3, has non-centrosymmetric ferroelectric structure, typically stable below -43 degree C in bulk. We have stabilized the epsilon-WO3 at room temperature (RT) and…

The optoelectronic properties of nanoscale systems such as carbon nanotubes (CNTs), graphene nanoribbons and transition metal dichalcogenides (TMDCs) are determined by their dielectric function. This complex, frequency dependent function is…

Materials Science · Physics 2021-11-10 Oisín Garrity , Alvaro Rodriguez , Niclas S. Mueller , Otakar Frank , Patryk Kusch